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The application of color centers in wide-bandgap semiconductors to nanoscale sensing and quantum information processing largely rests on our knowledge of the surrounding crystalline lattice, often obscured by the countless classes of point…

Materials Science · Physics 2022-01-17 Artur Lozovoi , Gyorgy Vizkelethy , Edward Bielejec , Carlos A. Meriles

Shallow, negatively-charged Nitrogen-Vacancy centers (NV-) in diamond have been proposed for high-sensitivity magnetometry and spin-polarization transfer applications. However, surface effects tend to favor and stabilize the less useful…

Mesoscale and Nanoscale Physics · Physics 2021-05-12 Federico Gorrini , Carla Dorigoni , Domingo Olivares-Postigo , Rakshyakar Giri , Pietro Aprà , Federico Picollo , Angelo Bifone

Nitrogen-Vacancy (NV) centers in diamond have been identified over the past few years as promising systems for a variety of applications, ranging from quantum information science to magnetic sensing. This relies on the unique optical and…

Quantum Physics · Physics 2018-12-19 I. Meirzada , Y. Hovav , S. A. Wolf , N. Bar-Gill

Although the spin properties of superficial shallow nitrogen-vacancy (NV) centers have been the subject of extensive scrutiny, considerably less attention has been devoted to studying the dynamics of NV charge conversion near the diamond…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 Siddharth Dhomkar , Harishankar Jayakumar , Pablo R. Zangara , Carlos A. Meriles

Scalable realizations of quantum network technologies utilizing the nitrogen vacancy center in diamond require creation of optically coherent NV centers in close proximity to a surface for coupling to optical structures. We create single NV…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Srivatsa Chakravarthi , Christian Pederson , Zeeshawn Kazi , Andrew Ivanov , Kai-Mei C. Fu

We report on pulsed-laser induced generation of nitrogen-vacancy (NV) centers in diamond facilitated by a solid-immersion lens (SIL). The SIL enables laser writing at energies as low as 5.8 nJ per pulse and allows vacancies to be formed…

Point defects in wide-bandgap semiconductors are emerging as versatile resources for nanoscale sensing and quantum information science but our understanding of the photo-ionization dynamics is presently incomplete. Here we use two-color…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Siddharth Dhomkar , Pablo R. Zangara , Jacob Henshaw , Carlos A. Meriles

The nitrogen-vacancy (NV) centre in diamond is emerging as a promising platform for solid-state quantum information processing and nanoscale metrology. Of interest in these applications is the manipulation of the NV charge, which can be…

The nitrogen-vacancy centre (NV) has drawn much attention for over a decade, yet detailed knowledge of the photophysics needs to be established. Under typical conditions, the NV can have two stable charge states, negative (NV-) or neutral…

Quantum Physics · Physics 2017-10-20 N. Aslam , G. Waldherr , P. Neumann , F. Jelezko , J. Wrachtrup

The fluorescent nitrogen-vacancy (NV) defect in diamond has remarkable photophysical properties, including high photostability, which allows stable fluorescence emission for hours; as a result, there has been much interest in using…

Nitrogen-vacancy (NV) centers in diamond are reliable single-photon emitters, with applications in quantum technologies and metrology. Two charge states are known for NV centers: NV$^0$ and NV$^-$, with the latter being mostly studied due…

Optics · Physics 2019-12-23 Magdalena Solà-Garcia , Sophie Meuret , Toon Coenen , Albert Polman

Optically-active spin qubits in wide-bandgap semiconductors exist in several charge states, though typically only specific charge states exhibit desirable spin or photonic properties. An understanding of how interconversion between…

Applied Physics · Physics 2024-05-03 A. A. Wood , A. Lozovoi , R. M. Goldblatt , C. A. Meriles , A. M. Martin

Charge control of color centers in semiconductors promises opportunities for novel forms of sensing and quantum information processing. Here, we articulate confocal fluorescence microscopy and magnetic resonance protocols to induce and…

Nitrogen vacancy (NV) centers in diamond exhibit long spin coherence times, optical initialization, and optical spin readout under ambient conditions, making them excellent quantum sensors. However, the conventional scheme for charge state…

The photophysics and charge state dynamics of the nitrogen vacancy (NV) center in diamond has been extensively investigated but is still not fully understood. In contrast to previous work, we find that NV$^{0}$ converts to NV$^{-}$ under…

Materials Science · Physics 2016-07-13 Peng Ji , M. V. Gurudev Dutt

The control of the charge state of nitrogen-vacancy (NV) centers in diamond is of primary importance for the stabilization of their quantum-optical properties, in applications ranging from quantum sensing to quantum computing. To this…

The negatively charged nitrogen-vacancy (NV) center in diamond is a leading solid-state quantum emitter, offering spin-photon interfaces over a wide temperature range with applications from electromagnetic sensing to bioimaging. While NV…

Control over the charge states of color centers in solids is necessary in order to fully utilize them in quantum technologies. However, the microscopic charge dynamics of deep defects in wide-bandgap semiconductors are complex, and much…

Mesoscale and Nanoscale Physics · Physics 2021-09-08 A. Gardill , I. Kemeny , M. C. Cambria , Y. Li , H. T. Dinani , A. Norambuena , J. R. Maze , V. Lordi , S. Kolkowitz

The nitrogen-vacancy (NV) center in diamond exists in different charge states with distinct photoluminescence properties, which are sensitive to the nanoscale electrochemical environment. Hence, the NV charge state is emerging as a powerful…

Mesoscale and Nanoscale Physics · Physics 2026-05-12 Patrick Voorhoeve , Hiroshi Abe , Takeshi Ohshima , Qiang Sun , Anita Quigley , Rob Kapsa , Nikolai Dontschuk , Philipp Reineck

The negatively charged nitrogen-vacancy (NV) center is one of the most significant and widely studied defects in diamond that plays a prominent role in quantum technologies. The precise engineering of the location and concentration of NV…

Materials Science · Physics 2025-03-11 Nima Ghafari Cherati , Anton Pershin , Ádám Gali
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