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We demonstrate a high-power narrow-linewidth ultraviolet (UV) laser system at 318.6 nm for direct 6S1/2-nP (n = 70 to 100) Rydberg excitation of cesium atoms. Based on commercial fiber lasers and efficient nonlinear frequency conversion…

Optics · Physics 2016-09-21 Jieying Wang , Jiandong Bai , Jun He , Junmin Wang

Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…

Optics · Physics 2018-10-24 Bachana Lomsadze , Brad. C. Smith , Steven T. Cundiff

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

We present an optical-optical double-resonance (OODR) spectrometer based on a 3.3 ${\mu}$m continuous wave pump and two cavity-enhanced probes: a frequency comb tunable in the 1.64 - 1.8 ${\mu}$m range, and a comb-referenced continuous wave…

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…

Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad…

We present a collection of double-lobed sources towards a 20 sq deg area of the Cygnus region at the northern sky, observed at 325 and 610~MHz with the Giant Metrewave Radio Telescope. The 10'' resolution achieved at 325 MHz is 5.5 times…

Astrophysics of Galaxies · Physics 2021-09-15 J. Saponara , P. Benaglia , I. Andruchow , C. H. Ishwara-Chandra , H. T. Intema

Using a turn-key Ti:sapphire femtosecond laser frequency comb, an off-the-shelf supercontinuum device, and Fabry-Perot mode filters, we report the generation of a 16 GHz frequency comb spanning a 90 nm band about a center wavelength of 566…

We demonstrate simple optical frequency combs based on semiconductor quantum well laser diodes. The frequency comb spectrum can be tailored by choice of material properties and quantum-well widths, providing spectral flexibility. Finally,…

Optics · Physics 2020-07-21 Mark Dong , Matthew W. Day , Herbert G. Winful , Steven T. Cundiff

We have developed an extreme ultraviolet (XUV) frequency comb for performing ultra-high precision spectroscopy on the many XUV transitions found in highly charged ions (HCI). Femtosecond pulses from a 100 MHz phase-stabilized near-infrared…

Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…

Optics · Physics 2009-11-13 Michael J. Thorpe , Jun Ye

Optical frequency combs based on mode-locked lasers have revolutionized many areas of science and technology, such as precision metrology, optical frequency synthesis or telecommunications. In recent years, a particular kind of frequency…

Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…

We have developed a hyperspectral imaging scheme that involves a combination of dual-comb spectroscopy and Hadamard-transform-based single-pixel imaging. The scheme enables us to obtain 12,000 hyperspectral images of amplitude and phase at…

Quantum cascade lasers (QCLs) facilitate compact optical frequency comb sources that operate in the mid-infrared and terahertz spectral regions, where many molecules have their fundamental absorption lines. Enhancing the optical bandwidth…

We demonstrate 1D simultaneous laser cooling of $^{87}$Rb and $^{85}$Rb atoms using an optical frequency comb. By adjusting the pulse repetition frequency and the offset frequency, the frequency comb spectrum is tuned to ensure that two…

Atomic Physics · Physics 2020-09-02 D. Buhin , D. Kovacic , F. Schmid , M. Kruljac , V. Vulic , T. Ban , D. Aumiler

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

While Rydberg atoms have shown tremendous potential to serve as accurate and sensitive detectors of microwaves and millimeter waves, their response is generally limited to a single narrow frequency band around a chosen microwave transition.…

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

We demonstrate a terahertz (THz) frequency comb that is flexible in terms of its frequency range and the number and spacing of comb lines. We use a combination of near-infrared laser diodes, phase modulation and opto-electronic frequency…