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Intense "blue-green" phosphorescence is commonly observed in near colourless lab-grown high-pressure high-temperature (HPHT) diamonds following optical excitation at or above the indirect bandgap. We have employed a holistic combination of…

Materials Science · Physics 2023-06-06 Jiahui Zhao , Ben L. Green , Ben G. Breeze , Mark E. Newton

Phosphorus-doped diamond is relevant for applications in sensing, optoelectronics and quantum photonics, since the unique optical properties of color centers in diamond can be combined with the n-type conductivity attained by the inclusion…

Irradiation of natural pink and brown diamond by middle-ultraviolet light (photon energy > 4.1 eV) is seen to induce anomalous fluorescence phenomena at N3 defect centres (structure N3-V). When diamonds primed in this fashion are…

Materials Science · Physics 2014-03-14 K S Byrne , J G Chapman , A N Luiten

Photoluminescence and thermally stimulated luminescence of synthetic and natural (morion and smoky) $\alpha$-quartz crystals doped with aluminum and alkali ions were studied. The photoluminescence spectrum is characterized with the main…

Materials Science · Physics 2021-09-08 A. N. Trukhin

Charge state instabilities have been a bottleneck for the implementation of solid-state spin systems and pose a major challenge to the development of spin-based quantum technologies. Here we investigate the stabilization of negatively…

We present photoluminescence studies as a function of temperature from a series of conjugated polymers and a conjugated molecule with distinctly different backbone conformations. The organic materials investigated here are: planar…

The coherence characteristics of a tin-vacancy color center in diamond are investigated through optical means including coherent population trapping between the ground state orbital levels and linewidth broadening effects. Due to the large…

The phosphorescence of boric acid at room temperature is a puzzling phenomenon subject to controversial interpretations although the role of structural defects has not yet been considered. Heat treatments of boric acid cause its…

We report on the creation and characterization of Pb-related color centers in diamond upon ion implantation and subse- quent thermal annealing. Their optical emission in photoluminescence (PL) regime consists of an articulated spectrum with…

In fluorescence spectra of nanodiamonds (NDs) synthesized at high pressure from adamantane and other organic compounds, very narrow (~1 nm) lines of unknown origin are observed in a wide spectroscopic range from ~500 to 800 nm. Here, we…

Pulsed laser excitation causes the luminescence of Nitrogen Vacancy centers in diamond to unexpectedly decrease with increasing pulse energy. This decrease is observed in both the negatively charged and neutral centers and is caused by…

Mesoscale and Nanoscale Physics · Physics 2017-12-22 Robert Chapman , Taras Plakhotnik

The nitrogen-vacancy (NV) centre in diamond is emerging as a promising platform for solid-state quantum information processing and nanoscale metrology. Of interest in these applications is the manipulation of the NV charge, which can be…

Symmetry considerations are used in presenting a model of the electronic structure and the associated dynamics of the nitrogen-vacancy center in diamond. The model accounts for the occurrence of optically induced spin polarization, for the…

Materials Science · Physics 2013-05-29 N. B. Manson , J. P. Harrison , M. J. Sellars

We implanted Fe$^+$ ions in nanodiamond (ND) powder containing negatively charged nitrogen-vacancy (NV-) centers and studied their Raman spectra and optically detected magnetic resonance (ODMR) in various applied magnetic fields with green…

In this work we use fluorescence from nitrogen-vacancy defects in diamond to detect and explore other paramagnetic defects in the diamond, such as P1 defects, which are commonly undetectable through optical detection of magnetic resonance…

Quantum Physics · Physics 2019-07-03 Nir Alfasi , Sergei Masis , Oleg Shtempluck , Eyal Buks

Biosensing based on optically trapped fluorescent nanodiamonds potentially allows to resolve biochemical processes inside living cells at a desired intracellular location. Towards this goal, we investigate near infrared (NIR) laser…

We report on measurements of the photoluminescence (PL) properties of single nitrogen-vacancy (NV) centers in diamond at temperatures between 4-300 K. We observe a strong reduction of the PL intensity and spin contrast between ca. 10-100 K…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Stefan Ernst , Patrick J. Scheidegger , Simon Diesch , Luca Lorenzelli , Christian L. Degen

The nitrogen-vacancy (NV) center is a photoluminescent defect in diamond that exists in different charge states, NV$^-$ and NV$^0$, that are sensitive to the NV's nanoscale environment. Here, we show that photoluminescence (PL) from NV…

The nitrogen-vacancy centre (NV) has drawn much attention for over a decade, yet detailed knowledge of the photophysics needs to be established. Under typical conditions, the NV can have two stable charge states, negative (NV-) or neutral…

Quantum Physics · Physics 2017-10-20 N. Aslam , G. Waldherr , P. Neumann , F. Jelezko , J. Wrachtrup

A comprehensive photoluminescence and mechanoluminescence analysis of ZnS:Mn2+ nano-phosphor with zinc blende structure is presented. The sample containing quantum dot-sized nanocrystallites were synthesized by the chemical precipitation…

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