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The interplay of dynamical nuclear polarization (DNP) and leakage current through a double quantum dot in the spin-blockade regime is analyzed. A finite DNP is built up due to a competition between hyperfine (HF) spin-flip transitions and…

Mesoscale and Nanoscale Physics · Physics 2013-07-30 Anders Mathias Lunde , Carlos López-Monís , Ioanna A. Vasiliadou , Luis L. Bonilla , Gloria Platero

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

In heavy atoms and ions, nuclear structure effects are significantly enhanced due to the overlap of the electron wave functions with the nucleus. This overlap rapidly increases with the nuclear charge $Z$. We study the energy level shifts…

Atomic Physics · Physics 2021-03-17 V. V. Flambaum , I. B. Samsonov , H. B. Tran Tan , A. V. Viatkina

Polarization transfers from an electron spin to a nuclear spin are essential for various physical tasks, such as dynamic nuclear polarization in nuclear magnetic resonance and quantum state transformations on hybrid electron-nuclear spin…

Quantum Physics · Physics 2015-11-11 Haidong Yuan , Robert Zeier , Nikolas Pomplun , Steffen J. Glaser , Navin Khaneja

Spin polarized states in nuclear matter with an effective nucleon-nucleon interaction are studied for a wide range of isospin asymmetries and densities. Based on a Fermi liquid theory, it is shown that there are a few possible scenarios of…

Nuclear Theory · Physics 2007-09-22 A. A. Isayev

Optically-pumped color centers in semiconductor powders can potentially induce high levels of nuclear spin polarization in surrounding solids or fluids at or near ambient conditions, but complications stemming from the random orientation of…

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic…

We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

Spontaneous nuclear polarization is predicted in double quantum dots in the spin-blocked electron transport regime. The polarization results from an instability of the zero-polarization state when singlet and triplet electron energy levels…

Mesoscale and Nanoscale Physics · Physics 2010-08-23 M. S. Rudner , L. S. Levitov

Optical spin pumping of color centers in diamond is presently attracting broad interest as a platform for dynamic nuclear polarization at room temperature, but the mechanisms involved in the generation and transport of polarization within…

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

Quantum Physics · Physics 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

In dissolution-dynamic nuclear polarization, nuclear spins are hyperpolarized at cryogenic temperatures using radicals and microwave irradiation. The hyperpolarized solid is dissolved with hot solvent and the solution is transferred to a…

Instrumentation and Detectors · Physics 2019-06-20 Karel Kouřil , Hana Kouřilová , Samuel Bartram , Malcolm H. Levitt , Benno Meier

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

A theory of dynamic polarization of the nuclear spin system via optically-oriented charge carriers in lead halide perovskites is developed and compared with the experiments performed on a FA$_{0.9}$Cs$_{0.1}$PbI$_{2.8}$Br$_{0.2}$ crystal.…

Mesoscale and Nanoscale Physics · Physics 2026-02-10 Mladen Kotur , Pavel S. Bazhin , Kirill V. Kavokin , Nataliia E. Kopteva , Dmitri R. Yakovlev , Dennis Kudlacik , Manfred Bayer

Isolated electron spins in semiconductor nanostructures are promising qubit candidates for a solid state quantum computer, There have seen truly impressive experimental progresses in the study of single spins in the past two years. In this…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Changxue Deng , Xuedong Hu

The nuclear spin state of a phosphorus donor ($^{31}$P) in isotopically enriched silicon-28 is an excellent host to store quantum information in the solid state. The spin's insensitivity to electric fields yields a solid-state qubit with…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 Guilherme Tosi , Fahd A. Mohiyaddin , Stefanie Tenberg , Arne Laucht , Andrea Morello

We consider nuclear spin dynamics in a two-electron double dot system near the intersection of the electron spin singlet $S$ and the lower energy component $T_{+}$ of the spin triplet. The electron spin interacts with nuclear spins and is…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Arne Brataas , Emmanuel I. Rashba

Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…

Quantum Physics · Physics 2026-04-21 Sundaresan Jayanthi , Adonis Lupulescu , Julia Grinshtein , Lucio Frydman