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It is usually considered that the spectrum of an optical cavity coupled to an atomic medium does not exhibit a normal-mode splitting unless the system satisfies the strong coupling condition, meaning the Rabi frequency of the coherent…

Quantum Physics · Physics 2017-01-06 Y. -H. Lien , G. Barontini , M. Scheucher , M. Mergenthaler , J. Goldwin , E. A. Hinds

We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultra-strong light-matter coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency and the…

Other Condensed Matter · Physics 2009-11-11 Cristiano Ciuti , Iacopo Carusotto

The prospect of controlling chemical reactivity using frequency-tunable optical microcavities has materialized over the past decade, evolving into a fascinating yet challenging new field of polaritonic chemistry, a multidisciplinary domain…

Chemical Physics · Physics 2025-10-07 Yaling Ke , Jakob Assan

Strong coupling of molecules to the vacuum field of micro cavities can modify the potential energy surfaces opening new photophysical and photochemical reaction pathways. While the influence of laser fields is usually described in terms of…

Quantum Physics · Physics 2016-02-08 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

The strong interaction of individual quantum emitters with resonant cavities is of fundamental interest for understanding light matter interactions. Plasmonic cavities hold the promise of attaining the strong coupling regime even under…

Optics · Physics 2016-06-28 Kotni Santhosh , Ora Bitton , Lev Chuntonov , Gilad Haran

A single quantum emitter can possess a very strong intrinsic nonlinearity, but its overall promise for nonlinear effects is hampered by the challenge of efficient coupling to incident photons. Common nonlinear optical materials, on the…

We investigate the possibility of achieving the strong coupling regime of cavity quantum electrodynamics using rare earth ions as impurities in monolithic optical resonators. We conclude that due to the weak oscillator strengths of the rare…

Quantum Physics · Physics 2015-05-13 D. L. McAuslan , J. J. Longdell , M. J. Sellars

The way molecules absorb, transfer, and emit light can be dramatically modified by coupling them to optical cavities. The extent of the modification is often defined by the cavity-molecule coupling strength. Evaluating this coupling…

Optics · Physics 2020-09-21 Adarsh B Vasista , William L Barnes

In the regime of strong coupling between molecular excitons and confined optical modes, the intra-molecular degrees of freedom are profoundly affected, leading to a reduced vibrational dressing of polaritons compared to bare electronically…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Javier del Pino , Florian A. Y. N. Schröder , Alex W. Chin , Johannes Feist , Francisco J. Garcia-Vidal

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

The experimental observation of quantum phenomena in strongly correlated many particle systems is difficult because of the short length- and timescales involved. Obtaining at the same time detailed control of individual constituents appears…

Quantum Physics · Physics 2007-05-23 Michael J. Hartmann , Fernando G. S. L. Brandao , Martin B. Plenio

Recent experiments of chemical reactions in optical cavities have shown great promise to alter and steer chemical reactions but still remain poorly understood theoretically. In particular the origin of resonant effects between the cavity…

Chemical Physics · Physics 2022-12-21 Derek S. Wang , Johannes Flick , Susanne F. Yelin

Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial…

We study the emission from a molecular photonic cavity formed by two proximal photonic crystal defect cavities containing a small number (<3) of In(Ga)As quantum dots. Under strong excitation we observe photoluminescence from the bonding…

The strong coupling between two subsystems consisting of quantum emitters and photonic modes, at which the level splitting of mixed quantum states occurs, has been a central subject of quantum physics and nanophotonics due to various…

Optics · Physics 2021-06-30 Renming Liu , Yi-Cong Yu , Xue-Hua Wang

This study investigates the dynamic behavior of polaritons in an optical cavity containing one million molecules, emphasizing the influence of molecular rotation and level disorder on the coupling between molecules and photons. Through…

Optics · Physics 2024-02-22 Wei Liu , Jingqi Chen , Wenjie Dou

We propose a realizable architecture using one-dimensional transmission line resonators to reach the strong coupling limit of cavity quantum electrodynamics in superconducting electrical circuits. The vacuum Rabi frequency for the coupling…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. M. Girvin , Ren-Shou Huang , Alexandre Blais , Andreas Wallraff , R. J. Schoelkopf

Physical and chemical properties of materials can be modified by a resonant optical mode. Such recent demonstrations have mostly relied on a planar cavity geometry, others have relied on a plasmonic resonator. However, the combination of…

Recent technological developments have made it increasingly easy to access the non-perturbative regimes of cavity quantum electrodynamics known as ultra or deep strong coupling, where the light-matter coupling becomes comparable to the bare…

Quantum Physics · Physics 2018-05-22 Carlos Sánchez Muñoz , Franco Nori , Simone De Liberato

Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of "single-photon strong…

Quantum Physics · Physics 2022-04-01 Javier Argüello-Luengo , Darrick E. Chang