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The swelling equilibrium of Olympic gels, which are composed of entangled cyclic polymers, is studied by Monte Carlo Simulations. In contrast to chemically crosslinked polymer networks, we observe that Olympic gels made of chains with a…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Jakob Fischer , Marco Werner , Jens-Uwe Sommer

Topological constraints (TCs) between polymers determine the behaviour of complex fluids such as creams, oils and plastics. Most of the polymer solutions used every day life employ linear chains; their behaviour is accurately captured by…

Soft Condensed Matter · Physics 2020-10-07 Fabio Landuzzi , Takenobu Nakamura , Davide Michieletto , Takahiro Sakaue

We consider the swelling kinetics of layered structures. We focus on the case of triblock copolymer mesogels, although our results are applicable to other layered structures including clays. We assume the mesogels are swollen by a solvent…

Condensed Matter · Physics 2007-05-23 C. -M. Chen , F. C. MacKintosh , D. R. M. Williams

We present results of Monte Carlo study of the monomer-monomer correlation functions, static structure factor and asphericity characteristics of a single homopolymer in the coil and globular states for three distinct architectures of the…

Soft Condensed Matter · Physics 2009-11-07 Edward G. Timoshenko , Yuri A. Kuznetsov , Ronan Connolly

The flow behaviors of polymer melt composed of short chains with ten beads between parallel plates are simulated by using a hybrid method of molecular dynamics and computational fluid dynamics. Three problems are solved: creep motion under…

Soft Condensed Matter · Physics 2014-01-20 Shugo Yasuda , Ryoichi Yamamoto

When a gel absorbs solvent from surrounding, stress field is created in the gel, and this causes complex dynamics of the swelling behavior. Here we study this effect for disk-shaped gel by rigorously solving the diffusio-mechanical coupling…

Soft Condensed Matter · Physics 2021-05-17 Xingkun Man , Masao Doi

We study a classical model of thermally fluctuating polymers confined to two dimensions, experiencing a grooved periodic potential, and subject to pulling forces both along and transverse to the grooves. The equilibrium polymer…

Soft Condensed Matter · Physics 2023-01-12 Abhijeet Melkani , Alexander Patapoff , Jayson Paulose

Novel kinetic models for both Dumbbell-like and rigid-rod like polymers are derived, based on the probability distribution function $f(t, x, n, \dot n)$ for a polymer molecule positioned at $x$ to be oriented along direction $n$ while…

Analysis of PDEs · Mathematics 2014-04-08 Pierre Degond , Hailiang Liu

The research is important for a molecular theory of liquid and has a wide interest as an example solving the problem when dynamic parameters of systems can be indirectly connected with their equilibrium properties. In frameworks of the…

Disordered Systems and Neural Networks · Physics 2007-05-23 Andrei N. Yakunin

We propose a nonlinear extension of the standard tube model for semidilute solutions of freely-sliding semiflexible polymers. Non-affine filament deformations at the entanglement scale, the renormalisation of direct interactions by thermal…

Soft Condensed Matter · Physics 2008-10-01 Pablo Fernandez , Steffen Grosser , Klaus Kroy

An exactly solvable family of models describing the wrinkling of substrate-supported inextensible elastic rings under compression is identified. The resulting wrinkle profiles are shown to be related to the buckled states of an unsupported…

Soft Condensed Matter · Physics 2022-08-30 Benjamin Foster , Nicolás Verschueren , Edgar Knobloch , Leonardo Gordillo

We present results from a systematic numerical study of decaying turbulence in a dilute polymer solution by using a shell-model version of the FENE-P equations. Our study leads to an appealing definition of drag reduction for the case of…

Statistical Mechanics · Physics 2009-11-10 Chirag Kalelkar , Rama Govindarajan , Rahul Pandit

The Kremer-Grest (KG) polymer model is a standard model for studying generic polymer properties in Molecular Dynamics simulations. It owes its popularity to its simplicity and computational efficiency, rather than its ability to represent…

Soft Condensed Matter · Physics 2020-03-16 Ralf Everaers , Hossein Ali Karimi-Varzaneh , Nils Hojdis , Frank Fleck , Carsten Svaneborg

We study the quantum dynamics of a suddenly released beam of particles using a background independent (polymer) quantization scheme. We show that, in the first order of approximation, the low-energy polymer distribution converges to the…

Quantum Physics · Physics 2015-06-22 A. Martín-Ruiz

We present a computationally efficient multiscale method for preparing equilibrated, isotropic long chain model polymer melts. As an application we generate Kremer-Grest melts of $1000$ chains with $200$ entanglements and $25000$-$2000$…

Soft Condensed Matter · Physics 2023-02-15 Carsten Svaneborg , Ralf Everaers

We study model near-critical polymer gelling systems made of gluten proteins dispersions stabilized at different distances from the gel point. We impose different shear rates and follow the time evolution of the stress. For sufficiently…

Soft Condensed Matter · Physics 2024-07-18 Ameur Louhichi , Marie-Hélène Morel , Laurence Ramos , Amélie Banc

Glassy polymers show strain hardening: at constant extensional load, their flow first accelerates, then arrests. Recent experiments under such loading have found this to be accompanied by a striking dip in the segmental relaxation time.…

Soft Condensed Matter · Physics 2015-06-11 S. M. Fielding , R. L. Moorcroft , R. G. Larson , M. E. Cates

The Euler buckling of rods is a long-studied mechanical instability, and it remains relevant to this day, as the constituent components in many biological and physical systems are linear polymers, such as microtubules or carbon nanotubes.…

Statistical Mechanics · Physics 2026-05-22 Richard Huang , David R. Nelson , Suraj Shankar

We use dissipative particle dynamics (DPD) simulations to study the effect of shear on domain morphology and kinetics of microphase separating critical diblock copolymer (BCP) bulk melts. The melt is confined within two parallel solid walls…

Soft Condensed Matter · Physics 2022-09-21 Ashish Kumar Singh , Awaneesh Singh

We study the dynamics of a single polymer subject to thermal fluctuations in a linear shear flow. The polymer is modeled as a finitely extendable nonlinear elastic FENE dumbbell. Both orientation and elongation dynamics are investigated…

Chaotic Dynamics · Physics 2015-06-26 A. Celani , A. Puliafito , K. Turitsyn
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