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The motion of an artificial micro-scale swimmer that uses a chemical reaction catalyzed on its own surface to achieve autonomous propulsion is fully characterized experimentally. It is shown that at short times, it has a substantial…

We introduce a novel mesoscopic computational model based on a multiphase-multicomponent lattice Boltzmann method for the simulation of self-phoretic particles in the presence of liquid-liquid interfaces. Our model features fully resolved…

Soft Condensed Matter · Physics 2022-06-22 Lucas Palacios , Andrea Scagliarini , Ignacio Pagonabarraga

Thermally induced particle flow in a charged colloidal suspension is studied in a fluid-mechanical approach. The force density acting on the charged boundary layer is derived in detail. From Stokes' equation with no-slip boundary conditions…

Soft Condensed Matter · Physics 2014-01-31 S. Fayolle , T. Bickel , A. Würger

The field of synthetic active matter has, thus far, been led by efforts to create point-like, isolated (yet interacting) self-propelled objects (\emph{e.g.} colloids, droplets, microrobots) and understanding their collective dynamics. The…

Soft Condensed Matter · Physics 2024-08-06 Manoj Kumar , Aniruddh Murali , Arvin Gopal Subramaniam , Rajesh Singh , Shashi Thutupalli

In this work we derive and analyze coarse-grained descriptions of self-propelled particles with selective attraction-repulsion interaction, where individuals may respond differently to their neighbours depending on their relative state of…

Soft Condensed Matter · Physics 2016-05-02 Robert Grossmann , Lutz Schimansky-Geier , Pawel Romanczuk

Self-diffusiophoretic particles exploit local concentration gradients of a solute species in order to self-propel at the micron scale. While an isolated chemically- and geometrically-isotropic particle cannot swim, we show that it can…

Soft Condensed Matter · Physics 2018-06-12 Akhil Varma , Thomas D. Montenegro-Johnson , Sebastien Michelin

Phoretic swimmers are a class of artificial active particles that has received significant attention in recent years. By making use of self-generated gradients (e.g. in temperature, electric potential or some chemical product) phoretic…

Soft Condensed Matter · Physics 2018-10-23 Maria Tătulea-Codrean , Eric Lauga

The penetrable-sphere model has been introduced in the literature to describe the peculiar thermodynamic behavior of some colloidal systems. In this model the interaction potential is $\phi(r)=\epsilon>0$ if the two spheres are overlapped…

Statistical Mechanics · Physics 2014-11-10 Andres Santos

We use a hydrodynamic reciprocal approach to phoretic motion to derive general expressions for the electrophoretic and thermophoretic mobility of weakly charged colloids in aqueous electrolyte solutions. Our approach shows that phoretic…

Soft Condensed Matter · Physics 2018-10-08 Jérôme Burelbach , Holger Stark

Active particles driven by a chemical reaction are the subject of intense research to date due to their rich physics, being intrinsically far from equilibrium, and their multiple technological applications. Recent attention in the field is…

Soft Condensed Matter · Physics 2023-10-02 Dolachai Boniface , Sergi G. Leyva , Ignacio Pagonabarraga , Pietro Tierno

The self-diffusion process of a hard sphere fluid confined by two parallel plates separated by a distance on the order of the particle diameter is studied. The starting point is a closed kinetic equation for the distribution function that…

Statistical Mechanics · Physics 2025-10-24 Manuel Mayo , María Isabel García de Soria , Pablo Maynar , José Javier Brey

Colloidal motors without moving parts can be propelled by self-diffusiophoresis, coupling molecular concentration gradients generated by surface chemical reactions to the velocity slip between solid Janus particles and the surrounding fluid…

Statistical Mechanics · Physics 2021-02-08 Pierre Gaspard , Raymond Kapral

Microscopic dynamical aspects of the propulsion of nanomotors by self-phoretic mechanisms are considered. Propulsion by self-diffusiophoresis relies on the mechanochemical coupling between the fluid velocity field and the concentration…

Statistical Mechanics · Physics 2018-01-04 Pierre Gaspard , Raymond Kapral

In this paper we develop a field-theoretic description for run and tumble chemotaxis, based on a density functional description of crystalline materials modified to capture orientational ordering. We show that this framework, with its…

Soft Condensed Matter · Physics 2021-03-10 Purba Chatterjee , Nigel Goldenfeld

We consider the efficiency of self-phoretic colloidal particles (swimmers) as a function of the heterogeneity in the surface reaction rate. The set of fluid, species, and electrostatic continuity equations is solved analytically using a…

Soft Condensed Matter · Physics 2016-06-22 Patrick Kreissl , Christian Holm , Joost de Graaf

Active drops emit/absorb chemical solutes, whose concentration gradients cause interfacial flows driving their own transport and the propulsion of the droplet. Such non-linear coupling enables active drops to achieve directed…

Fluid Dynamics · Physics 2022-12-01 Nikhil Desai , Sebastien Michelin

Phoretic mechanisms, whereby gradients of chemical solutes induce surface-driven flows, have recently been used to generate directed propulsion of patterned colloidal particles. When the chemical solutes diffuse slowly, an instability…

Fluid Dynamics · Physics 2019-12-18 Sébastien Michelin , Simon Game , Eric Lauga , Eric Keaveny , Demetrios Papageourgiou

Janus phoretic colloids (JPs) self-propel as a result of self-generated chemical gradients and exhibit spontaneous nontrivial dynamics within phoretic suspensions, on length scales much larger than the microscopic swimmer size. Such…

Fluid Dynamics · Physics 2021-11-29 Tullio Traverso , Sebastien Michelin

Chemically-active colloids modify the concentration of chemical solutes surrounding them in order to self-propel. In doing so, they generate long-ranged hydrodynamic flows and chemical gradients that modify the trajectories of other…

Fluid Dynamics · Physics 2021-11-29 Francisco Rojas-Perez , Blaise Delmotte , Sebastien Michelin

Self-phoretic Janus particles move by inducing -- via non-equilibrium chemical reactions occurring on their surfaces -- changes in the chemical composition of the solution in which they are immersed. This process leads to gradients in…

Soft Condensed Matter · Physics 2018-01-30 W. E. Uspal , M. N. Popescu , M. Tasinkevych , S. Dietrich