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Recently, based on the phase-field modeling, it was predicted that Hf1-xZrxO2 (HZO) exhibits the morphotropic phase boundary (MPB) in its compositional phase diagram. Here, we investigate the effect of structural changes between tetragonal…

Materials Science · Physics 2021-05-05 Alireza Kashir , Hyunsang Hwang

A first-principles-derived approach is used to study structural, piezoelectric and dielectric properties of Pb(Zr_{1-x}Ti_{x})O_{3} (PZT) solid solutions near the morphotropic phase boundary at low temperature. Three ferroelectric phases…

Materials Science · Physics 2007-05-23 L. Bellaiche , A. Garcia , David Vanderbilt

Many ferroelectric solid solutions exhibit enhanced electro-mechanical properties at the morphotropic boundary separating two phases with different orientations of polarization. The mechanism of properties enhancement is associated with…

Materials Science · Physics 2015-05-19 Dragan Damjanovic

A new lead-free (1-x)Li0.12Na0.88NbO3-xBaTiO3 (0 to x to 40) piezoelectric ceramics have been prepared using conventional ceramics processing route. Structural analysis revealed an existence of morphotropic phase boundary (MPB), separating…

Materials Science · Physics 2014-12-24 Supratim Mitra , Ajit R. Kulkarni

Ceramic solid solutions of PbZr(1-x)TixO3 (PZT) with compositions of about x= 0.50 are well-known for their extraordinarily large piezoelectric responses. The latter are highly anisotropic, and it was recently shown that, for the…

Materials Science · Physics 2007-05-23 B. Noheda , D. E. Cox

Strong piezoelectricity in the perovskite-type PbZr(1-x)TixO3 (PZT) and Pb(Zn1/3Nb2/3)O3-PbTiO3 (PZN-PT) systems is generally associated with the existence of a morphotropic phase boundary (MPB) separating regions with rhombohedral and…

Materials Science · Physics 2009-11-07 D. E. Cox , B. Noheda , G. Shirane , Y. Uesu , K. Fujishiro , Y. Yamada

Piezoelectric PZT solid solutions were studied as a function of pressure and temperature. Moderate pressure is found to induce phase transitions to monoclinic phases (Cm,Cc) for Ti-rich PZT, which are the same ferroelectric phases…

Materials Science · Physics 2009-05-14 Jérôme Rouquette , Julien Haines , Véronique Bornand , Philippe Papet

Atomistic control of phase boundaries is crucial for optimizing the functional properties of solid-solution ferroelectrics, yet their microstructural mechanisms remain elusive. Here, we harness machine-learning-driven molecular dynamics to…

Materials Science · Physics 2025-05-09 Weiru Wen , Fan-Da Zeng , Ben Xu , Bi Ke , Zhipeng Xing , Hao-Cheng Thong , Ke Wang

The structural evolution of the strain-driven morphotropic phase boundary (MPB) in BiFeO3 films has been investigated using synchrotron x-ray diffractometry in conjunction with scanning probe microscopy. Our results demonstrate the…

In piezoelectric ceramics the changes in the phase stabilities versus stress and temperature in the vicinity of the phase boundary play a central role. The present study was dedicated to the classical piezoelectric, lead-zirconate-titanate…

Materials Science · Physics 2015-06-04 J. Frantti , Y. Fujioka , J. Zhang , S. Wang , S. C. Vogel , R. M. Nieminen , A. M. Asiri , Y. Zhao , A. Y. Obaid

The contributory mechanisms associated with high piezoelectric response in piezoelectric ceramics have been examined by in-situ electric field dependent high energy synchro x-ray diffraction study. A comparative study of electric field…

Materials Science · Physics 2015-08-25 Lalitha K. V. , Chris M. Fancher , Jacob L. Jones , Rajeev Ranjan

The electromechanical response of PbZr0.52Ti0.48O3 (PZT) near the morphotropic phase boundary (MPB) is strongly influenced by crystallographic texture and residual stress, both of which affect domain switching behavior. While these effects…

Materials Science · Physics 2025-05-19 Saujatya Mandal , Debashish Das

The symmetry was examined using neutron diffraction method on Pb(Zn1/3Nb2/3)O3 -9%PbTiO3 (PZN/9PT) which has a composition at the morphotropic phase boundary (MPB) between Pb(Zn1/3Nb2/3)O3 and PbTiO3. The results were compared with those of…

Properties of Pb(Zr_{1-x}Ti_x)O_3 (PZT) for compositions x near the morphotropic phase boundary and under an electric field are simulated using an ab-initio based approach. Applying an electric field of [111] orientation to tetragonal PZT…

Materials Science · Physics 2009-11-07 L. Bellaiche , A. Garcia , David Vanderbilt

The novel strain-driven morphotropic phase boundary (MPB) in highly-strained BiFeO3 thin film is featured by ordered mixed phase nanodomains (MPNs). Through scanning probe microscopy and synchrotron X-ray diffraction, eight structural…

Materials Science · Physics 2012-03-01 Lu You , Zuhuang Chen , Xi Zou , Hui Ding , Weigang Chen , Lang Chen , Guoliang Yuan , Junling Wang

We observed that electric field induces phase transition from tetragonal to rhombohedral in polycrystalline morphotropic lead zirconate titanate (PZT) films, as reported in 2011 for bulk PZT. Moreover, we evidenced that this field-induced…

Materials Science · Physics 2015-01-27 V Kovacova , N Vaxelaire , G Le Rhun , P Gergaud , T Schmitz-Kempen , E Defay

Solid solution BiFe1-xCoxO3 shows anti-ferromagnetic order and pyroelectric order, simultaneously. It has been known that BiFe1-xCoxO3 exhibits a structural phase transition between monoclinic and tetragonal phases as x increases. This…

Materials Science · Physics 2021-12-15 Hiroshi Katsumoto , Kunihiko Yamauchi , Tamio Oguchi

The coexisting rhombohedral-like (R', MA) and tetragonal-like (T', MC) monoclinic phases in compressively strained bismuth ferrite thin films exhibit exceptional piezoelectric and magnetic properties. While previous studies have largely…

Physically parallel to ferroelectric morphotropic phase boundary, a phase boundary separating two ferromagnetic phase of different crystallographic symmetries was found in TbxDy1-xCo2. High-resolution synchrotron XRD has been carried out to…

Materials Science · Physics 2013-04-26 Dongyan Zhang , Sen Yang , Pangpang Wang , Yu Wang , Jieqiong Wang , Xiaoping Song

Multiferroic particulate composites have been fabricated by taking the morphotropic phase boundary composition of ferroelectric phase Bi(Ni1/2Ti1/2)O3-PbTiO3 and magnetic phase (Ni,Zn)Fe2O4. The ferroelectric phase has coexisting monoclinic…

Materials Science · Physics 2018-08-06 Rishikesh Pandey , Uma Shankar , Sher Singh Meena , Akhilesh Kumar Singh