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We report heat capacity measurements of SrCu$_2$(BO$_3$)$_2$ under high pressure along with simulations of relevant quantum spin models and map out the $(P,T)$ phase diagram of the material. We find a first-order quantum phase transition…

A Muon Spin Rotation ($\mu$+SR) study was conducted to investigate the magnetic properties of SrCu2(BO3)2 (SCBO) as a function of temperature/pressure. Measurements in zero field and transverse field confirm the absence of long range…

The layered material SrCu$_2$(BO$_3$)$_2$ has long been studied because of its fascinating physics in a magnetic field and under pressure. Many of its properties are remarkably well described by the Shastry-Sutherland model (SSM) - a…

Strongly Correlated Electrons · Physics 2023-10-04 Patrick C. G. Vlaar , Philippe Corboz

Magnetic and vibrational excitations in SrCu$_2$(BO$_3$)$_2$ are studied using Raman spectroscopy at hydrostatic pressures up to 34 kbar and temperatures down to 2.6 K. The frequency of a particular optical phonon, the so-called pantograph…

Strongly Correlated Electrons · Physics 2020-05-06 Simon Bettler , Lena Stoppel , Zewu Yan , Severian Gvasaliya , Andrey Zheludev

Using density-functional theory (DFT) band-structure calculations, we study the crystal structure, the lattice dynamics, and the magnetic interactions in the Shastry-Sutherland magnet SrCu$_2$(BO$_3$)$_2$ under pressure, concentrating on…

Strongly Correlated Electrons · Physics 2020-06-22 Danis I. Badrtdinov , Alexander A. Tsirlin , Vladimir V. Mazurenko , Frédéric Mila

The Shastry-Sutherland model, which consists of a set of spin 1/2 dimers on a 2-dimensional square lattice, is simple and soluble, but captures a central theme of condensed matter physics by sitting precariously on the quantum edge between…

Strongly Correlated Electrons · Physics 2012-02-20 S. Haravifard , A. Banerjee , J. C. Lang , G. Srajer , D. M. Silevitch , B. D. Gaulin , H. A. Dabkowska , T. F. Rosenbaum

Motivated by the intriguing properties of the Shastry-Sutherland compound SrCu2(BO3)2 under pressure, with a still debated intermediate plaquette phase appearing at around 20 kbar and a possible deconfined critical point at higher pressure…

We report results of nuclear magnetic resonance (NMR) experiments in SrCu2(BO3)2, a quasi two-dimensional spin system with a singlet ground state. When magnetic field is applied along the c-axis, each of the quadrupole split Cu resonance…

Strongly Correlated Electrons · Physics 2013-03-05 K. Kodama , J. Yamazaki , M. Takigawa , H. Kageyama , K. Onizuka , Y. Ueda

We calculate the electron spin resonance (ESR) spectra of the quasi-two-dimensional dimer spin liquid SrCu2(BO3)2 as a function of magnetic field B. Using the standard Lanczos method, we solve a Shastry-Sutherland Hamiltonian with…

Other Condensed Matter · Physics 2009-11-10 S. El Shawish , J. Bonca , C. D. Batista , I. sega

Inelastic neutron scattering profiles of spin waves in the dilute quasi-one-dimensional Ising-like antiferromagnet CsCo_{0.83}Mg_{0.17}Br_3 have been investigated. Calculations of S^{xx}(Q,omega), based on an effective spin Hamiltonian,…

Condensed Matter · Physics 2009-11-07 Y. S. Yang , F. Marsiglio , M. Madsen , B. D. Gaulin , R. B. Rogge , J. A. Fernandez-Baca

We present magnetic torque measurements on the Shastry-Sutherland quantum spin system SrCu$_2$(BO$_3$)$_2$ in fields up to 31 T and temperatures down to 50 mK. A new quantum phase is observed in a 1 T field range above the 1/8 plateau, in…

Strongly Correlated Electrons · Physics 2008-04-01 F. Levy , I. Sheikin , C. Berthier , M. Horvatic , M. Takigawa , H. Kageyama , T. Waki , Y. Ueda

We report results of 11B NMR and susceptibility measurements on the quasi 2D frustrated dimer spin system SrCu2(BO3)2 under high pressure. At 2.4 GPa and in a magnetic field of 7 T, NMR lines split with decreasing temperature in two steps.…

Strongly Correlated Electrons · Physics 2009-11-13 Takeshi Waki , Koichi Arai , Masashi Takigawa , Yuta Saiga , Yoshiya Uwatoko , Hiroshi Kageyama , Yutaka Ueda

The orthogonal dimer structure in the SrCu2(BO3)2 spin-1/2 magnet provides a realization of the Shastry-Sutherland model. Using a dimer-product variational wave function, we map out the phase diagram of the Shastry-Sutherland model…

Strongly Correlated Electrons · Physics 2015-03-17 Judit Romhanyi , Keisuke Totsuka , Karlo Penc

The study of interacting spin systems is of fundamental importance for modern condensed matter physics. On frustrated lattices, magnetic exchange interactions cannot be simultaneously satisfied, and often give rise to competing exotic…

We report the observation of magnetic superstructure in a magnetization plateau state of SrCu2(BO3)2, a frustrated quasi-two-dimensional quantum spin system. The Cu and B nuclear magnetic resonance (NMR) spectra at 35 mllikelvin indicate an…

Strongly Correlated Electrons · Physics 2009-11-07 K. Kodama , M. Takigawa , M. Horvatic , C. Berthier , H. Kageyama , Y. Ueda , S. Miyahara , F. Becca , F. Mila

We use a variety of series expansion methods at both zero and finite temperature to study an antiferromagnetic Heisenberg spin model proposed recently by Miyahara and Ueda for the quasi two-dimensional material SrCu$_2$(BO$_3$)$_2$. We…

Strongly Correlated Electrons · Physics 2009-10-31 Zheng Weihong , C. J. Hamer , J. Oitmaa

We study an extended Shastry-Sutherland model for SrCu_2(BO_3)_2 and analyze the low lying parts of the energy spectrum by means of a perturbative unitary transformation based on flow equations. The derivation of the 1-magnon dispersion…

Strongly Correlated Electrons · Physics 2016-04-20 Christian Knetter , Alexander Buehler , Erwin Mueller-Hartmann , Goetz S. Uhrig

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

High-pressure and high-field electron spin resonance (ESR) measurements have been performed on a single crystal of the orthogonal-dimer spin system SrCu$_{2}$(BO$_{3}$)$_{2}$. With frequencies below 1 THz, ESR signals associated with…

Strongly Correlated Electrons · Physics 2018-02-21 Takahiro Sakurai , Yuki Hirao , Keigo Hijii , Susumu Okubo , Hitoshi Ohta , Yoshiya Uwatoko , Kazutaka Kudo , Yoji Koike

The magnetic interactions in the antiferromagnetic (AFM) Dirac semimetal candidate SrMnSb$_2$ are investigated using \textit{ab initio} linear response theory and inelastic neutron scattering (INS). Our calculations reveal that the first…

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