Related papers: Free-electron coupling to surface polaritons media…
Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…
Free-electron beams serve as uniquely versatile probes of microscopic structure and composition, and have repeatedly revolutionized atomic-scale imaging, from solid-state physics to structural biology. Over the past decade, the manipulation…
Surface Plasmon Polaritons (SPP) are exploited due to their intriguing properties for photonic circuits fabrication and miniaturization, for surface enhanced spectroscopies and imaging beyond the diffraction limit. However, the excitation…
Exciton-polaritons (EPs) are part-light part-matter quasiparticles that combine large exciton-mediated nonlinearities with long-range coherence, ideal for energy harvesting and nonlinear optics. Optimizing EPs for these applications is…
The inelastic interaction between flying particles and optical nanocavities gives rise to entangled states in which some excitations of the latter are paired with changes in the energy or momentum of the former. In particular, entanglement…
Semiconductor nanoparticles and nanostructures in the strong coupling regime exhibit an intriguing energy scale in the optical frequencies, which is specified by the Rabi splitting between the upper and lower exciton-polariton states.…
Electron microscopy techniques such as electron energy-loss spectroscopy (EELS) facilitate the spatio-spectral characterization of plasmonic nanostructures. In this work, a time-dependent perspective is presented, which significantly…
Surface plasmon polaritons (SPPs) are central to application areas such as sensing, energy harvesting, and nanoscale optics, and are typically excited via spatial structuring -- an approach lacking dynamic control. We demonstrate that…
Spatial modulation of electron beams is an essential tool for various applications such as nanolithography and imaging, yet its implementations are severely limited and inherently non-tunable. Conversely, light-driven electron spatial…
Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here we use longitudinally polarized light…
Manipulating the spin polarization of electron beams using light is highly desirable but exceedingly challenging, as the approaches proposed in previous studies using free-space light usually require enormous laser intensities. Here, we…
We exploit free-space interactions between electron beams and tailored light fields to imprint on-demand phase profiles on the electron wave functions. Through rigorous semiclassical theory involving a quantum description of the electrons,…
Surface plasmon-polaritons have recently attracted renewed interest in the scientific community for their potential in sub-wavelength optics, light generation and non-destructive sensing. Given that they cannot be directly excited by freely…
We describe an experimental system that allows one to easily access the dispersion curve of exciton-polaritons in a microcavity. Our approach is based on two spatial light modulators (SLM), one for changing the excitation angles (momenta),…
We illustrate that the surface plasmon polariton (SPP) excitation through the prism coupling method is fundamentally limited by destructive interference of spatial light components. We propose that the destructive interference can be…
We demonstrate spatially-resolved measurements of spontaneous and stimulated electron-photon interactions in nanoscale optical near fields using electron energy-loss spectroscopy (EELS), cathodoluminescence spectroscopy (CL), and…
Exciton-polaritons (EPs) arising from strong light-matter coupling offer new pathways for controlling optoelectronic properties. While typically requiring closed optical cavities for strong coupling, we demonstrate that 2D metal-organic…
Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting.…
Spin-polarized electron beam sources enable studies of spin-dependent electric and magnetic effects at the nanoscale. We propose a method of creating spin-polarized electrons on an integrated photonics chip by laser driven nanophotonic…
In this paper, we have developed a theory describing surface exciton polariton (SEPs) that accounts for the spatial dispersion of the dielectric constant connected with exciton momentum. Due to strong coupling between light and bulk…