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The structure of polar liquids and electrolytic solutions, such as water and aqueous electrolytes, at interfaces underlies numerous phenomena in physics, chemistry, biology, and engineering. In this work, we develop a continuum theory that…

Soft Condensed Matter · Physics 2022-07-13 J. Pedro de Souza , Alexei A. Kornyshev , Martin Z. Bazant

The interaction of charges in dielectric materials is screened by the dielectric constant of the bulk dielectric. In dielectric theories, screening is assigned to the surface charge appearing from preferential orientations of dipoles along…

Soft Condensed Matter · Physics 2019-09-04 Salman Seyedi , Daniel R. Martin , Dmitry V. Matyushov

The dynamics of a thin layer of liquid, between a flat solid substrate and an infinitely-thick layer of saturated vapor, is examined. The liquid and vapor are two phases of the same fluid, governed by the diffuse-interface model. The…

Statistical Mechanics · Physics 2021-09-27 E. S. Benilov

Evaporative mass flux is governed by interfacial state of liquid and vapor phases. For closely similar pressures and mass fluxes of liquid water into its own vapor, discontinuity between interfacial liquid and vapor temperatures in the…

Chemical Physics · Physics 2019-09-19 Parham Jafari , Amit Amritkar , Hadi Ghasemi

We have studied the real part of the dielectric constant of water from 100 Hz to 1 MHz. We have found that there is a frequency where the dielectric constant is independent of temperature, and called this the isopermitive point. Below this…

Chemical Physics · Physics 2015-05-20 A. Angulo-Sherman , H. Mercado-Uribe

We propose a unified model combining the first-order liquid-liquid and the second-order ferroelectric phase transitions models and explaining various features of the $\lambda$-point of liquid water within a single theoretical framework. It…

Soft Condensed Matter · Physics 2012-01-31 Peter O. Fedichev , Leonid I. Menshikov

Investigations of dielectric properties of water in nanoconfinement are highly relevant for various applications. Here, using a simple capacitor model, we show that the low dielectric constant of nanoconfined water found in molecular…

Soft Condensed Matter · Physics 2018-04-24 Chao Zhang

Recent experiments have shown that the out-of-plane dielectric constant of water confined in nanoslits of graphite and hexagonal boron nitride (hBN) is vanishingly small. Despite extensive effort based mainly on classical force-field…

Chemical Physics · Physics 2022-11-28 Thomas Dufils , Christoph Schran , Ji Chen , Andre K. Geim , Laura Fumagalli , Angelos Michaelides

We demonstrate that with two small modifications, the popular dielectric continuum model is capable of predicting, with high accuracy, ion solvation thermodynamics in numerous polar solvents, and ion solvation free energies in…

We calculate the effective macroscopic dielectric constant $\varepsilon_a$ of a periodic array of spherical nanocrystals (NCs) with dielectric constant $\varepsilon$ immersed in the medium with dielectric constant $\varepsilon_m \ll…

Mesoscale and Nanoscale Physics · Physics 2016-03-21 K. V. Reich , B. I. Shklovskii

A coarse grained description of a two phase fluid is used to study the steady state configuration of the interface separating the coexisting phases, and the motion of the contact line at which the interface intersects a solid boundary. The…

Statistical Mechanics · Physics 2009-10-31 Hsuan-Yi Chen , David Jasnow , Jorge Vinals

In this work, the electrohydrodynamic (EHD) instability induced by a unipolar charge injection is extended from a single-phase dielectric liquid to a two-phase system that consists of a liquid-air interface. A volume of fluid (VOF) model…

Fluid Dynamics · Physics 2022-01-05 Qiang Liu , Alberto T. Pérez , R. Deepak Selvakumar , Pengfei Yang , Jian Wu

We consider longwave mode of the interface instability in the system comprising of two immiscible fluid layers. The fluids fill out plane horizontal cavity which is subjected to horizontal harmonic vibration. The analysis is performed…

patt-sol · Physics 2007-05-23 Mikhail V. Khenner , Dmitrii V. Lyubimov

In this work we present the dielectric behavior of water with a novel flexible model that improved all three sites water models Different concentrations of the ionic liquid 1- butyl-3-methylimidazolium [bmim]…

Mesoscale water-hydrophobic interfaces are of fundamental importance in multiple disciplines, but their molecular properties have remained elusive for decades due to experimental complications and alternate theoretical explanations.…

Chemical Physics · Physics 2024-05-06 Lixue Shi , R. Allen LaCour , Xiaoqi Lang , Joseph P. Heindel , Teresa Head-Gordon , Wei Min

The in-plane dielectric constant of nanoconfined water has attracted growing interest over the last years. Nevertheless, this magnitude is not well-defined at the nanoscale due to its dependence on the arbitrary choice of water width. We…

Soft Condensed Matter · Physics 2026-05-08 Jon Zubeltzu

Electrostatic interactions between point charges embedded into interfaces separating dielectric media are omnipresent in soft matter systems and often control their stability. Such interactions are typically complicated and do not resemble…

Soft Condensed Matter · Physics 2020-09-09 Alexander Morozov , Iain Muntz , Job H. J. Thijssen , Davide Marenduzzo

We study the variation of the dielectric response of a dielectric liquid (e.g. water) when a salt is added to the solution. Employing field-theoretical methods we expand the Gibbs free-energy to first order in a loop expansion and calculate…

Soft Condensed Matter · Physics 2012-07-06 Amir Levy , David Andelman , Henri Orland

We study the effective forces acting between colloidal particles trapped at a fluid interface which itself is exposed to a pressure field. To this end we apply what we call the ``force approach'', which relies solely on the condition of…

Soft Condensed Matter · Physics 2008-03-31 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

We generalize the predictions for attractions between over-all neutral surfaces induced by charge fluctuations/correlations to non-uniform systems that include dielectric discontinuities, as is the case for mixed charged lipid membranes in…

Soft Condensed Matter · Physics 2009-10-31 Rebecca Menes , Philip Pincus , Bean Stein