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Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…

We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…

Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…

Chemical Physics · Physics 2015-05-13 X. G. Xu , S. O. Konorov , J. W. Hepburn , V. Milner

Field-enhanced infrared molecular spectroscopy has been widely applied in chemical analysis, environment monitoring, and food and drug safety. The sensitivity of molecular spectroscopy critically depends on the electromagnetic field…

Atomic Force Microscopy - Infrared (AFM-IR) spectroscopy allows spectroscopic studies in the mid-infrared spectral region with a spatial resolution better than 50 nm. We show that the high spatial resolution can be used to perform…

Quantitative Methods · Quantitative Biology 2017-04-06 Luca Quaroni , Katarzyna Pogoda , Joanna-Wiltowska Zuber , Wojciech Kwiatek

Two dimensional spectroscopy is a powerful dynamical study method that has been developed in the last two decades. In 2D IR there are three experimental time periods during which the system vibrational modes of interest are excited, evolved…

Chemical Physics · Physics 2021-04-12 S. Tahereh Alavi

This paper reviews the state of art technology of laser induced breakdown spectroscopy (LIBS). Research on LIBS is gaining momentum in the field of instrumentation and data analysis technique due to its wide application in various field…

Optics · Physics 2014-07-02 V. N. Rai

Advances in silicon photonics have resulted in rapidly increasing complexity of integrated circuits. New methods are desirable that allow direct characterization of individual optical components in-situ, without the need for additional…

Context. Filamentary structures appear to be ubiquitous in the interstellar medium. Being able to detect and characterize them is the first step toward understanding their origin, their evolution, and their role in the Galactic cycle of…

Astrophysics of Galaxies · Physics 2022-12-14 J. -S. Carrière , L. Montier , K. Ferrière , I. Ristorcelli

Multiparametric radiological imaging is vital for detection, characterization and diagnosis of many different diseases. The use of radiomics for quantitative extraction of textural features from radiological imaging is increasing moving…

Computer Vision and Pattern Recognition · Computer Science 2020-02-07 Vishwa S. Parekh , Michael A. Jacobs

Integrated photonic devices have become pivotal elements across most research fields that involve light-based applications. A particularly versatile category of this technology are programmable photonic integrated processors, which are…

Structured illumination can reject out-of-focus signal from a sample, enabling high-speed and high-contrast imaging over large areas with widefield detection optics. Currently, this optical-sectioning technique is limited by image…

Accelerator mass spectrometry (AMS) is a widely-used technique with multiple applications, including geology, molecular biology and archeology. In order to achieve a high dynamic range, AMS requires tandem accelerators and large magnets,…

Quantum Physics · Physics 2023-05-23 Radu Ionicioiu

Numerous molecules exhibit unique absorption bands in the fingerprint infrared (IR) region, allowing chemical identification and detection. This makes IR spectroscopy an essential tool in biomedical diagnostics, sensing, and material…

Optics · Physics 2022-02-04 Anna V. Paterova , Zi S. D. Toa , Hongzhi Yang , Leonid A. Krivitsky

Infrared (IR) spectroscopy is an indispensable tool for many practical applications including material analysis and sensing. Existing IR spectroscopy techniques face challenges related to the inferior performance and the high cost of…

Optics · Physics 2017-03-13 Anna Paterova , Shaun Lung , Dmitry Kalashnikov , Leonid Krivitsky

A novel characterization method to measure the pulse duration of ultrafast near-IR pulses is introduced, which uses simple tabletop optics, is relatively inexpensive, and is expected to work in a broad wavelength range. Our diagnostic tool…

Optics · Physics 2023-10-18 Rafeeq Syed , Cornelis J. G. J. Uiterwaal

Vibrational properties of molecular crystals are constantly used as structural fingerprints, in order to identify both the chemical nature and the structural arrangement of molecules. The simulation of these properties is typically very…

Computational Physics · Physics 2019-10-09 Nathaniel Raimbault , Andrea Grisafi , Michele Ceriotti , Mariana Rossi

X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free…

In the present work, we give an analytical non-perturbative treatment of mode-mode coupling and anharmonicity occurring in molecular vibrational systems analyzed by 2D-infrared spectroscopy. This analytical description allows a detailed…

Chemical Physics · Physics 2013-09-04 Kuo Kan Liang , Albert A. Villaeys

Stimulated Raman scattering (SRS) microscopy offers great potential to surpass fluorescent-based approaches, owing to the sharp linewidth of Raman vibrations amenable to super-multiplex cell imaging, but currently lacks one crucial…