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O2 and O3 have been long considered the most robust individual biosignature gases in a planetary atmosphere, yet multiple mechanisms that may produce them in the absence of life have been described. However, these abiotic planetary…
In the next few years, intensity-mapping surveys that target lines such as CO, Ly$\alpha$, and CII stand to provide powerful probes of high-redshift astrophysics. However, these line emissions are highly non-Gaussian, and so the typical…
UV ice photodesorption is an important non-thermal desorption pathway in many interstellar environments that has been invoked to explain observations of cold molecules in disks, clouds and cloud cores. Systematic laboratory studies of the…
Atomic nitrogen bound-bound radiation is a major component of the radiative heat flux on hypersonic vehicles entering nitrogen-dominated atmospheres, yet its prediction is limited by substantial parametric uncertainty in the published…
We study the transfer of spectral weight in the photoemission and optical spectra of strongly correlated electron systems. Within the LISA, that becomes exact in the limit of large lattice coordination, we consider and compare two models of…
CO$_2$ is an important, stable, and abundant molecule in the Universe, but it is very difficult to detect because it has no observable pure rotational transitions. The unique sensitivity and resolution of the James Webb Space Telescope…
Accurate and comprehensive H2 pressure-induced broadening data for CO2 infrared lines over a wide temperature range are essential for modeling atmospheric opacity of exoplanets. However, available data are currently limited, some of which…
We used the CRIRES spectrograph on the VLT to study the ro-vibrational 12CO/13CO, the Pfund beta and H2 emission between 4.59 and 4.72mu wavelengths toward the BN object, the disk candidate source n, and a proposed dust density enhancement…
Remote observation of spectroscopic emissions is a potential tool for the identification and quantification of various species in comets. CO Cameron band (to trace \cod) and atomic oxygen emissions (to trace H$_2$O and/or CO$_2$, CO) have…
Carbon dioxide is abundant in ice mantles of dust grains; some is found in the pure crystalline form as inferred from the double peak splitting of the bending profile at about 650 cm$^{-1}$. To study how CO$_2$ segregates into the pure form…
We present a study of the dynamical behavior of a Ziff-Gulari-Barshad model with CO desorption and lateral diffusion. Depending on the values of the desorption and diffusion parameters, the system presents a discontinuous phase transition…
Band oscillator strengths for electronic transitions in CO were obtained at the Synchrotron Radiation Center of the University of Wisconsin-Madison. Our focus was on transitions that are observed in interstellar spectra with the Far…
We present an experimental and theoretical study of the electronic band structure of ReS2 and ReSe2 at high hydrostatic pressures. The experiments are performed by photoreflectance spectroscopy and are analyzed in terms of ab initio…
We developed a mid-infrared optical frequency comb-based Fourier-transform spectrometer and performed a line-shape study of the fundamental vibrational band of CO perturbed by N${_2}$, which is crucial for atmospheric science and…
The diffusion of molecules on interstellar grain surfaces is one of the most important driving forces for the molecular complexity in the interstellar medium. Due to the lack of laboratory measurements, astrochemical modeling of grain…
In this work we investigate the dissociation of CO$_2$ on Cu(110) by performing density functional theory calculations using the vdW-DF2 exchange-correlation functional, with a potential energy surface parameterized using artificial neural…
Infrared spectra of the CO2-N2 dimer are observed in the carbon dioxide nu3 asymmetric stretch region (~2350 cm-1) using a tunable infrared optical parametric oscillator to probe a pulsed slit jet supersonic expansion. Previous results for…
In the near future, extremely-large ground-based telescopes may conduct some of the first searches for life beyond the solar system. High-spectral resolution observations of reflected light from nearby exoplanetary atmospheres could be used…
We analyze JWST/NIRSpec observations of the CO rovibrational v=1-0 band at 4.67um around the dust-embedded southern active galactic nucleus (AGN) of NGC3256 (d=40Mpc; L(IR)=10^11.6 Lsun). We classify the CO v=1-0 spectra into three…
Direct imaging spectroscopy with future space-based telescopes will constrain terrestrial planet atmospheric composition and potentially detect biosignature gases. One promising indication of life is abundant atmospheric O2. However,…