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In this work, we reveal giant magneto-optical responses in two-dimensional(2D) antiferromagnets with nearly flat electronic bands, based on first-principles calculations and group-theoretical analysis. We identify a record-large…

Materials Science · Physics 2025-06-23 Ping Yang , Wanxiang Feng , Siyuan Liu , Shan Guan , Liwei Wen , Wei Jiang , Gui-Bin Liu , Yugui Yao

Controlling magnetism by using electric fields is a goal of research towards novel spintronic devices and future nano-electronics. For this reason, multiferroic heterostructures attract much interest. Here we provide experimental evidence,…

We present a theoretical examination of the magneto-electric response in the recently discovered multiferroic insulator Cu$_2$OSeO$_3$. Combining Monte Carlo simulation and Ginzburg-Landau analysis we predict the response in each of the…

Strongly Correlated Electrons · Physics 2013-10-22 Ye-Hua Liu , Jung Hoon Han , A. A. Omrani , H. M. Rønnow , You-Quan Li

Ba2CoGe2O7, crystallizing in the noncentrosymmetric but nonpolar structure, belongs to a special class of multiferroic materials, whose properties are predetermined by the rotoinversion symmetry. Unlike inversion, the rotoinversion symmetry…

Materials Science · Physics 2015-06-23 I. V. Solovyev

Understanding the magnetic and ferroelectric ordering of magnetoelectric multiferroic materials at the nanoscale necessitates a versatile imaging method with high spatial resolution. Here, soft X-ray ptychography is employed to…

We present a laterally resolved X-ray magnetic dichroism study of the magnetic proximity effect in a highly ordered oxide system, i.e. NiO films on Fe3O4(110). We found that the magnetic interface shows an ultrasharp electronic, magnetic…

Materials Science · Physics 2008-01-10 I. P. Krug , F. U. Hillebrecht , H. Gomonaj , M. Haverkort , A. Tanaka , L. H. Tjeng , C. M. Schneider

Recent experimental studies have demonstrated the possibility of utilizing strong terahertz pulses to manipulate individual ferroic orders on pico- and femtosecond timescales. Here, we extend these findings and showcase the simultaneous…

Strongly Correlated Electrons · Physics 2025-02-25 Daniel A. Bustamante Lopez , Dominik M. Juraschek , Michael Fechner , Xianghan Xu , Sang-Wook Cheong , Wanzheng Hu

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

Strongly Correlated Electrons · Physics 2021-03-17 G. van der Laan , S. W. Lovesey

Multiferroic TbMnO3 is investigated using x-ray diffraction in high magnetic fields. Measurements on first and second harmonic structural reflections due to modulations induced by the Mn and Tb magnetic order are presented as function of…

Strongly Correlated Electrons · Physics 2008-07-29 J. Strempfer , B. Bohnenbuck , I. Zegkinoglou , N. Aliouane , S. Landsgesell , M. v. Zimmermann , D. N. Argyriou

BiFeO$_3$ is the most famous multiferroic material, but it has no strong spontaneous magnetization due to its antiferromagnetism. Here we show that giant ferroelectric polarization and strong spontaneous magnetization can be both realized…

Materials Science · Physics 2019-06-13 Peng Chen , Bang-Gui Liu

Magnetic rare-earth orthoferrites $R$FeO$_3$ host a variety of functional properties from multiferroicity and strong magnetostriction, to spin-reorientation transitions and ultrafast light-driven manipulation of magnetism, which can be…

Materials Science · Physics 2023-04-12 Danila Amoroso , Bertrand Dupe , Matthieu J. Verstraete

We present results of an {\it ab initio} density functional theory study of three bismuth-based multiferroics, BiFeO$_{3}$, Bi$_{2}$FeCrO$_{6}$, and BiCrO$_{3}$. We disuss differences in the crystal and electronic structure of the three…

Materials Science · Physics 2007-05-23 Pio Baettig , Claude Ederer , Nicola A. Spaldin

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

Hexagonal LuFeO$_3$ has drawn a lot of research attention due to its contentious room-temperature multiferroicity. Due to the unstability of hexagonal phase in the bulk form, most experimental studies focused on LuFeO$_3$ thin films which…

Materials Science · Physics 2016-03-09 L. Lin , H. M. Zhang , M. F. Liu , Shoudong Shen , S. Zhou , D. Li , X. Wang , Z. B. Yan , Z. D. Zhang , Jun Zhao , Shuai Dong , J. -M. Liu

The leading order nonlinear (NL) susceptibility, $\chi_3$, in a paramagnet is negative and diverges as $T \rightarrow 0$. This divergence is destroyed when spins correlate and the NL response provides unique insights into magnetic order.…

By performing systematic $ab$ $initio$ density functional calculations, here we study two relativity-induced properties of atomically thin ferromagnetic (FM) Cr$_2$Ge$_2$Te$_6$ films [monolayer (ML), bilayer (BL) and trilayer (TL) as well…

Mesoscale and Nanoscale Physics · Physics 2018-09-25 Yimei Fang , Shunqing Wu , Zi-Zhong Zhu , Guang-Yu Guo

Multiferroic perovskites that exhibit room temperature magnetization and polarization have immense potential in the next generation of magneto-electric and spintronic memory devices. In this work, the magnetic and ferroelectric properties…

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

To sum up, we show in the present paper that magnetic response in Nb$_2$O$_2$F$_3$ at the high-temperatures ($T>$90 K) is related to the orbital selective regime, when part of the electrons form molecular orbitals while other electrons have…

Materials Science · Physics 2017-05-24 V. V. Gapontsev , D. I. Khomskii , S. V. Streltsov

In a collinear magnet, the predominant magnetic moments are collectively aligned along a specific spatial orientation, and this alignment may yield intriguing phenomena such as spin orientation driven polarization. It is well known that…

Materials Science · Physics 2025-12-12 Yixun Zhang , Longju Yu , Yizhou Tong , Ying Sun , Xu Li , Hong Jian Zhao , Yanming Ma