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Quantum effects play a significant role in nanometric plasmonic devices, such as small metal clusters and metallic nanoshells. For structures containing a large number of electrons, ab-initio methods such as the time-dependent density…

Mesoscale and Nanoscale Physics · Physics 2018-09-27 Giovanni Manfredi , Paul-Antoine Hervieux , Fatema Tanjia

As the continual experimental advances made in Electron energy loss spectroscopy (EELS) and cathodoluminescence (CL) open the door to practical exploitations of plasmonic effects in metal nanoparticles, there is an increasing need for…

Mesoscale and Nanoscale Physics · Physics 2016-05-31 Yu Luo , Matthias Kraft , J. B. Pendry

Quantum plasmonics is a rapidly growing field of research that involves the study of the quantum properties of light and its interaction with matter at the nanoscale. Here, surface plasmons - electromagnetic excitations coupled to electron…

Quantum Physics · Physics 2013-12-25 M. S. Tame , K. R. McEnery , S. K. Ozdemir , J. Lee , S. A. Maier , M. S. Kim

Interaction of electromagnetic radiation with time-variant objects is a fundamental problem whose study involves foundational principles of classical electrodynamics. Such study is a necessary preliminary step for delineating the novel…

Applied Physics · Physics 2019-05-08 Grigorii Ptitcyn , Mohammad S. Mirmoosa , Sergei A. Tretyakov

Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…

The interaction of electromagnetic waves with metallic nanostructures generates resonant oscillations of the conduction-band electrons at the metal surface. These resonances can lead to large enhancements of the incident field and to the…

Optics · Physics 2018-05-09 Ferran Vidal-Codina , Ngoc-Cuong Nguyen , Jaime Peraire

We introduce an approach to determining the required waveforms to coherently control the optical energy localization in plasmonic nanosystems. This approach is based on the impulsive localized excitation of the nanosystem and time reversal…

Disordered Systems and Neural Networks · Physics 2007-05-23 Xiangting Li , Mark I. Stockman

Understanding and mastering the mechanical properties of metallic nanoparticles is crucial for their use in a wide range of applications. In this context, we use atomic-scale (Molecular Dynamics) and continuous (Finite Elements)…

Materials Science · Physics 2023-03-14 Matteo Erbi , Hakim Amara , Riccardo Gatti

A novel theoretical approach to the dynamics analysis of excitation of plasmon modes in nanoparticles is presented. This approach is based on the biorthogonal plasmon mode expansion and it leads to the predictions of time-dynamics of…

Materials Science · Physics 2007-05-23 Isaak D. Mayergoyz , Zhenyu Zhang , Giovanni Miano

The collective response of metal nanostructures to optical excitation leads to localized plasmon generation with nanoscale field confinement driving applications in e.g. quantum optics, optoelectronics, and nanophotonics, where a bottleneck…

Rapid modulation of the electromagnetic response in both time and space creates temporal boundaries in the medium and leads to time-reflection and time-refraction of light and to the eventual formation of the photonic time crystal within…

Optics · Physics 2024-10-01 Evgenii E. Narimanov

We present an approach for generating local numerical basis sets of improving accuracy for first-principles nanoplasmonics simulations within time-dependent density functional theory. The method is demonstrated for copper, silver, and gold…

Materials Science · Physics 2015-09-04 Tuomas P. Rossi , Susi Lehtola , Arto Sakko , Martti J. Puska , Risto M. Nieminen

Routine investigations of plasmonic phenomena at the quantum level present a formidable computational challenge due to the large system sizes and ultrafast timescales involved. This Feature Article highlights the use of density functional…

Mesoscale and Nanoscale Physics · Physics 2025-06-19 Nikhil S. Chellam , Subhajyoti Chaudhuri , Abhisek Ghosal , Sajal K. Giri , George C. Schatz

Plasmonic gap structures are among the few configurations capable of generating extreme light confinement, finding applications in surface-enhanced spectroscopy, ultrasensitive detection, photocatalysis and more. Their plasmonic response…

Mesoscale and Nanoscale Physics · Physics 2025-02-21 Pu Zhang , Christos Tserkezis , N. Asger Mortensen

Quantum aspects, such as electron tunneling between closely separated metallic nanoparticles, are crucial for understanding the plasmonic response of nanoscale systems. We explore quantum effects on the response of the conductively coupled…

Materials Science · Physics 2015-12-08 Tuomas P. Rossi , Asier Zugarramurdi , Martti J. Puska , Risto M. Nieminen

Time crystals are an eagerly sought phase of matter with broken time-translation symmetry. Quantum time crystals with discretely broken time-translation symmetry have been demonstrated in trapped ions, atoms and spins while continuously…

Optics · Physics 2023-08-03 Tongjun Liu , Jun-Yu Ou , Kevin F. MacDonald , Nikolay I. Zheludev

We present an ab-initio study of the hybridization of localized surface plasmons in a metal nanoparticle dimer. The atomic structure, which is often neglected in theoretical studies of quantum nanoplasmonics, has a strong impact on the…

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

Simultaneous spatio-temporal confinement of energetic electron pulses to femtosecond and nanometer scales is a topic of great interest in the scientific community, given the potential impact of such development on a wide spectrum of…

A promising trend in plasmonics involves shrinking the size of plasmon-supporting structures down to a few nanometers, thus enabling control over light-matter interaction at extreme-subwavelength scales. In this limit, quantum mechanical…