Related papers: Hidden correlations in stochastic photoinduced dyn…
We study photon correlations generated by scattering from three-level systems (3LS) in one dimension. The two systems studied are a 3LS in a semi-infinite waveguide (3LS plus a mirror) and two 3LS in an infinite waveguide (double 3LS). Our…
The photochemistry of a molecular ensemble coupled to a resonance cavity and triggered by a femtosecond laser pulse is investigated from a real-time, quantum dynamics perspective with the multi-configuration time-dependent Hartree method.…
Photoemission from a solid surface provides a wealth of information about the electronic structure of the surface and its dynamic evolution. Ultrafast pump-probe experiments are particularly useful to study the dynamic interactions of…
The kinetic processes in nanoparticle-based catalysis are dominated by large fluctuations and spatiotemporal heterogeneities, in particular for diffusion-influenced reactions which are far from equilibrium. Here, we report results from…
Interferometric methods, renowned for their reliability and precision, play a vital role in phase imaging. Interferometry typically requires high coherence and stability between the measured and the reference beam. The presence of rapid…
Understanding the interaction of kilojoule, picosecond laser pulse with long-scale length preplasma or homogeneous near critical density (NCD) plasma is crucial for guiding experiments at national short-pulse laser facilities. Using full…
We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…
We describe some general results that constrain the dynamical fluctuations that can occur in non-equilibrium steady states, with a focus on molecular dynamics. That is, we consider Hamiltonian systems, coupled to external heat baths, and…
Stimulated photon-photon scattering is a predicted consequence of quantum electrodynamics that has yet to be measured directly. Measuring the cross-section for stimulated photon-photon scattering is the aim of a flagship experiment for NSF…
The photon statistics and bunching of a semiconductor laser with external optical feedback are investigated experimentally and theoretically. In a chaotic regime, the photon number distribution is measured and undergoes a transition from…
Understanding the nature of the photoexcitation and ultrafast charge dynamics pathways in organic halide perovskite nanocubes and their aggregation into superlattices is key for the potential applications as tunable light emitters, photon…
The absorption of ultraviolet light creates excitations in DNA, which subsequently start moving in the helix. Their fate is important for an understanding of photo damage, and is determined by the interplay of electronic couplings between…
We give a detailed account of equilibrium and non-equilibrium fluctuational electrodynamics of hyperbolic metamaterials. We show the unifying aspects of two different approaches; one utilizes the second kind of fluctuation dissipation…
Superionic conductors, or solid-state ion-conductors surpassing 0.01 S/cm in conductivity, can enable more energy dense batteries, robust artificial ion pumps, and optimized fuel cells. However, tailoring superionic conductors require…
The currently existing theory of fluorescence correlation spectroscopy(FCS) is based on the linear fluctuation theory originally developed by Einstein, Onsager, Lax, and others as a phenomenological approach to equilibrium fluctuations in…
We numerically investigate photo-responses of the charge ordered state upon stimuli of pulsed laser light, especially paying attention to the differences in the pulse width, whose shortness has been a key to experimentally realize large…
Impacts of quantum stochasticity on the dynamics of an ultra-relativistic electron beam head-on colliding with a linearly polarized ultra-intense laser pulse are theoretically investigated in a quasi-classical regime. Generally, the angular…
The tight inter-band correlation and the lag-wavelength relation among UV/optical continua of active galactic nuclei have been firmly established. They are usually understood within the widespread reprocessing scenario, however, the implied…
In this paper we describe an ultrafast scanning electron microscope setup developed for the research of inelastic scattering of electrons at optical near-fields of periodic dielectric nanostructures. Electron emission from the Schottky…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…