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Performing an analysis within density functional theory, we develop insight into the structural and electronic properties of the oxide heterostructure LaAlO3/SrTiO3. Electrostatic surface effects are decomposed from the internal lattice…

Materials Science · Physics 2015-05-13 U. Schwingenschloegl , C. Schuster

We report calculations of the electronic structure and optical properties of doped $n$-type perovskite BaSnO3 and layered perovskites. While doped BaSnO$_3$ retains its transparency for energies below the valence to conduction band onset,…

Materials Science · Physics 2015-02-03 Yuwei Li , Lijun Zhang , Yanming Ma , David J. Singh

La-doped SrSnO3 (LSSO) is known as one of deep-ultraviolet (DUV)-transparent conducting oxides with an energy bandgap of ~4.6 eV. Since LSSO can be grown heteroepitaxially on more wide bandgap substrates such as MgO (Eg ~7.8 eV), LSSO is…

Materials Science · Physics 2020-01-29 Mian Wei , Anup V. Sanchela , Bin Feng , Yuichi Ikuhara , Hai Jun Cho , Hiromichi Ohta

Molecular beam epitaxy (MBE) is a state-of-the-art technique for depositing thin films with precise stoichiometric control. However, when depositing oxides of perovskite-type ABO3, this process becomes challenging as controlling the flux…

Materials Science · Physics 2024-10-02 Jasnamol Palakkal , Tobias Meyer , Márton Major , Laurin Elias Bierschenk , Lambert Alff

Although over the past number of years there have been many advances in the materials aspects of topological insulators (TI), one of the ongoing challenges with these materials is the protection of them against aging. In particular, the…

Materials Science · Physics 2015-10-08 Maryam Salehi , Matthew Brahlek , Nikesh Koirala , Jisoo Moon , Liang Wu , N. P. Armitage , Seongshik Oh

Strontium titanate, SrTiO3, a widely used substrate material for electronic oxide thin film devices, has provided many interesting features. In a combination with a similar oxide material, LaAlO3, it has recently received great interest. It…

Materials Science · Physics 2013-05-29 Alexey S. Kalabukhov , Robert Gunnarsson , Johan Borjesson , Eva Olsson , Tord Claeson , Dag Winkler

In this paper we use density functional theory combined with dynamical mean-field theory (DFT+DMFT) to study interface effects between thin films of the correlated metal CaVO$_3$ and the two typical substrate materials SrTiO$_3$ and…

Strongly Correlated Electrons · Physics 2021-01-04 Sophie Beck , Claude Ederer

The presence of amorphous oxide layers can significantly affect the coherent time of superconducting qubits due to their high dielectric loss. Typically, the surface oxides of superconductor films exhibit lossy and unstable behavior when…

Materials Science · Physics 2024-05-08 Zengqian Ding , Boyi zhou , Tao Wang , Lina Yang , Yanfu Wu , Xiao Cai , Kanglin Xiong , Jiagui Feng

Solution-processed organic semiconductors enable the fabrication of large-area and flexible electronics by means of cost-effective, solution-based mass manufacturing techniques. However, for many applications an insoluble active layer can…

Polar discontinuities and redox reactions provide alternative paths to create two-dimensional electron liquids (2DELs) at oxide interfaces. Herein, we report high mobility 2DELs at interfaces involving SrTiO3 (STO) achieved using polar…

Materials Science · Physics 2017-10-24 Y. Z. Chen , R. J. Green , R. Sutarto , F. He , S. Linderoth , G. A. Sawatzky , N. Pryds

We report on the successful synthesis of highly conductive PdCoO2 ultrathin films on Al2O3 (0001) by pulsed laser deposition. The thin films grow along the c-axis of the layered delafossite structure of PdCoO2, corresponding to the…

Strongly Correlated Electrons · Physics 2018-04-24 T. Harada , K. Fujiwara , A. Tsukazaki

Transparent conducting oxides (TCOs) represent a remarkable class of materials that possess both excellent electrical conductivity and high optical transparency, which are typically considered mutually exclusive in traditional materials. In…

Materials Science · Physics 2024-10-22 Jarnail Singh , Pankaj Bhardwaj

A chemical-free technique for fabricating submicron complex oxide structures has been developed based on selective epitaxial growth. The crystallinity and hence the conductivity of the complex oxide is inhibited by amorphous SrTiO3 (STO).…

Superconductivity · Physics 2007-05-23 P. Morales , M. DiCiano , J. Y. T. Wei

Oxide electronics relies on the availability of epitaxial oxide thin films. The extreme flexibility of the chemical composition of ABO3 perovskites and the broad spectrum of properties they cover, inspire the creativity of scientists and…

Materials Science · Physics 2014-04-01 Florencio Sanchez , Carmen Ocal , Josep Fontcuberta

We report a detailed study performed on La2Zr2O7 (LZO) pyrochlore material grown by Metal-Organic Decomposition (MOD) method as buffer layers for YBa2Cu3O7-x (YBCO) coated conductors. High quality epitaxial LZO thin films have been obtained…

4d transition metal oxides have emerged as promising materials for numerous applications including high mobility electronics. SrNbO$_{3}$ is one such candidate material, serving as a good donor material in interfacial oxide systems and…

Materials Science · Physics 2022-10-31 Suresh Thapa , Sydney Provence , Steve M. Heald , Marcelo A. Kuroda , Ryan B. Comes

We optimize the deposition of CH3NH3PbI3 perovskite into mesoporous electrodes consisting of anodic TiO2 nanotube layers. By a simple spin coating approach, complete filling of the tube scaffolds is obtained, that leads to interdigitated…

Surface morphology of the substrate and bottom layers plays a critical role in the epitaxial growth of oxide thin films. Here, we report on the self-organized formation of a step-terrace structure in SrRuO3 (SRO) thin films grown using…

It is highly desirable to search for promising two-dimensional (2D) monolayer materials for deep insight of 2D materials and applications. We use first-principles method to investigate tetragonal perovskite oxide monolayers as 2D materials.…

Mesoscale and Nanoscale Physics · Physics 2019-07-08 Xiang-Bo Xiao , Bang-Gui Liu

The crystal structures of LaAlO3 films grown by pulsed laser deposition on SrTiO3 substrates at oxygen pressure of 10-3 mbar or 10-5 mbar, where kinetics of ablated species hardly depend on oxygen background pressure, are compared. Our…

Materials Science · Physics 2014-10-10 Jihwey Park , Yeong-Ah Soh , Gabriel Aeppli , Adrian David , Weinan Lin , Tom Wu