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Related papers: Isotopologue-selective laser cooling of molecules

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Mass spectrometry is used in a wide range of scientific disciplines including proteomics, pharmaceutics, forensics, and fundamental physics and chemistry. Given this ubiquity, there is a worldwide effort to improve the efficiency and…

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

Atomic Physics · Physics 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

Doppler and Sisyphus cooling of $^{174}$YbOH are achieved and studied. This polyatomic molecule has high sensitivity to physics beyond the Standard Model and represents a new class of species for future high-precision probes of new…

YbF has been identified as a molecule that can be used to investigate charge-parity symmetry violations that are beyond the Standard Model of particle physics. Cooling to sub-milli-Kelvin is advantageous for experiments that probe…

Chemical Physics · Physics 2022-12-14 Thomas D. Persinger , Jiande Han , Anh T. Le , Timothy C. Steimle , Michael C. Heaven

We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…

Atomic Physics · Physics 2020-08-05 Benjamin L. Augenbraun , John M. Doyle , Tanya Zelevinsky , Ivan Kozyryev

A full density-matrix simulation is performed for optical deflection of a barium monofluoride (BaF) beam. Pairs of counter-propagating laser pulses are used for stimulated absorption followed by stimulated emission. The scheme produces a…

Atomic Physics · Physics 2023-01-18 A. Marsman , D. Heinrich , M. Horbatsch , E. A. Hessels

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…

Atomic Physics · Physics 2017-04-05 S. Truppe , H. J. Williams , N. J. Fitch , M. Hambach , T. E. Wall , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…

To achieve Bose-Einstein condensation, one may implement evaporative cooling by dynamically regulating the power of laser beams forming the optical dipole trap. We propose and experimentally demonstrate a protocol of Bayesian optimization…

Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…

We explore, theoretically and experimentally, a method for cooling a broadband heat reservoir, via its laser-assisted collisions with two-level atoms followed by their fluorescence. This method is shown to be advantageous compared to…

Quantum Physics · Physics 2015-03-02 D. Gelbwaser-Klimovsky , K. Szczygielski , U. Vogl , A. Saß , R. Alicki , G. Kurizki , M. Weitz

We describe a controllable and precise laser tweezers for Bose-Einstein condensates of ultracold atomic gases. In our configuration, a laser beam is used to locally modify the sign of the scattering length in the vicinity of a trapped BEC.…

Other Condensed Matter · Physics 2009-11-13 Alicia V. Carpentier , Juan Belmonte-Beitia , Humberto Michinel , Victor M. Perez-Garcia

$^{133}\text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive…

Quantum Physics · Physics 2017-09-13 David Hucul , Justin E. Christensen , Eric R. Hudson , Wesley C. Campbell

We present a study of Sisyphus cooling of molecules: the scattering of a single-photon remove a substantial amount of the molecular kinetic energy and an optical pumping step allow to repeat the process. A review of the produced cold…

Chemical Physics · Physics 2014-04-11 Daniel Comparat

E.A. Schoene et al., in arXiv:1012.3207 [Phys. Rev.A, 82, 023419 (2010)] give incorrect interpretation of their experimental results. Really we observe a temporary capture and additional cooling of atoms in the presence of the orthogonal…

General Physics · Physics 2011-01-13 V. A. Kuz'menko

Recent work with laser-cooled molecules in attractive optical traps has shown that the differential AC Stark shifts arising from the trap light itself can become problematic, limiting collisional shielding efficiencies, rotational coherence…

Atomic Physics · Physics 2022-06-08 Yukai Lu , Connor M. Holland , Lawrence W. Cheuk

A method of electron beam cooling is considered which can be used for linear colliders. The electron beam is cooled during collision with focused powerful laser pulse. The ultimate transverse emittances are much below those achievable by…

High Energy Physics - Experiment · Physics 2009-10-31 Valery Telnov

Optical pumping of barium monofluoride (BaF) within a cryogenic neon matrix is demonstrated. Interestingly, with an applied magnetic field of 2~G, optical pumping is found to be considerably more efficient for a laser beam with…

This paper analyses the cooling of a single particle in a harmonic trap with red-detuned laser light with fewer approximations than previously done in the literature. We avoid the adiabatic elimination of the excited atomic state but are…

Quantum Physics · Physics 2015-05-27 Tony Blake , Andreas Kurcz , Norah S. Saleem , Almut Beige

The resonant laser cooling of circular accelerator beams of relativistic charged particle is studied. It is shown that in the approximation of the given external electromagnetic wave amplitude (small gain free electron laser) the emittance…

Accelerator Physics · Physics 2007-05-23 R. V. Tumanian