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Controlling the ferroelectricity and magnetism in multiferroic materials has been an important research topic. We report the formation of a highly polarized state in multiferroic DyMnO3 single crystals which develops well above the magnetic…

Materials Science · Physics 2014-09-05 Tao Zou , Zhiling Dun , Huibo Cao , Mengze Zhu , Daniel Coulter , Haidong Zhou , Xianglin Ke

While doping is widely used for tuning physical properties of perovskites in experiments, it remains a challenge to exactly know how doping achieves the desired effects. Here, we propose an empirical and computationally tractable model to…

Materials Science · Physics 2019-01-30 J. Liu , L. Jin , Z. Jiang , L. Liu , L. Himanen , J. Wei , N. Zhang , D. Wang , C. -L. Jia

We report an electric-field poling study of the geometric-driven improper ferroelectric h-ErMnO$_3$. From a detailed dielectric analysis we deduce the temperature and frequency dependent range for which single-crystalline h-ErMnO$_3$…

The polar metal is a material that hosts both polar distortion and metallicity. Such a material is expected to show exotic magneto-electric phenomena if superconducts. Here, we theoretically explore ferroelectric and superconducting…

Superconductivity · Physics 2021-05-26 Minjae Ghim , Nobuya Sato , Ryosuke Akashi , Seung-Hoon Jhi , Shinji Tsuneyuki

The evolution of electronic (spin and charge) excitations upon carrier doping is an extremely important issue in superconducting layered cuprates and the knowledge of its asymmetry between electron- and hole-dopings is still fragmentary.…

Films of all-important compound hafnia (HfO2) can be prepared in an orthorhombic ferroelectric (FE) state that is ideal for applications, e.g. in memories or negative-capacitance field-effect transistors. The origin of this FE state remains…

Materials Science · Physics 2020-07-15 Sangita Dutta , Hugo Aramberri , Tony Schenk , Jorge Íñiguez

We use first-principles calculations based on density functional theory to investigate the interplay between oxygen vacancies, A-site cation size / tolerance factor, epitaxial strain, ferroelectricity and magnetism in the perovskite…

Materials Science · Physics 2021-03-09 Astrid Marthinsen , Carina Faber , Ulrich Aschauer , Nicola A. Spaldin , Sverre M. Selbach

Hexagonal YMnO$_3$ is well known for the co-occurrence of ferroelectricity and antiferromagnetism at low temperatures. Using temperature-dependent spectroscopic ellipsometry at an $a$-plane oriented single crystal, we show how the…

Materials Science · Physics 2015-03-16 Steffen Richter , Stefan G. Ebbinghaus , Marius Grundmann , Rüdiger Schmidt-Grund

The effect of electron doping on the structural, transport, and magnetic properties of Mn (IV) - rich Ca1-xYxMnO3 (x < 0.2) samples have been investigated using neutron diffraction, neutron depolarization, magnetization and resistivity…

Materials Science · Physics 2016-02-09 Neetika Sharma , A. Das , C. L. Prajapat , Amit Kumar , M. R. Singh

The structural and magnetic properties of polycrystalline YMn1-xMxO3 (M = Ti, Fe, Ga; x = 0, 0.1) have been studied by neutron powder diffraction and magnetic measurements to probe the effect of Mn site doping on the frustration behavior…

Materials Science · Physics 2013-08-13 Neetika , A. Das , C. L. Prajapat , S. S. Meena

We use a combination of first-principles density functional calculations and spin-dynamics simulations to explain the unusual diffuse inelastic neutron scattering in the hexagonal multiferroic yttrium manganite, YMnO$_3$. Using symmetry…

Materials Science · Physics 2023-12-15 Tara N. Tošić , Arkadiy Simonov , Nicola A. Spaldin

Collinear dipole orders such as ferroelectricity and antiferroelectricity have developed rapidly in last decades. While, the noncollinear dipole orders are rarely touched in solids. Noncollinear dipole orders can provide a route to realize…

Materials Science · Physics 2024-11-01 Xinyu Yang , Jun Chen , Shan-Shan Wang , Shuai Dong

The ferroelectric properties of nanoscale silicon doped HfO$_2$ promise a multitude of applications ranging from ferroelectric memory to energy-related applications. The reason for the unexpected behavior has not been clearly proven and…

Materials Science · Physics 2018-01-03 Christopher Künneth , Robin Materlik , Max Falkowski , Alfred Kersch

Doping is a widely used method to tune physical properties of ferroelectric perovskites. Since doping can induce charges due to the substitution of certain elements, charge effects shall be considered in doped samples. To understand how…

Materials Science · Physics 2020-06-17 J. Liu , L. Liu , J. Zhang , L. Jin , D. Wang , J. Wei , Z. -G. Ye , C. -L. Jia

We systematically investigate the effect of strain and doping on the polar metal phase in lithium osmate, LiOsO$_3$, using first-principles calculations. We demonstrate that the polar metal phase in LiOsO$_3$ can be controlled by biaxial…

Materials Science · Physics 2020-04-28 Awadhesh Narayan

SrTiO$_{3}$ is an incipient ferroelectric and an exceptionally dilute superconductor with a dome-like dependence on carrier concentration. Stabilization of a polar phase through chemical substitution or strain significantly enhances the…

Superconductivity · Physics 2024-11-13 Alex Hallett , John W. Harter

Hybrid magnonic quantum systems have drawn increased attention in recent years for coherent quantum information processing, but too large magnetic damping is a persistent concern when metallic magnets are used. Their intrinsic damping is…

Materials Science · Physics 2024-01-17 Zhihao Jiang , Axel Hoffmann , André Schleife

We design a multiferroic metal that combines seemingly incompatible ferromagnetism, ferroelectricity, and metallicity by hole doping a two-dimensional (2D) ferroelectric with high density of states near the Fermi level. The strong…

Materials Science · Physics 2021-08-12 Xu Duan , Jiawei Huang , Bin Xu , Shi Liu

Ferroelectricity in crystals is associated with the displacement of ions or rotations of polar units. Here we consider the dipole created by donor doping ($D^+$) and the corresponding bound polaron ($e^-$).A dipole of 6.15 Debye is…

Materials Science · Physics 2022-07-06 Kazuki Morita , Yu Kumagai , Fumiyasu Oba , Aron Walsh

Hexagonal YMnO$_{3}$ is a prototype antiferromagnet which exhibits multiferroic behavior with the ferroelectric and magnetic transitions occurring at different temperatures. We observe an out-of-plane canting of the Mn$^{3+}$ magnetic…

Strongly Correlated Electrons · Physics 2022-09-22 M. Ramakrishnan , Y. Joly , Q. N. Meier , M. Fechner , M. Porer , S. Parchenko , Y. W. Windsor , E. M. Bothschafter , F. Lichtenberg , U. Staub