Related papers: Signatures of spinon dynamics and phase structure …
Recent investigations on the dipolar-octupolar compounds Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$ suggest that they may stabilize so-called $\pi$-flux octupolar quantum spin ice ($\pi$-O-QSI), a novel three-dimensional quantum spin liquid…
The identification of fractionalized excitations in quantum spin liquids (QSLs) remains a central challenge in condensed matter physics. In dipolar-octupolar (DO) pyrochlores, such as $\text{Ce}_2\text{Zr}_2\text{O}_7$, the candidate…
Motivated by the rapid experimental progress of quantum spin ice materials, we study the dynamical properties of pyrochlore spin ice in the U(1) spin liquid phases. In particular, we focus on the spinon excitations that appear at high…
Recent experiments on Ce$_2$Zr$_2$O$_7$ suggest that this material may host a novel form of quantum spin ice, a three-dimensional quantum spin liquid with an emergent photon. The Ce$^{3+}$ local moments on the pyrochlore lattice are…
We study the quantum spin dynamics of a frustrated XXZ model on a pyrochlore lattice by using large-scale quantum Monte Carlo simulation and stochastic analytic continuation. In the low-temperature quantum spin ice regime, we observe…
Inspired by the progress on the spin liquid candidates Ce$_2$Sn$_2$O$_7$ and Ce$_2$Zr$_2$O$_7$ where the Ce ions carry the dipole-octupole doublets, we analyze the distinction between the thermodynamic and spectroscopic measurements for the…
Two dimensional coherent spectroscopy (2DCS) probes the nonlinear optical response of correlated systems. An interesting application is the study of fractionalized excitations, which are challenging to distinguish unambiguously in linear…
Recently there have been a number of experiments on Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$, suggesting that these materials host a three-dimensional quantum spin liquid with emergent photons and fractionalized spinon excitations. However,…
With recent advances in terahertz (THz) sources and detection, two-dimensional coherent spectroscopy (2DCS), which allows to probe nonlinear responses in a two-frequency plane, now reaches the meV regime relevant for quasiparticle…
Electronic spins can form long-range entangled phases of condensed matter named quantum spin liquids. Their existence is conceptualized in models of two- or three-dimensional frustrated magnets that evade symmetry-breaking order down to…
Two-dimensional coherent spectroscopy (2DCS) is a nonlinear spectroscopy technique capable of identifying whether apparent continua in linear response are made out of multiplets of sharp deconfined quasiparticles. This makes it a potent…
Two-dimensional coherent spectroscopy (2DCS) with terahertz radiation offers a promising new avenue for the exploration of many-body phenomena in quantum magnets. This includes the potential diagnosis of fractionalized excitations, for…
The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Remarkably, the spin ices provide one of very few…
Realistic model Hamiltonians for quantum spin liquids frequently exhibit a large separation of energy scales between their elementary excitations. At intermediate, experimentally relevant temperatures, some excitations are sparse and hop…
Most materials freeze when cooled to sufficiently low temperature. We find that magnetic dipoles randomly distributed in a solid matrix condense into a spin liquid with spectral properties on cooling that are the diametric opposite of those…
Unambiguous identification of fractionalized excitations in quantum spin liquids has been a long-standing issue in correlated topological phases. Conventional spectroscopic probes, such as the dynamical spin structure factor, can only…
We investigate the signatures of fractionalization in quantum spin liquids by studying different phases of the Kitaev honeycomb model in the presence of an out-of-plane magnetic field through which the model becomes non-integrable. Using…
Fractionalization remains one of the most fascinating manifestations of strong interactions in quantum many-body systems. In quantum magnetism, the existence of spinons -- collective magnetic excitations that behave as quasiparticles with…
We consider gapped Z2 spin liquids, where spinon quasiparticles may carry fractional quantum numbers of space group symmetry. In particular, spinons can carry fractional crystal momentum. We show that such quantum number fractionalization…
The experimental characterization of quantum spin liquids poses significant challenges due to the absence of long-range magnetic order, even at absolute zero temperature. The identification of these states of matter often relies on the…