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Artificially reproducing the biological light reactions responsible for the remarkably efficient photon-to-charge conversion in photosynthetic complexes represents a new direction for the future development of photovoltaic devices. Here, we…

Quantum Physics · Physics 2013-12-25 C. Creatore , M. A. Parker , S. Emmott , A. W. Chin

When dense high-energy lepton bunches collide, the beam particles can experience rest-frame electromagnetic fields which greatly exceed the QED critical one. Here it is demonstrated that beamstrahlung efficiently converts lepton energy to…

High Energy Physics - Phenomenology · Physics 2021-11-18 Matteo Tamburini , Sebastian Meuren

The high efficiency of charge generation within organic photovoltaic blends apparently contrasts with the strong "classical" attraction between newly formed electron-hole pairs. Several factors have been identified as possible facilitators…

Mesoscale and Nanoscale Physics · Physics 2017-09-07 Mosè Casalegno , Raffaele Pastore , Julien Idé , Riccardo Po , Guido Raos

We discuss theoretical approaches to nonlinear optical spectroscopy of molecular junctions. Optical response functions are derived in the form convenient for implementation of Green function techniques, and their expressions in terms of…

Mesoscale and Nanoscale Physics · Physics 2016-06-28 Yi Gao , Michael Galperin

Electronic conductance through a single molecule is sensitive towards its structural orientation between two electrodes, owing to the distribution of molecular orbitals and their coupling to the electrode levels, that are governed by…

Mesoscale and Nanoscale Physics · Physics 2023-08-11 Koushik R. Das , Sudipta Dutta

An effective self-consistent model is derived and used to study the dynamics of an electron gas confined in a nonparabolic and anisotropic quantum well. This approach is based on the equations of quantum hydrodynamics, which incorporate…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Jerome Hurst , Kevin Leveque-Simon , Paul-Antoine Hervieux , Giovanni Manfredi , Fernando Haas

Using benzene sandwiched between two Au leads as a model system, we investigate from first principles the change in molecular conductance caused by different atomic structures around the metal-molecule contact. Our motivation is the…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

Intense spatio-spectral twin beams generated in the regime with pump depletion are analyzed applying a suggested quantum model that treats the signal, idler and pump fields in the same way. The model assumes the signal and idler fields in…

Quantum Physics · Physics 2017-09-26 Jan Perina

We study current rectification effect in an asymmetric molecule HOOC-C$_6$H$_4$-(CH$_2$)$_n$ sandwiched between two Aluminum electrodes using an {\sl ab initio} nonequilibrium Green function method. The conductance of the system decreases…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yan-hong Zhou , Xiao-hong Zheng , Ying Xu , Zhao Yang Zeng

We study inelastic electron tunneling through a molecular junction using the non-equilibrium Green function (NEGF) formalism. The effect of the mutual influence between the phonon and the electron subsystems on the electron tunneling…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Michael Galperin , Mark A. Ratner , Abraham Nitzan

The light-harvesting efficiency of a photoactive molecular complex is largely determined by the properties of its electronic quantum states. Those, in turn, are influenced by molecular vibrational states of the nuclear degrees of freedom.…

Biological Physics · Physics 2019-10-23 Hong-Guang Duan , Michael Thorwart , R. J. Dwayne Miller

Recent breakthroughs in quantum-dot circuit-quantum-electrodynamics (circuit-QED) systems are important both from a fundamental perspective and from the point of view of quantum photonic devices. However, understanding the applications of…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Jincheng Lu , Rongqian Wang , Jie Ren , Manas Kulkarni , Jian-Hua Jiang

Non-Hermitian quantum systems, governed by nonunitary evolution, offer powerful tools for manipulating quantum states through engineered loss. A prime example is coherent absorption, where quantum states undergo phase-dependent partial or…

Coupling between molecules and vacuum photon fields inside an optical cavity has proven to be an effective way to engineer molecular properties, in particular reactivity. To ease the rationalization of cavity induced effects we introduce an…

Chemical Physics · Physics 2022-04-06 Rosario R. Riso , Tor S. Haugland , Enrico Ronca , Henrik Koch

Strong correlations in two conjugate variables are the signature of quantum entanglement and have played a key role in the development of modern physics. Entangled photons have become a standard tool in quantum information and foundations.…

Quantum Physics · Physics 2019-07-24 Wuhong Zhang , Robert Fickler , Enno Giese , Lixiang Chen , Robert W. Boyd

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

Electromigrated nanoscale junctions have proven very useful for studying electronic transport at the single-molecule scale. However, confirming that conduction is through precisely the molecule of interest and not some contaminant or metal…

Mesoscale and Nanoscale Physics · Physics 2008-09-04 D. R. Ward , G. D. Scott , Z. K. Keane , N. J. Halas , D. Natelson

We analyze electronic excitations (excitations generated by adding or removing one electron) in the bulk of fractional quantum Hall states in Jain sequence states, using composite fermion Chern-Simons field theory. Starting from meanfield…

Mesoscale and Nanoscale Physics · Physics 2024-09-23 Xinlei Yue , Ady Stern

The linear thermoelectric properties of molecular junctions are theoretically studied close to room temperature within a model including electron-electron and electron-vibration interactions on the molecule. A nonequilibrium adiabatic…

Mesoscale and Nanoscale Physics · Physics 2015-11-26 C. A. Perroni , D. Ninno , V. Cataudella

We provide a unified theory of luminescence spectra of coupled light-matter systems realized with semiconductor heterostructures in microcavities, encompassing: i) the spontaneous emission case, where the system decays from a prepared…

Mesoscale and Nanoscale Physics · Physics 2009-07-09 Fabrice P. Laussy , Elena del Valle , Carlos Tejedor