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A mixed basis approach based on density functional theory is extended to one-dimensional(1D) systems. The basis functions here are taken to be the localized B-splines for the two finite non-periodic dimensions and the plane waves for the…

Materials Science · Physics 2016-04-20 Chung-Yuan Ren , Yia-Chung Chang , Chen-Shiung Hsue

We propose a framework to construct the ground-state energy and density matrix of an N-electron system by solving selfconsistently a set of single-particle equations. The method can be viewed as a non-trivial extension of the Kohn-Sham…

Chemical Physics · Physics 2009-11-13 D. Van Neck , S. Verdonck , G. Bonny , P. W. Ayers , M. Waroquier

We show how spectral functions for quantum impurity models can be calculated very accurately using a complete set of ``discarded'' numerical renormalization group eigenstates, recently introduced by Anders and Schiller. The only…

Strongly Correlated Electrons · Physics 2009-11-11 Andreas Weichselbaum , Jan von Delft

We present an \textit{ab initio} theory for superconductors, based on a unique mapping between the statistical density operator at equilibrium, on the one hand, and the corresponding one-body reduced density matrix $\gamma$ and the…

Superconductivity · Physics 2019-06-06 Jonathan Schmidt , Carlos L. Benavides-Riveros , Miguel A. L. Marques

A new method for calculating optical absorption spectra within linear-scaling density-functional theory (LS-DFT) is presented, incorporating a scheme for optimizing a set of localized orbitals to accurately represent unoccupied Kohn-Sham…

Materials Science · Physics 2015-05-30 Laura E. Ratcliff , Nicholas D. M. Hine , Peter D. Haynes

We develop a Green's function approach to quasiparticle excitations of open-shell systems within the GW approximation. It is shown that accurate calculations of the characteristic multiplet structure require a precise knowledge of the self…

Materials Science · Physics 2014-09-11 Johannes Lischner , Jack Deslippe , Manish Jain , Steven G. Louie

We present a new charge self-consistent scheme combining Density Functional and Dynamical Mean Field Theory, which uses Green's function of multiple scattering-type. In this implementation the many-body effects are incorporated into the…

Strongly Correlated Electrons · Physics 2017-10-11 A. Östlin , L. Vitos , L. Chioncel

Kohn-Sham (KS) density functional theory (DFT) is a very efficient method for calculating various properties of solids as, for instance, the total energy, the electron density, or the electronic band structure. The KS-DFT method leads to…

Materials Science · Physics 2019-09-20 Fabien Tran , Jan Doumont , Leila Kalantari , Ahmad W. Huran , Miguel A. L. Marques , Peter Blaha

Broadly speaking, the calculation of core spectra such as electron energy loss spectra (EELS) at the level of density functional theory (DFT) usually relies one of two approaches: conceptually more complex but computationally efficient…

As the second component of SPARC (Simulation Package for Ab-initio Real-space Calculations), we present an accurate and efficient finite-difference formulation and parallel implementation of Density Functional Theory (DFT) for extended…

Computational Physics · Physics 2017-05-24 Swarnava Ghosh , Phanish Suryanarayana

As the first component of SPARC (Simulation Package for Ab-initio Real-space Calculations), we present an accurate and efficient finite-difference formulation and parallel implementation of Density Functional Theory (DFT) for isolated…

Computational Physics · Physics 2017-01-04 Swarnava Ghosh , Phanish Suryanarayana

We re-adapt a spectral renormalization method, introduced in nonlinear optics, to solve the Kohn-Sham (KS) equations of density functional theory (DFT), with a focus on functionals based on the strictly-correlated electrons (SCE) regime,…

Strongly Correlated Electrons · Physics 2020-04-23 Juri Grossi , Ziad H. Musslimani , Michael Seidl , Paola Gori-Giorgi

Several different approximations and techniques have been developed for the calculation of atomic structure, ionization, and excitation of atoms and ions. These techniques have been used to compute large amounts of spectroscopic data of…

Astrophysics · Physics 2007-05-23 Manuel A. Bautista

We numerically investigate the Spin Density Functional theory for superconductors (SpinSCDFT) and the approximated exchange-correlation functional, derived and presented in the preceding paper I. As a test system we employ a free electron…

Superconductivity · Physics 2016-05-10 A. Linscheid , A. Sanna , E. K. U. Gross

In this work we give a comprehensive derivation of an exact and numerically feasible method to perform ab-initio calculations of quantum particles interacting with a quantized electromagnetic field. We present a hierachy of…

Accurate first-principles calculations for the energies, charge distributions, and spin symmetries of many-electron systems are essential to understand and predict the electronic and structural properties of molecules and materials.…

Chemical Physics · Physics 2024-01-24 Yuming Shi , Yi Shi , Adam Wasserman

A grid-based real-space implementation of the Projector Augmented Wave (PAW) method of P. E. Blochl [Phys. Rev. B 50, 17953 (1994)] for Density Functional Theory (DFT) calculations is presented. The use of uniform 3D real-space grids for…

Materials Science · Physics 2009-11-10 J. J. Mortensen , L. B. Hansen , K. W. Jacobsen

We present a method which enables solid-state density functional theory calculations to be applied to systems of almost unlimited size. Computations of physical effects up to the micron length scale but which nevertheless depend on the…

Materials Science · Physics 2021-01-04 Tristan Müller , Sangeeta Sharma , E. K. U. Gross , J. K. Dewhurst

We investigate the pseudospectrum of the Kerr black hole, which indicates the instability of the spectrum of quasinormal modes (QNMs) of the Kerr black hole. Methodologically, we use the hyperboloidal framework to cast the QNM problem into…

General Relativity and Quantum Cosmology · Physics 2025-03-13 Rong-Gen Cai , Li-Ming Cao , Jia-Ning Chen , Zong-Kuan Guo , Liang-Bi Wu , Yu-Sen Zhou

Spectral polynomial approximation of smooth functions allows real-time manipulation of and computation with them, as in the Chebfun system. Extension of the technique to two-dimensional and three-dimensional functions on hyperrectangles has…

Numerical Analysis · Mathematics 2019-01-21 Kevin W. Aiton , Tobin A. Driscoll
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