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Multipolar order in bulk crystalline solids is characterized by multipole densities -- denoted as polarizations in this work -- that cannot be cleanly defined using the concepts of classical electromagnetism. Here we use group theory to…
This paper presents a first-principle and global perspective of electromagnetic chirality. It follows for this purpose a bottom-up construction, from the description of chiral particles or metaparticles (microscopic scale), through the…
Electric and magnetic multipole densities in crystalline solids, including the familiar electric dipole density in ferroelectrics and the magnetic dipole density in ferromagnets, are of central importance for our understanding of ordered…
Chiral and axial materials offer platforms for intriguing phenomena, such as cross-correlated responses and chirality-induced spin selectivity. However, quantifying the properties of such materials has generally been considered challenging.…
Four types of atomic-scale multipoles, electric, magnetic, magnetic toroidal, and electric toroidal multipoles, give a complete set to describe arbitrary degrees of freedom for coupled charge, spin, and orbital of electrons. We here present…
In this short article, we overview a concept of electronic toroidal multipoles, and their ordering with associated physical properties in non-magnetic and magnetic materials. The toroidal multipoles are introduced as microscopic electronic…
Mutual interplay between the electronic degrees of freedom in solids, such as charge, spin, orbital, sublattice, and bond degrees of freedom, is a source of cross-correlated phenomena with unconventional electronic ordered states. Such…
Chirality refers to the asymmetry of objects that cannot be superimposed on their mirror image. It is a concept that exists in various scientific fields and has profound consequences. Although these are perhaps most widely recognized within…
Microscopic origin of chirality and possible electric-field induced rotation and rotation-field induced electric polarization are investigated. By building up a realistic tight-binding model for elemental Te crystal in terms of…
Here by combining a symmetry-based analysis with numerical computations we predict a new kind of magnetic ordering - antichiral ferromagnetism. The relationship between chiral and antichiral magnetic order is conceptually similar to the…
Natural optical activity is the paradigmatic example of an effect originating in the weak spatial inhomogeneity of the electromagnetic field on the atomic scale. In molecules, such effects are well described by the multipole theory of…
Plasmonic chirality exhibits great potential for novel nanooptical devices due to the generation of a strong chiroptical response. Previous reports on plasmonic chirality explanations are mainly based on phase retardation and coupling. We…
In solid state physics, any symmetry breaking is known to be associated with emergence of an order parameter. However, the order parameter for molecular and crystal chirality, which is a consequence of parity and mirror symmetry breaking,…
It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…
A feature of the "modern theory" is that electric polarization is not well-defined in a metallic ground state. A different approach invokes the general existence of a complete set of exponentially localized Wannier functions, with respect…
In chemistry and biochemistry, chirality represents the structural asymmetry characterized by non-superimposable mirror images for a material like DNA. In physics, however, chirality commonly refers to the spin-momentum locking of a…
The multipole moment is an established concept of electrons in solids. Entanglement of spin, orbital, and sublattice degrees of freedom is described by the multipole moment, and spontaneous multipole order is a ubiquitous phenomenon in…
A whole series of expressions for four species of multipoles (electric, magnetic, magnetic toroidal, and electric toroidal) is provided as a complete basis set to describe arbitrary single-centered spinful electron systems. A compact…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
Spin-dependent electric dipole operators are investigated group-theoretically for the emergence of an electric dipole induced by a single spin or by two spins, where the spin dependences are completely classified up to the quadratic order.…