Related papers: Metastable doubly-charged Rydberg molecules
In molecules like hydrogen, most chemical bonds are formed by sharing two electrons from each atom in the bonding molecular orbital (two-center-two-electron (2c2e) bonding). There are, however, different kinds of chemical bonding. The I3-…
Rydberg atom arrays constitute a promising quantum information platform, where control over several hundred qubits has been demonstrated. Further scaling could significantly benefit from coupling to integrated optical or electronic devices,…
Optically trapped Rydberg atoms are a suitable platform to explore quantum many-body physics mediated by long-range atom--atom interactions that can be engineered through externally applied light fields. However, this approach is limited to…
Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…
Highly excited Rydberg atoms inherit their level structure, symmetries, and scaling behavior from the hydrogen atom. We demonstrate that these fundamental properties enable a thermodynamic limit of a single Rydberg atom subjected to…
We propose a promising hybrid quantum system, where a highly-excited atom strongly interacts with a superconducting LC oscillator via the electric field of capacitor. An external electrostatic field is applied to tune the energy spectrum of…
As resonantly interacting trimers of the type AAB are progressively squeezed from $D=3$ to $D=2$, unatomic states emerge. We calculated the contacts from the high momentum tail of the single particle densities. The sharp increase of the…
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit…
Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies.…
The structure of the low-lying rotational levels of the X$^+$ $ ^2 \Sigma_g ^+$ ($v^+=0$) vibronic ground state of para-H$_2^+$ has been determined by combining frequency-comb calibrated continuous-wave high-resolution laser spectroscopy of…
High-fidelity entangled Bell states are of great interest in quantum physics. Entanglement of ultracold neutral atoms in two spatially separated optical dipole traps is promising for implementation of quantum computing and quantum…
Rydberg atom arrays are powerful platforms for studying quantum many-body systems. We consider the Rydberg-Ising Hamiltonian on periodic chains and numerically study ensembles of states generated by random global pulse sequences subject to…
The formation of ultralong-range Rydberg molecules is a result of the attractive interaction between Rydberg electron and polarizable ground state atom in an ultracold gas. In the nondegenerate case the backaction of the polarizable atom on…
Three-body F\"orster resonances at long-range interactions of Rydberg atoms were first predicted and observed in Cs Rydberg atoms by R.Faoro et al., Nature Comm. 6, 8173 (2015). In these resonances, one of the atoms carries away an energy…
Coupling electronic and vibrational degrees of freedom of Rydberg atoms held in optical tweezer arrays offers a flexible mechanism for creating and controlling atom-atom interactions. We find that the state-dependent coupling between…
Obtaining full control over the internal and external quantum states of molecules is the central goal of ultracold chemistry and allows for the study of coherent molecular dynamics, collisions and tests of fundamental laws of physics. When…
Rydberg atoms in dc electric fields acquire static dipole moments. When the atoms are close to a surface producing an inhomogeneous electric field, such as by the adsorbates on an atom chip, depending on the sign of the dipole moment of the…
Atoms in highly excited Rydberg states exhibit remarkable properties and constitute a powerful tool for studying quantum phenomena in strongly interacting many-particle systems. We investigate alkali atoms that are held in a ring lattice…
Bound states of massive particles, such as nuclei, atoms or molecules, constitute the bulk of the visible world around us. In contrast, photons typically only interact weakly. We report the observation of traveling three-photon bound states…
We report the creation of a sample of over 1000 ultracold $^{87}$RbCs molecules in the lowest rovibrational ground state, from an atomic mixture of $^{87}$Rb and Cs, by magnetoassociation on an interspecies Feshbach resonance followed by…