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We consider the problem of determining the spectrum of an electronic spin via polarization transfer to coupled nuclear spins and their subsequent readout. This suggests applications for employing dynamic nuclear polarization (DNP) for…

Quantum Physics · Physics 2021-10-19 Moniish Elanchezhian , Arjun Pillai , Teemu Virtanen , Ashok Ajoy

A method and codes for two-step correlation calculation of heavy-atom molecules have been developed, employing the generalized relativistic effective core potential and relativistic coupled cluster (RCC) methods at the first step, followed…

Chemical Physics · Physics 2009-11-07 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov , V. F. Ezhov , E. Eliav , U. Kaldor

The connections between the Random Phase Approximation (RPA) and Many-Body Perturbation Theory (MBPT) and its all order generalisation, the Coupled- Cluster Theory (CCT) have been explored. Explicit expressions have been derived for the…

Background: Time-reversal-invariance violation, or equivalently CP violation, may explain the observed cosmological baryon asymmetry as well as signal physics beyond the Standard Model. In the decay of polarized neutrons, the triple…

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

Parity-violating nuclear force, as may be accessed from parity violation studies in nuclear systems, represents an area of nonleptonic weak interactions which has been the subject of experimental investigations for several decades. In the…

High Energy Physics - Phenomenology · Physics 2009-11-13 W-Y. P. Hwang , Chih-Yi Wen

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Spin complexes comprising the nitrogen-vacancy (NV) center and neighboring spins are being considered as a building block for a new generation of spintronic and quantum information processing devices. Because assembling identical spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-08 Abdelghani Laraoui , Florian Dolde , Christian Burk , Friedemann Reinhard , Jörg Wrachtrup , Carlos A. Meriles

Experiments searching for the electric dipole moment (EDM) of the electron $d_e$ utilise atomic/molecular states with one or more uncompensated electron spins, and these paramagnetic systems have recently achieved remarkable sensitivity to…

High Energy Physics - Phenomenology · Physics 2020-08-12 V. V. Flambaum , M. Pospelov , A. Ritz , Y. V. Stadnik

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

Materials Science · Physics 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

In order to explore the effects of high levels of electron correlation on the real-time coupled cluster formalism and algorithmic behavior, we introduce a time-dependent implementation of the CC3 singles, doubles and approximate triples…

Chemical Physics · Physics 2025-01-23 Zhe Wang , Håkon Emil Kristiansen , Thomas Bondo Pedersen , T. Daniel Crawford

We develop a method based on the relativistic coupled-cluster theory to incorporate a perturbative interaction to the no-pair Dirac-Coulomb atomic Hamiltonian. The method is general and suitable to incorporate any perturbation Hamiltonian…

Atomic Physics · Physics 2012-09-06 S. Chattopadhyay , B. K. Mani , D. Angom

A permanent electric dipole moment of fundamental spin-1/2 particles violates both parity (P) and time re- versal (T) symmetry, and hence, also charge-parity (CP) symmetry since there is no sign of CPT-violation. The search for a neutron…

Currently the theoretical uncertainty limits the interpretation of the atomic parity non-conservation (PNC) measurements. We calculate the PNC $5s$ - $6s$ electric dipole transition amplitude in rubidium and demonstrate that rubidium is a…

Atomic Physics · Physics 2013-05-14 V. A. Dzuba , V. V. Flambaum , B. Roberts

The atomic parity non-conservation(PNC) experiments has reached accuracies which have important implications for physics beyond the standard model. An optical rotation experiment to measure the atomic PNC of the 3P1(6s6p)--1P1(6s6p) in Yb…

Atomic Physics · Physics 2007-05-23 Angom Dilip Singh , Bhanu Pratap Das

The electric dipole moment of atomic $^{199}$Hg induced by the nuclear Schiff moment and tensor-pseudotensor electron-nucleus interactions has been calculated. For this, we have developed and employed a novel method based on the…

Atomic Physics · Physics 2009-12-29 K. V. P. Latha , D. Angom , B. P. Das , D. Mukherjee

Finite temperature results in various effects on the properties of nuclear structure and excitations of relevance for nuclear processes in hot stellar environments. Here we introduce the self-consistent finite temperature relativistic…

Nuclear Theory · Physics 2023-10-03 Amandeep Kaur , Esra Yüksel , Nils Paar

The RPA long range correlations are known to play a significant role in understanding the depletion of single particle-hole states observed in (e, e') and (e, e'p) measurements. Here the Random Phase Approximation (RPA) theory, implemented…

Nuclear Theory · Physics 2009-11-11 M. Dupuis , S. Karataglidis , E. Bauge , J. P. Delaroche , D. Gogny

Several experimental investigations have observed parity violation in nuclear systems-a consequence of the weak force between quarks. We apply the $1/N_c$ expansion of QCD to the P-violating T-conserving component of the nucleon-nucleon…

Nuclear Theory · Physics 2015-03-05 Daniel R. Phillips , Daris Samart , Carlos Schat

Understanding the origins of spin lifetimes in hybrid quantum systems is a matter of current importance in several areas of quantum information and sensing. Methods that spectrally map spin relaxation processes provide insight into their…

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