Related papers: Revealing Quadrupolar Excitations with Non-Linear …
Identifying quantum spin liquids, magnon breakdown, or fractionalized excitations in quantum magnets is an ongoing challenge due to the ambiguity of possible origins of excitation continua occurring in linear response probes. Recently, it…
Two-dimensional coherent spectroscopy (2DCS) is an established method for characterizing molecules and has been proposed in the THz regime as a new tool for probing exotic excitations of quantum magnets; however, the precise nature of the…
Two-dimensional coherent spectroscopy (2DCS) is a nonlinear spectroscopy technique capable of identifying whether apparent continua in linear response are made out of multiplets of sharp deconfined quasiparticles. This makes it a potent…
Two dimensional coherent spectroscopy (2DCS) probes the nonlinear optical response of correlated systems. An interesting application is the study of fractionalized excitations, which are challenging to distinguish unambiguously in linear…
We use a Rydberg quantum simulator to demonstrate a new form of spectroscopy, called quench spectroscopy, which probes the low-energy excitations of a many-body system. We illustrate the method on a two-dimensional simulation of the…
The square-lattice quantum Heisenberg antiferromagnet displays a pronounced anomaly of unknown origin in its magnetic excitation spectrum. The anomaly manifests itself only for short wavelength excitations propagating along the direction…
Inelastic neutron scattering (INS) has traditionally been one of the primary methods for investigating quantum magnets, particularly in identifying a continuum of excitations as a hallmark of spin fractionalization in quantum spin liquids…
Assemblies of interacting quantum particles often surprise us with properties that are difficult to predict. One of the simplest quantum many-body systems is the spin 1/2 Heisenberg antiferromagnetic chain, a linear array of interacting…
One-dimensional (1D) magnetic insulators have attracted significant interest as a platform for studying emergent phenomena such as quasiparticle fractionalization and quantum criticality. The antiferromagnetic Heisenberg chain of spins-1/2…
Two-dimensional correlation spectroscopy (2DCS) based on the nonlinear optical response of excitons to sequences of ultrafast pulses, has the potential to provide some unique insights into carrier dynamics in semiconductors. The most…
With recent advances in terahertz (THz) sources and detection, two-dimensional coherent spectroscopy (2DCS), which allows to probe nonlinear responses in a two-frequency plane, now reaches the meV regime relevant for quasiparticle…
The microscopic origins of emergent behaviours in condensed matter systems are encoded in their excitations. In ordinary magnetic materials, single spin-flips give rise to collective dipolar magnetic excitations called magnons. Likewise,…
Two-dimensional coherent spectroscopy (2DCS) with terahertz radiation offers a promising new avenue for the exploration of many-body phenomena in quantum magnets. This includes the potential diagnosis of fractionalized excitations, for…
We study nonlinear response in quantum spin systems {near infinite-randomness critical points}. Nonlinear dynamical probes, such as two-dimensional (2D) coherent spectroscopy, can diagnose the nearly localized character of excitations in…
Exotic spin-multipolar ordering in spin transition metal insulators has so far eluded unambiguous experimental observation. A less studied, but perhaps more feasible fingerprint of multipole character emerges in the excitation spectrum in…
Resonant inelastic x-ray scattering (RIXS) is an evolving tool for investigating spin dynamics of strongly correlated materials, which complements inelastic neutron scattering. Both techniques have found that non-spin-conserving (NSC)…
Two-dimensional coherent terahertz spectroscopy (2DCS) emerges as a valuable tool to probe the nature, couplings, and lifetimes of excitations in quantum materials. It thus promises to identify unique signatures of spin liquid states in…
Topological non-collinear magnetic phases of matter are at the heart of many proposals for future information nanotechnology, with novel device concepts based on ultra-thin films and nanowires. Their operation requires understanding and…
Investigation of dynamical excitations is difficult but crucial to the understanding of many exotic quantum phenomena discovered in quantum materials. This is particularly true for highly frustrated quantum antiferromagnets whose dynamical…
In this paper, equations describing one-dimensional Non-Heisenberg model are studied by use of generalized coherent states in real parameterization and then dissipative spin wave equation for dipole and quadrupole branches is obtained if…