Related papers: Tracking chirality in photoelectron circular dichr…
3D photoelectron angular distributions (PADs) are measured from an atomic target ionized by ultrafast, elliptical fields of opposite handedness. Comparing these PADs to one another and to numeric simulations, a difficult to avoid systematic…
Chirality is a pervasive property of matter that underpins many important phenomena across physics, chemistry and biology. Given its broad significance, the development of protocols for rational control of chirality in solid state systems…
Controlling optical chirality at the subwavelength scales is essential for many applications of nanophotonic structures in polarization optics, sensing, and nonlinear photonics. Achieving a strong chiroptical response in planar dielectric…
The variation of the optical absorption of carbon nanotubes with their geometry has been a long standing question at the heart of both metrological and applicative issues, in particular because optical spectroscopy is one of the primary…
Circular dichroism covering the telecommunication band is experimentally demonstrated in a semiconductor-based three-dimensional chiral photonic crystal (PhC). We design a rotationally-stacked woodpile PhC structure where neighboring layers…
Chiroptical techniques for detecting and characterizing the chirality of matter and artificial nanostructures are traditionally based on their interaction with chiral light, typically circularly-polarized fields propagating in free space.…
We derive a set of design requirements that lead to structures suitable for molecular circular dichroism (CD) enhancement. Achirality of the structure and two suitably selected sequentially incident beams of opposite helicity ensures that…
Chirality is a fundamental property of electrons with the relativistic spectrum found in graphene and topological insulators. It plays a crucial role in relativistic phenomena, such as Klein tunneling, but it is difficult to visualize…
We show that the photoelectron angular distributions produced by elliptical and cross-polarized two-color laser fields interacting with randomly oriented chiral molecules decompose into four irreducible representations of the $D_{2h}$ point…
Visualizing and controlling electron dynamics over femtosecond timescale play a key role in the design of next-generation electronic devices. Using simulations, we demonstrate the electronic oscillation inside the naphthalene molecule can…
Chirality is an intriguing property of certain molecules, materials or artificial nanostructures, which allows them to interact with the spin angular momentum of the impinging light field. Due to their chiral geometry, they can distinguish…
We compare the various chirality measures most widely used in the literature to quantify chiral symmetry in extended solids, i.e., the continuous chirality measure, the Hausdorff distance, and the angular momentum. By studying these…
In continuum mechanics, the non-centrosymmetric micropolar theory is usually used to capture the chirality inherent in materials. However when reduced to a two dimensional (2D) isotropic problem, the resulting model becomes non-chiral.…
Circular dichroism (CD), i.e. the differential response of a system to left and right circularly polarized light, is one of the only techniques capable of providing morphological information of certain samples. In biology, for instance, CD…
This paper presents a first-principle and global perspective of electromagnetic chirality. It follows for this purpose a bottom-up construction, from the description of chiral particles or metaparticles (microscopic scale), through the…
A techniques, describing electron dynamics for magnetic models closed to cyclical accelerators, is developed and applied to the analysis of electromagnetic radiation emitted by charged particles. Formulas for the angular characteristics of…
We propose an alternative approach to the description and analysis of photoelectron angular distributions (PADs) resulting from isotropic samples in the case of few-photon absorption via electric fields of arbitrary polarization. As we…
Molecular chirality is conventionally understood as space-inversion-symmetry breaking in the equilibrium structure of molecules. Less well known is that achiral molecules can be made chiral through extreme rotational excitation. Here, we…
Chiral phonons have been proposed to be involved in various physical phenomena, yet the chirality of molecular normal modes has not been well defined mathematically. Here we examine two approaches for assigning and quantifying the chirality…
Circular dichroism (CD) is in widespread use as a means of determining enantiomeric excess. We show how slow-light phenomena in dispersive structured media allow for a reduction in the required optical path length of an order of magnitude.…