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Dynamic Nuclear Polarization (DNP) presently stands as the preferred strategy to enhance the sensitivity of nuclear magnetic resonance measurements, but its application relies on the use of high-frequency microwave to manipulate electron…

Mesoscale and Nanoscale Physics · Physics 2022-02-02 Carlos A. Meriles , Pablo R. Zangara

Scanning probe microscopy with multi-qubit sensors offers the potential to improve imaging speed and measure previously inaccessible quantities, such as two-point correlations. We develop a multiplexed quantum sensing approach with scanning…

Quantum Physics · Physics 2025-10-09 William S. Huxter , Federico Dalmagioni , Christian L. Degen

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

The efficiency of dipole-dipole coupling driven coherence transfer experiments in solid-state NMR spectroscopy of powder samples is limited by dispersion of the orientation of the internuclear vectors relative to the external magnetic…

Quantum Physics · Physics 2009-11-13 N. Khaneja , C. Kehlet , S. J. Glaser , N. C. Nielsen

In recent years, nitrogen-vacancy (NV) color centers in diamond have become excellent solid-state quantum sensors due to their electronic spin properties. Especially for their easy optical initialization and detection, together with their…

Diamonds with nitrogen-vacancy (NV) center ensembles are one of the most promising solid-state quantum platforms for various sensing applications. The combination of a long spin dephasing time ($T_2^*$) and a high NV center concentration is…

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of…

Solid state spins in diamond, in particular negatively charged nitrogen-vacancy centers (NV), are leading contenders in the field of quantum sensing. While addressing of single NVs offers nanoscale spatial resolution, many implementations…

Quantum Physics · Physics 2023-01-11 Yuchun Zhu , Elena Losero , Christophe Galland , Valentin Goblot

For decades, searches for exotic spin interactions have used increasingly-precise laboratory measurements to test various theoretical models of particle physics. However, most searches have focused on interaction length scales greater than…

Quantum Physics · Physics 2022-07-04 P. -H. Chu , N. Ristoff , J. Smits , N. Jackson , Y. J. Kim , I. Savukov , V. M. Acosta

We present a new method for high-resolution nanoscale magnetic resonance imaging (nano-MRI) that combines the high spin sensitivity of nanowire-based magnetic resonance detection with high spectral resolution nuclear magnetic resonance…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 William Rose , Holger Haas , Angela Q. Chen , Nari Jeon , Lincoln J. Lauhon , David G. Cory , Raffi Budakian

We present the architecture of the versatile NMR spectrometer with software-defined radio (SDR) technology and its application to the dynamically controlled pulsed magnetic fields. The pulse-field technology is the only solution to access…

Strongly Correlated Electrons · Physics 2021-11-24 Yoshihiko Ihara , Kaoru Hayashi , Tomoki Kanda , Kazuki Matsui , Koichi Kindo , Yoshimitsu Kohama

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

Spin ensembles of nitrogen vacancy (NV) centers in diamond are emerging as powerful spin-based sensors for magnetic, electric and thermal field imaging with high spatial and temporal resolution. Here we characterize the formation of…

Materials Science · Physics 2019-11-13 Tim R. Eichhorn , Claire A. McLellan , Ania C. B. Jayich

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…

Wide field-of-view magnetic field microscopy has been realised by probing shifts in optically detected magnetic resonance (ODMR) spectrum of Nitrogen Vacancy (NV) defect centers in diamond. However, these widefield diamond NV magnetometers…

Mesoscale and Nanoscale Physics · Physics 2022-02-28 Madhur Parashar , Anuj Bathla , Dasika Shishir , Alok Gokhale , Sharba Bandyopadhyay , Kasturi Saha

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang

Optically active spin defects in solids offer promising platforms to investigate nuclear spin clusters with high sensitivity and atomic-site resolution. To leverage near-surface defects for molecular structure analysis in chemical and…

Scalar couplings between covalently bound nuclear spins are a ubiquitous feature in nuclear magnetic resonance (NMR) experiments, imparting valuable information to NMR spectra regarding molecular structure and conformation. Such couplings…

Chemical Physics · Physics 2011-12-26 Micah Ledbetter , Giacomo Saielli , Alessandro Bagno , Nhan Tran , Michael Romalis

We introduce a double quantum (DQ) 4-Ramsey measurement protocol that enables wide-field magnetic imaging using nitrogen vacancy (NV) centers in diamond, with enhanced homogeneity of the magnetic sensitivity relative to conventional single…

We investigate the application of amplitude-shaped control pulses for enhancing the time and frequency resolution of multipulse quantum sensing sequences. Using the electronic spin of a single nitrogen vacancy center in diamond and up to…

Quantum Physics · Physics 2018-01-03 J. Zopes , K. Sasaki , K. S. Cujia , J. M. Boss , K. Chang , T. F. Segawa , K. M. Itoh , C. L. Degen