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Quantum computers are special purpose machines that are expected to be particularly useful in simulating strongly correlated chemical systems. The quantum computer excels at treating a moderate number of orbitals within an active space in a…

Single-particle methods based on Kohn-Sham unoccupied states to describe near-edge X-ray absorption (XAS) spectra are routinely applied for the description of K-edge spectra, as there is no complication due to spin-orbit (SO) coupling. L-…

Materials Science · Physics 2026-02-26 Esther A. B. Johnsen , Naoki Horiuchi , Toma Susi , Michael Walter

It is imperative that useful quantum computers be very difficult to simulate classically; otherwise classical computers could be used for the applications envisioned for the quantum ones. Perfect quantum computers are unarguably…

Quantum Physics · Physics 2020-11-26 Yiqing Zhou , E. Miles Stoudenmire , Xavier Waintal

Computed tomography (CT) is an important imaging technique used in medical analysis of the internal structure of the human body. Previously, image segmentation methods were required after acquiring reconstructed CT images to obtain…

Quantum Physics · Physics 2024-09-17 Kyungtaek Jun

We introduce a machine-learning-based approach to enhance the sensitivity of optical-extreme ultraviolet (XUV) transient absorption spectroscopy. A reference spectrum is used as input to a three-layer feed-forward neural network, allowing…

Optics · Physics 2023-05-04 Tobias Heinrich , Hung-Tzu Chang , Sergey Zayko , Murat Sivis , Claus Ropers

Gaussian boson sampling, a computational model that is widely believed to admit quantum supremacy, has already been experimentally demonstrated and is claimed to surpass the classical simulation capabilities of even the most powerful…

Quantum Physics · Physics 2023-11-17 Minzhao Liu , Changhun Oh , Junyu Liu , Liang Jiang , Yuri Alexeev

To simulate bosons on a qubit- or qudit-based quantum computer, one has to regularize the theory by truncating infinite-dimensional local Hilbert spaces to finite dimensions. In the search for practical quantum applications, it is important…

Quantum Physics · Physics 2024-04-03 Masanori Hanada , Junyu Liu , Enrico Rinaldi , Masaki Tezuka

Simulations of scattering processes are essential in understanding the physics of our universe. Computing relevant scattering quantities from ab initio methods is extremely difficult on classical devices because of the substantial…

The recent rapid experimental advancement in the engineering of quantum many-body systems opens the avenue to controlled studies of fundamental physics problems via digital or analog quantum simulations. Here, we systematically analyze the…

Strongly Correlated Electrons · Physics 2022-02-25 Johannes Knaute , Philipp Hauke

The promise of quantum computing to circumvent the exponential scaling of quantum chemistry has sparked a race to develop chemistry algorithms for quantum architecture. However, most works neglect the quantum-inherent shot noise, let alone…

The validation of a previous work on the optimization of material discrimination in spectral x-ray imaging is reported. Using Monte Carlo simulations based on the BEAMnrc package, material decomposition was performed on the projection…

Medical Physics · Physics 2015-06-18 Syen J. Nik , Rune S. Thing , Richard Watts , Tony Dale , Bryn Currie , Juergen Meyer

Conventional absorption spectroscopy relies on coherent laser sources, and in turn suffers from the inherent limitation of shot noise, especially in estimating weak absorption. Here we propose a measurement strategy with correlated photons…

Quantum Physics · Physics 2025-04-17 Zhucheng Zhang , Xue Zhang , Jing Liu , Hui Dong

The throughout knowledge of a X-ray beam spectrum is mandatory to assess the quality of its source device. Since the techniques to directly measurement such spectra are expensive and laborious, the X-ray spectrum reconstruction using…

Computational Physics · Physics 2014-11-12 Olavo Henrique Menin , Alexandre Souto Martinez , Alessandro Martins da Costa

Quantum batteries are predicted to have the potential to outperform their classical counterparts and are therefore an important element in the development of quantum technologies. Of particular interest is the role of correlations in…

We have studied the Stark effect in the soft x-ray region for various small molecules by calculating the field-dependent x-ray absorption spectra. This effect is explained in terms of the response of molecular orbitals (core and valence),…

Chemical Physics · Physics 2025-03-26 Avdhoot Datar , Catherine Wright , Devin A. Matthews

The complex-scaling method can be used to calculate molecular resonances within the Born-Oppenheimer approximation, assuming the electronic coordinates are dilated independently of the nuclear coordinates. With this method, one will…

Quantum Physics · Physics 2021-06-16 Teng Bian , Sabre Kais

Many quantum algorithms can be seen as a transition from a well-defined initial quantum state of a complex quantum system, to an unknown target quantum state, corresponding to a certain eigenvalue either of the Hamiltonian or of a…

Quantum Physics · Physics 2022-07-19 Aikaterini Mandilara , Daniil Fedotov , Vladimir M. Akulin

Quantum computing could impact various industries, with the automotive industry with many computational challenges, from optimizing supply chains and manufacturing to vehicle engineering, being particularly promising. This chapter…

We present quantum algorithms for the estimation of n-time correlation functions, the local and non-local density of states, and dynamical linear response functions. These algorithms are all based on block-encodings - a versatile technique…

Quantum Physics · Physics 2020-08-19 Patrick Rall

Quantum computing has recently exhibited great potentials in predicting chemical properties for various applications in drug discovery, material design, and catalyst optimization. Progress has been made in simulating small molecules, such…