Related papers: Dual-grating single-shot pump-probe technique
Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…
The simulation of rare events is one of the key problems in atomistic simulations. Towards its solution a plethora of methods have been proposed. Here we combine two such methods metadynamics and inte-grated tempering sampling. In…
Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…
Ultrafast-optical-pump -- structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying…
The development of many optical quantum technologies depends on the availability of solid-state single quantum emitters with near-perfect optical coherence. However, a standing issue that limits systematic improvement is the significant…
Phase-sensitive pump-probe hyperspectral imaging is a precise technique for absolute two-beam measurements of the optical Kerr coefficient ($n_2$). The irradiance profile is characterized and background effects are rejected by rastering the…
We present a fast active microrheology technique exploring the phase response of a microscopic probe particle trapped in a linear viscoelastic fluid using optical tweezers under an external perturbation. Thus, we experimentally determine…
This paper describes a scheme for pump-probe experiments that can be performed at LCLS and at the European XFEL and determines what additional hardware development will be required to bring these experiments to fruition. It is proposed to…
Ultrafast pump-probe experiments open the possibility to track fundamental material behaviour like changes in its electronic configuration in real time. To date, most of these experiments are performed using an electron or a high-energy…
We theoretically investigate the generation of two entangled beams of light in the process of single-pass type-I noncollinear frequency degenerate parametric downconversion with an ultrashort pulsed pump. We find the spatio-temporal…
We describe an ultrafast time resolved pump-probe spectroscopy setup aimed at studying the switching of nanophotonic structures. Both fs pump and probe pulses can be independently tuned over broad frequency range between 3850 and 21050…
Pump-probe methods are a ubiquitous tool in the field of ultrafast dynamic measurements. In recent years, x-ray free-electron laser experiments have gained importance due to their ability to probe with high chemical selectivity and at…
Single-shot characterization techniques are crucial when dealing with shot-to-shot pulse-shape fluctuations (e.g., unstable laser systems, high-power, or with low repetition rate) since the scanning configurations cannot measure single…
We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…
Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…
We introduce an ultrafast, bright, entangled twin-beam source generated by type-0 parametric down-conversion in periodically-poled lithium niobate at MHz repetition rate, with continuously tunable Schmidt number $K$ set by the pump pulse…
We present a pump-probe technique for monitoring ultrafast polarizability changes. In particular, we use it to measure the plasma density created at the temporal focus of a self-compressing higher-order pump soliton in gas-filled…
Bright single photon emission from single quantum dots in suspended circular Bragg grating microcavities is demonstrated. This geometry has been designed to achieve efficient (> 50 %) single photon extraction into a near-Gaussian shaped…
We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…