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We reveal by first-principles calculations that the interlayer binding in a twisted MoS2/MoTe2 heterobilayer decreases with increasing twist angle, due to the increase of the interlayer overlapping degree, a geometric quantity describing…

Materials Science · Physics 2020-10-07 W. T. Geng , V. Wang , J. B. Lin , T. Ohno , J. Nara

Manipulating the interlayer magnetic coupling in van der Waals magnetic materials and heterostructures is the key to tailoring their magnetic and electronic properties for various electronic applications and fundamental studies in condensed…

Materials Science · Physics 2020-08-19 Zhe Li , Jiaheng Li , Ke He , Xiangang Wan , Wenhui Duan , Yong Xu

The interlayer couplings in commensurate and incommensurate bilayer structures of transition metal dichalcogenides are investigated with perturbative treatment. The interlayer coupling in \pm K valleys can be decomposed into a series of…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 Yong Wang , Zhan Wang , Wang Yao , Gui-Bin Liu , Hongyi Yu

Layered two-dimensional (2D) materials exhibit unique properties, expanding opportunities in material design. We investigate MX$_2$ transition metal dichalcogenides (TMDCs) (M = Mo, W; X = S, Se, Te) in homo- and heterobilayers with…

Materials Science · Physics 2025-03-13 Yu-Hsiu Lin , William P. Comaskey , Jose L. Mendoza-Cortes

Layered MA$_2$Z$_4$ compounds, structural relatives of MoS$_2$ discovered in 2020, exhibit rich magnetic behavior arising from reduced dimensionality, noncentrosymmetric lattice symmetries, and stacking-dependent exchange interactions.…

Materials Science · Physics 2026-02-10 Brandon Pedroza-Rojas , David W. Facemyer , Ariadna Sánchez-Castillo

In this work, we have presented a first principle simulation study on the electronic properties of MoS2/MX2/MoS2 (M=Mo or W; X=S or Se) trilayer heterostrcuture. We have investigated the effect of stacking configuration, bi-axial…

Computational Physics · Physics 2018-02-27 Kanak Datta , Quazi D. M. Khosru

Recent experimental synthesis of ambient-stable MoSi2N4 monolayer have garnered enormous research interests. The intercalation morphology of MoSi2N4 - composed of a transition metal nitride (Mo-N) inner sub-monolayer sandwiched by two…

The interlayer coupling is emerging as a new parameter for tuning the physical properties of two-dimensional (2D) van der Waals materials. When two identical semiconductor monolayers are stacked with a twist angle, the periodic interlayer…

Mesoscale and Nanoscale Physics · Physics 2022-09-16 Jing Liang , Dongyang Yang , Jingda Wu , Jerry I Dadap , Kenji Watanabe , Takashi Taniguchi , Ziliang Ye

The atomic-level vdW heterostructures have been one of the most interesting quantum material systems, due to their exotic physical properties. The interlayer coupling in these systems plays a critical role to realize novel physical…

Strongly Correlated Electrons · Physics 2021-03-16 Xiaoli Ma , Shaohua Fu , Jianwei Ding , Meng Liu , Ang Bian , Fang Hong , Jia-Tao Sun , Xiaoxian Zhang , Xiaohui Yu , Dawei He

The recent synthesis of MoSi2N4 material, along with theoretical predictions encompassing the entire family of chemical analogs, has opened up a new array of low-dimensional materials for a diverse range of optoelectronics and photovoltaics…

Materials Science · Physics 2023-09-21 Muhammad Sufyan Ramzan , Tomasz Woźniak , Agnieszka Kuc , Caterina Cocchi

Based on first-principles calculations, we have investigated the structural stability, electronic structures, and thermal properties of the monolayer XSi2N4 (X= Ti, Mo, W) and their lateral (LH) and vertical heterostructures (VH). We find…

Materials Science · Physics 2022-03-29 Ghulam Hussain , Mazia Asghar , Muhammad Waqas Iqbal , Hamid Ullah , Carmine Autieri

Interlayer coupling can significantly influence the physical properties of layered transition metal compounds. The superconductivity in layered Mo$_2$C systems, belonging to the emergent family of MXene, has garnered considerable attention.…

Superconductivity · Physics 2024-02-22 Can Hong , Danhong Wu , Xi-Bo Li , Feipeng Zheng

Van der Waals (vdW) heterobilayers formed by two-dimensional (2D) transition metal dichalcogenides (TMDCs) created a promising platform for various electronic and optical properties. ab initio band results indicate that the band offset of…

Materials Science · Physics 2020-09-04 Yuanyuan Wang , Fengping Li , Wei Wei , Baibiao Huang , Ying Dai

Two-dimensional materials with ferroelectric properties break the size effect of conventional ferroelectric materials and unlock unprecedented potentials of ferroelectric-related application at small length scales. In this work, using…

Materials Science · Physics 2022-03-25 Bo Xu , Junkai Deng , Xiangdong Ding , Jun Sun , Jefferson Zhe Liu

To have a fully ab initio description of the Moir\'e pattern in a transition metal dichalcogenide heterobilayer, we have carried out density functional theory calculations, taking accounts of both atomic registry in and the lattice…

Materials Science · Physics 2020-02-03 W. T. Geng , V. Wang , Y. C. Liu , T. Ohno , J. Nara

The recently experimentally synthesized monolayer $\mathrm{MoSi_2N_4}$ and $\mathrm{WSi_2N_4}$ (\textcolor[rgb]{0.00,0.00,1.00}{Science 369, 670-674 (2020})) lack inversion symmetry, which allows them to become piezoelectric. In this work,…

Materials Science · Physics 2020-12-29 San-Dong Guo , Yu-Tong Zhu , Wen-Qi Mu , Lei Wang , Xing-Qiu Chen

Recently, two-dimensional monolayer MoSi2N4 with hexagonal structure was successfully synthesized in experiment (Hong et al 2020 Science 369, 670). The fabricated monolayer MoSi2N4 is predicted to have excellent mechanical properties.…

Mesoscale and Nanoscale Physics · Physics 2021-04-14 Qingfang Li , Wanxin Zhou , Xiangang Wan , Jian Zhou

Van der Waals (vdW) coupling is emerging as a powerful method to engineer and tailor physical properties of atomically thin two-dimensional (2D) materials. In graphene/graphene and graphene/boron-nitride structures it leads to interesting…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Kaihui Liu , Liming Zhang , Ting Cao , Chenhao Jin , Diana Qiu , Qin Zhou , Alex Zettl , Peidong Yang , Steve G. Louie , Feng Wang

Little is known about the role of weak interlayer coupling in the second harmonic generation (SHG) effects of two-dimensional van der Waals (vdW) systems. In this article, taking homo-bilayer $MoS_2/MoS_2$ and hetero-bilayer $MoS_2/MoSe_2$…

Computational Physics · Physics 2022-02-02 Xiao Jiang , Lei Kang , Bing Huang

Semiconductor heterostructures provide a powerful platform for the engineering of excitons. Here we report the excitonic properties of two-dimensional (2D) heterostructures that consist of monolayer MoS2 and WS2 stacked epitaxially or…

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