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High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require…

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

High harmonic spectroscopy can access structural and dynamical information on molecular systems encoded in amplitude and phase of high harmonic generation (HHG) signals4. However, measurement of the harmonic phase is a daunting task. Here…

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

Chiral (highly helical) extreme ultraviolet (XUV) sources are pivotal for investigating chiroptical phenomena on the ultrafast electronic timescale. Table-top, coherent High Harmonic Generation (HHG)-based sources are particularly…

Optics · Physics 2025-03-07 Eran Ben Arosh , Eldar Ragonis , Lev Merensky , Avner Fleischer

The advancement of the ultrafast pulse shaping and waveform synthesis allowed to coherently control the atomic and electronic motions in matter. The temporal resolution of the waveform synthesis is inversely proportional to the broadening…

Optics · Physics 2024-06-04 Husain Alqattan , Dandan Hui , Vladimir Pervak , Mohammed Th. Hassan

Femtosecond extreme ultraviolet wave packet interferometry (XUV-WPI) was applied to study resonant inter-atomic Coulombic decay (ICD) in the HeNe dimer. The high demands on phase stability and sensitivity for vibronic XUV-WPI of…

Advances in attosecond core-level spectroscopies have successfully unlocked the fastest dynamics involving high-energy electrons. Yet, these techniques are not conventionally regarded as an appropriate probe for low-energy quasiparticle…

Continuous-wave coherent radiation in the vacuum ultraviolet (VUV)wavelength region at 121 nm will be essential for future laser-cooling of trapped antihydrogen [1]. Cold antihydrogen will enable both tests of the fundamental symmetry…

Optics · Physics 2012-08-20 Daniel Kolbe , Martin Scheid , Jochen Walz

High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

Irradiation of a medium by short intense pulses from x-ray / XUV free electron lasers can result in saturated photoionization of inner electronic shells. As a result an inversion of populations between core levels appears. The resulting…

Quantum Physics · Physics 2019-01-30 Andrei Benediktovitch , Vinay P. Majety , Nina Rohringer

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

Atomic Physics · Physics 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…

Atomic Physics · Physics 2022-04-15 L. Ortmann , C. Hofmann , I. A. Ivanov , A. S. Landsman

We show how bright, fully coherent, hard x-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By using longer-wavelength mid-infrared driving lasers of moderate peak intensity, full phase matching of the…

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

We report on the development of a high-order harmonic generation (HHG)-based ultrafast high-repetition-rate (250 kHz) monochromatic extreme ultraviolet (21.6 eV) source with polarization tunability, specifically designed for multi-modal…

Recently nonthermal radio transients from the quiet sun have been discovered and it has been hypothesised using rough calculations that they might be important for coronal heating. It is well realized that energy calculations using coherent…

Solar and Stellar Astrophysics · Physics 2021-09-08 Surajit Mondal
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