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The interaction of atomic orbitals at the interface of perovskite oxide heterostructures has been investigated for its profound impact on the band structures and electronic properties, giving rise to unique electronic states and a variety…

The discovery of ambient-pressure superconductivity with $T_{c,\text{onset}} > 40$ K in {\LNO} (LNO) thin films grown on the SrLaAlO$_4$ (SLAO) substrate with compressive ($\varepsilon\approx-2\%$) epitaxial strain provides a unique…

The discovery of nickelate superconductors has opened a new arena for studying the behavior of correlated electron liquids that give rise to unconventional superconductivity. While critical information about a material's charge dynamics is…

Understanding the interaction between plasmonic nanoparticles and transparent conductive oxides is instrumental to the development of next-generation photovoltaic, opto-electronic and energy-efficient solid-state lighting devices. We…

For La-doped BaSnO$_\text{3}$ thin films grown by pulsed laser deposition, we combine chemical surface characterization and electronic transport studies to probe the evolution of electronic states in the band structure for different…

The three-dimensional ternary LiFeO2 compound presents various unusual essential properties. The main features are thoroughly explored by the density functional and many-body perturbation theory. The concise physical/chemical picture, the…

Materials Science · Physics 2023-01-04 Vo Khuong Dien , Nguyen Thi Han , Wu-Pei Su , Ming-Fa Lin

Lanthanum manganite, LaMnO (LMO) is the parent compound for a class of hole doped(e.g. La1-xCaxMnO3, La1-xSrxMnO3) and electron doped (e.g. . La1-xCexMnO3, La1-xSnxMnO3) perovskite complex oxide materials. Strong correlation between the…

Materials Science · Physics 2017-06-01 Arun Singh Chouhan

The orbital excitations of a series of transition-metal compounds are studied by means of optical spectroscopy. Our aim was to identify signatures of collective orbital excitations by comparison with experimental and theoretical results for…

The near-field interaction due to a strong electromagnetic field induced by resonant localized plasmons can result in a strong coupling of excitonic states or formation of hybrid exciton-plasmon modes in quantum confined structures. This…

Mesoscale and Nanoscale Physics · Physics 2019-04-01 Yuba Poudel , Gary N. Lim , Mojtaba Moazzezi , Zachariah Hennighausen , Yuri Rostovtsev , Francis DSouza , Swastik Kar , Arup Neogi

Metallic systems with delocalized valence electrons host collective charge density oscillations known as plasmons. On the other hand, conventional insulators do not have free electrons and the low energy charge degrees of freedom are pinned…

Stimulated by experimental advances in electrolyte gating methods, we investigate theoretically percolation in thin films of inhomogenous complex oxides, such as La$_{1-x}$Sr$_{x}$CoO$_{3}$ (LSCO), induced by a combination of bulk chemical…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 Peter P. Orth , Rafael M. Fernandes , Jeff Walter , C. Leighton , B. I. Shklovskii

Metal nanoparticle (NP) surface coatings are known to significantly enhance the ultra-violet luminescence intensity of ZnO. Although there is general agreement that resonantly excited Localized Surface Plasmons (LSPs) in metal NPs can…

Electron correlations play a dominant role in the charge dynamics of the cuprates. We use resonant inelastic x-ray scattering (RIXS) to track the doping dependence of the collective charge excitations in electron doped…

We investigated theoretically the exciton-plasmon coupling effects on the population dynamics and the absorption properties of a hybrid nanosystem composed of a metal nanoparticle (MNP) and a V-type three level semiconductor quantum dot…

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to \emph{collective} magnetic excitations in $S=1$ systems by probing the Ni $L_3$-edge of La$_{2-x}$Sr$_x$NiO$_4$ ($x = 0, 0.33,…

We investigate high-energy spin excitations in hole-doped La$_{2-x}$Ca$_{x}$CuO$_{4-\delta}$ films across a broad Ca doping range $x = 0.05-0.50$ using resonant inelastic x-ray scattering (RIXS). Polarization analysis and incident-photon…

Ambient-pressure superconductivity in compressively strained bilayer nickelate films enables direct spectroscopic tests of pairing scenarios, yet how magnetism evolves with carrier doping remains largely unexplored. Here we use Ni…

We report the first single crystal growth of the correlated metal LaNiO3 using a high-pressure optical-image floating zone furnace. The crystals were studied using single crystal/powder x-ray diffraction, resistivity, specific heat, and…

Materials Science · Physics 2017-10-17 Junjie Zhang , Hong Zheng , Yang Ren , J. F. Mitchell

Oxygen packaging in transition metal oxides determines the metal-oxygen hybridization and electronic occupation at metal orbitals. Strontium vanadate (SrVO$_3$), having a single electron in a $3d$ orbital, is thought to be the simplest…

Li2GeO3, a ternary electrolyte compound of Li+-based battery, presents the unusual essential properties. The main features are thoroughly explored from the first-principles calculations. The concise pictures, the critical orbital…

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