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An 1d model with time-dependent random hopping is proposed to describe charge transport in DNA. It admits to investigate both diffusion of electrons and their tunneling between different sites in DNA. The tunneling appears to be strongly…

Soft Condensed Matter · Physics 2009-11-07 E. I. Kats , V. V. Lebedev

The spin-dependent propagation of electrons in helical nanowires is investigated. We show that the interplay of spin angular momentum and nanowire chirality, under spin-orbit interaction, lifts the symmetry between left and right…

Materials Science · Physics 2021-10-28 Diego A. Hoff , Luis G. C. Rego

A dynamical model is presented for chiral change in DNA molecules. The model is an extension of the conventional elastic model which incorporates the structure of base pairs and uses a spinor representation for the DNA configuration…

Biological Physics · Physics 2011-10-06 Teruaki Okushima , Hiroshi Kuratsuji

The chiral-induced spin selectivity (CISS) effect, a phenomenon where the chirality of molecules imparts significant spin selectivity to electron transfer processes, has garnered increasing interest among the chemistry, biology, and physics…

Chemical Physics · Physics 2025-09-05 Tian-Yi Zhang , Yue Mao , Ai-Min Guo , Qing-Feng Sun

In chemistry and biochemistry, chirality represents the structural asymmetry characterized by non-superimposable mirror images for a material like DNA. In physics, however, chirality commonly refers to the spin-momentum locking of a…

Materials Science · Physics 2024-08-07 Binghai Yan

The spin dynamics of electrons in chiral molecular systems remain a topic of intense interest, particularly regarding whether geometric chirality inherently induces spin polarization in current-carrying electrons. In this work, we employ ab…

Interatomic hopping mediated by spin-orbit coupling (SOC) entangles spin, orbital and sublattice degrees of freedom of electrons, leading to the emergence of intriguing phenomena such as novel topological insulators and exotic…

Materials Science · Physics 2024-07-16 Masaki Kato , Masao Ogata

The observation of spin-dependent transmission of electrons through chiral molecules has led to the discovery of chiral-induced spin selectivity (CISS). The remarkably high efficiency of the spin polarizing effect has recently gained…

Mesoscale and Nanoscale Physics · Physics 2024-03-01 Ashish Moharana , Yael Kapon , Fabian Kammerbauer , David Anthofer , Shira Yochelis , Mathias Kläui , Yossi Paltiel , Angela Wittmann

Highly spin selective transport of electrons through a helically shaped electrostatic potential is demonstrated in the frame of a minimal model approach. The effect is significant even in the case of weak spin-orbit coupling. Two main…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 R. Gutierrez , E. Diaz , R. Naaman , G. Cuniberti

Chirality-induced spin selectivity (CISS) was recently observed in photo-excited donor-chiral bridge-acceptor molecules, but a predictive theory able to explain available experiments is still lacking. Here we show that low-energy torsional…

Chirality-induced spin selectivity (CISS) refers to the fact that electrons get spin polarized after passing through organic chiral molecules in a nanoscale device. In CISS, chiral molecules are commonly believed to be a spin filter through…

Mesoscale and Nanoscale Physics · Physics 2022-12-06 Yotam Wolf , Yizhou Liu , Jiewen Xiao , Noejung Park , Binghai Yan

Recent observations of considerable spin polarization in photoemission from metal surfaces through monolayers of chiral molecules were followed by several efforts to rationalize the results as the effect of spin-orbit interaction that…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Joel Gersten , Kristen Kaasbjerg , Abraham Nitzan

In this paper we outline a physically motivated framework for describing spin-selective recombination processes in chiral systems, from which we derive spin-selective reaction operators for recombination reactions of donor-bridge-acceptor…

Chemical Physics · Physics 2023-03-09 Thomas P. Fay , David T. Limmer

We present a theoretical analysis of the environment effects on charge transport in double-stranded synthetic poly(G)-poly(C) DNA molecules attached to two ideal leads. Coupling of the DNA to the environment results in two effects: (i)…

Soft Condensed Matter · Physics 2009-07-13 A. V. Malyshev , E. Diaz , F. Dominguez-Adame , V. A. Malyshev

The observation of chiral-induced spin selectivity (CISS) in biological molecules still awaits a full theoretical explanation. In a recent Rapid Communication, Varela et al. [Phys. Rev. B 101, 241410(R) (2020)] presented a model for…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Ora Entin-Wohlman , Amnon Aharony , Yasuhiro Utsumi

We consider a polaron model where molecular \emph{rotations} are important. Here, the usual hopping between neighboring sites is affected directly by the electron-phonon interaction via a {\em twist-dependent} hopping amplitude. This model…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Wei Zhang , Alexander O. Govorov , Sergio E. Ulloa

A generation, propagation, and transfer of phonon angular momenta are examined on thermal transport in chiral insulative and diamagnetic crystals of $\alpha$-quartz. We found that thermally-driven phonons carry chirality-dependent angular…

Materials Science · Physics 2024-01-31 Kazuki Ohe , Hiroaki Shishido , Masaki Kato , Shoyo Utsumi , Hiroyasu Matsuura , Yoshihiko Togawa

We show how a spin polarization can be generated through the photo-induced electron transfer of an achiral donor-acceptor complex following chiral light excitation. In particular, we illustrate the basic energetic and symmetry requirements…

Chemical Physics · Physics 2026-03-10 Sindhana Pannir-Sivajothi , David T. Limmer

The role of chirality in determining the spin dynamics of photoinduced electron transfer in donor-acceptor molecules remains an open question. Although chirality-induced spin selectivity (CISS) has been demonstrated in molecules bound to…

In many organic molecules the strong coupling of excess charges to vibrational modes leads to the formation of polarons, i.e., a localized state of a charge carrier and a molecular deformation. Incoherent hopping of polarons along the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Benjamin B. Schmidt , Matthias H. Hettler , Gerd Schön