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Extraction of information in the form of oscillations from noisy data of natural phenomena such as sounds, earthquakes, ionospheric and brain activity, and various emissions from cosmic objects is extremely difficult. As a method for…

We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…

Two-dimensional infrared (2DIR) spectroscopy is widely used to study molecular dynamics but it is typically restricted to solid and liquid phase samples and modest spectral resolution. Only recently, its potential to study gas-phase…

Optics · Physics 2022-11-01 Grzegorz Kowzan , Thomas K. Allison

Accurate characterization using static light scattering (SLS) and dynamic light scattering (DLS) methods mandates the measurement and analysis of singly-scattered light. In turbid samples, the suppression of multiple scattering is therefore…

Soft Condensed Matter · Physics 2012-09-18 Ian Block , Frank Scheffold

The third-order response lies at the heart of simulating and interpreting nonlinear spectroscopies ranging from two dimensional infrared (2D-IR) to 2D electronic (2D-ES), and 2D sum frequency generation (2D-SFG). The extra time and…

Chemical Physics · Physics 2022-09-21 Kenneth A. Jung , Thomas E. Markland

Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…

Optics · Physics 2020-10-21 Bachana Lomsadze , Steven T. Cundiff

Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…

Quantum Physics · Physics 2021-03-31 André Anda , Jared H. Cole

Electronic energy transfer in photosynthesis occurs over a range of time scales and under a variety of intermolecular coupling conditions. Recent work has shown that electronic coupling between chromophores can lead to coherent oscillations…

We propose two dimensional x-ray coherent correlation spectroscopy (2DXCS) for the study of interactions between core-electron and valence transitions. This technique might find experimental applications in the future when very high…

Quantum Physics · Physics 2009-11-13 Igor V. Schweigert , Shaul Mukamel

Two-dimensional mass spectrometry (2D MS) is a method for tandem mass spectrometry that enables the correlation between precursor and fragment ions without the need for ion isolation. On a Fourier transform ion cyclotron resonance mass…

Diffuse correlation spectroscopy (DCS) is a powerful tool for assessing microvascular hemodynamic in deep tissues. Recent advances in sensors, lasers, and deep learning have further boosted the development of new DCS methods. However,…

Nuclear magnetic resonance spectroscopy (MRS) allows for the determination of atomic structures and concentrations of different chemicals in a biochemical sample of interest. MRS is used in vivo clinically to aid in the diagnosis of several…

Medical Physics · Physics 2021-05-04 Zohaib Iqbal , Dan Nguyen , M. Albert Thomas , Steve Jiang

We develop a technique to measure radial velocities of stars from spectra that present four sets of lines. The algorithm is an extension of the two-dimensional cross-correlation method TODCOR to four dimensions. It computes the correlation…

Astrophysics · Physics 2011-02-11 Guillermo Torres , David W. Latham , R. P. Stefanik

Laser dynamics underpin a broad range of modern photonic technologies and continue to reveal rich nonlinear behaviors. However, existing spectroscopic tools, most notably time-stretched dispersive Fourier transform spectroscopy (TS-DFT),…

To precisely measure and evaluate X-ray generation and evolution in a hohlraum during an implosion process, we present a two-dimensional (2D) time- and space-resolved diagnostic method by combining a compressed ultrafast photography (CUP)…

Instrumentation and Detectors · Physics 2021-10-13 Shijian Li , Qiangqiang Wang , Xuri Yao , Zhurong Cao , Jie Liu , Qing Zhao

Two dimensional spectroscopy is a powerful dynamical study method that has been developed in the last two decades. In 2D IR there are three experimental time periods during which the system vibrational modes of interest are excited, evolved…

Chemical Physics · Physics 2021-04-12 S. Tahereh Alavi

Two-dimensional (2D) vibrational spectroscopy is a powerful means of investigating the structure and dynamics of complex molecules in condensed phases. However, even in theory, analysis of 2D spectra resulting from complex inter- and…

Chemical Physics · Physics 2025-01-07 Ryotaro Hoshino , Yoshitaka Tanimura

The correlation holography reconstructs 3D objects as a distribution of two-point correlation of the random field detected by two dimensional detector arrays. Here, we describe a hybrid method, a combination of optical and computational…

Optics · Physics 2017-08-02 Rakesh Kumar Singh

Recently, a method of recording holograms of coherently illuminated three-dimensional scene without two-wave interference was demonstrated. The method is an extension of the coded aperture correlation holography from incoherent to coherent…

Optics · Physics 2023-07-19 Nathaniel Hai , Joseph Rosen

Femtosecond coherent multidimensional spectroscopy is demonstrated for an ultracold gas. For this, a setup for phase modulation spectroscopy is used to probe the $3^2\mathrm{S}_{1/2} - 2^2\mathrm{P}_{1/2, 3/2}$ transition in an 800…

Atomic Physics · Physics 2023-01-16 Friedemann Landmesser , Tobias Sixt , Katrin Dulitz , Lukas Bruder , Frank Stienkemeier
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