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The Free-Electron Laser (FEL) FLASH offers the worldwide still unique capability to study ultrafast processes with high-flux, high-repetition rate XUV and soft X-ray pulses. The vast majority of experiments at FLASH are of pump-probe type.…
Wide field-of-view imaging of fast processes in a microscope requires high light intensities motivating the use of lasers as light sources. However, due to their long spatial coherence length lasers are inappropriate for such applications…
We report on the possibility to obtain a high-quality inverted Doppler-free resonance in D1 line of alkali-metal atoms in the single-frequency regime. The counter-propagating optical fields with linear and mutually orthogonal polarizations…
Achieving efficient nonlinear optical frequency conversion in small volumes is key for future on-chip photonic devices that would provide a higher-speed alternative to modern electronics. However, the already intrinsically low conversion…
We have shown earlier that hyperfine spectroscopy in a vapor cell using co-propagating pump-probe beams has many advantages over the usual technique of saturated-absorption spectroscopy using counter-propagating beams. The main advantages…
Control over intensity, shape, direction, and phase of coherent light is essential in numerous fields, reaching from gravitational wave astronomy over quantum metrology and ultrafast sciences to semi-conductor fabrication. Modern laser…
Free-space optical (FSO) communications has the potential to revolutionize wireless communications due to its advantages of inherent security, high-directionality, high available bandwidth and small physical footprint. The effects of…
We present a method for measuring the magnetic field that allows hyperfine and Zeeman optical pumping, excitation and detection of magnetic resonance by means of a single laser beam with time-modulated ellipticity. This improvement allows…
We present design and realization of an ultra-broadband optical spectrometer capable of measuring the spectral intensity of multi-octave-spanning light sources on a single-pulse basis with a dynamic range of up to 8 orders of magnitude. The…
Linear (spectro) polarimetry is usually performed using separate photon flux measurements after spatial or temporal polarization modulation. Such classical polarimeters are limited in sensitivity and accuracy by systematic effects and…
Recording of transient absorption microscopy images requires fast detection of minute optical density changes, which is typically achieved with high-repetition-rate laser sources and lock-in detection. Here, we present a highly flexible and…
We present an approach to spectropolarimetry which requires neither moving parts nor time dependent modulation, and which offers the prospect of achieving high sensitivity. The technique applies equally well, in principle, in the optical,…
Frequency comb-referenced measurements of sub-Doppler laser saturation dip absorption lines in the $v_1+v_3$ band of acetylene near $1.5\,\mu \mathrm{m}$ are reported. These measurements include transitions involving higher rotational…
We introduce an approach for performing spectrally resolved electron microscopy without the need for an electron spectrometer. The method involves an electron beam prepared as a coherent superposition of multiple paths, one of which passes…
We demonstrate an approach to two-dimensional electronic spectroscopy (2DES) that combines the benefits of shot-to-shot detection at high-repetition rates with the simplicity of a broadband white light continuum input and conventional…
We study modulation-free methods for producing sub-Doppler, dispersive line shapes for laser stabilization near the potassium D2 transitions at 767 nm. Polarization spectroscopy is performed and a comparison is made between the use of a…
We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or…
Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…
Using a novel approach to ultrafast resonant pump-probe spectroscopy we investigate the spectral shape and dynamics of absorption features related to the A exciton in an hBN/MoSe$_2$/hBN van der Waals heterostructure. While in a pure…
We present a setup to perform sub shot noise measurements of the phase quadrature for intense pulsed light without the use of a separate local oscillator. A Mach--Zehnder interferometer with an unbalanced arm length is used to detect the…