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Using diffusion Monte Carlo (DMC) and density functional theory (DFT) calculations, we examined the structural stability and interlayer binding properties of PtSe$_2$, a representative transition metal dichalcogenide (TMD) with strong…

We present a multi-scale density functional theory (DFT) informed molecular dynamics and tight-binding (TB) approach to capture the interdependent atomic and electronic structures of twisted bilayer graphene. We calibrate the flat band…

Mesoscale and Nanoscale Physics · Physics 2022-03-17 Nicolas Leconte , Srivani Javvaji , Jiaqi An , Appalakondaiah Samudrala , Jeil Jung

Twisted double bilayer graphene has recently emerged as an interesting moir\'e material that exhibits strong correlation phenomena that are tunable by an applied electric field. Here we study the atomic and electronic properties of three…

We apply a multiscale modeling approach to study lattice reconstruction in marginally twisted bilayers of transition metal dichalcogenides (TMD). For this, we develop DFT-parametrized interpolation formulae for interlayer adhesion energies…

Mesoscale and Nanoscale Physics · Physics 2020-05-21 V. V. Enaldiev , V. Zólyomi , C. Yelgel , S. J. Magorrian , V. I. Fal'ko

The creation of moir\'e superlattices in twisted bilayers of two-dimensional crystals has been utilised to engineer quantum material properties in graphene and transition metal dichalcogenide (TMD) semiconductors. Here, we examine the…

Mesoscale and Nanoscale Physics · Physics 2024-05-27 J. G. McHugh , V. V. Enaldiev , V. I. Fal'ko

$\alpha$-graphyne is a two-dimensional sheet of $sp$-$sp^2$ hybridized carbon atoms in a honeycomb lattice. While the geometrical structure is similar to that of graphene, the hybridized triple bonds give rise to electronic structure that…

Materials Science · Physics 2017-08-04 Hyeondeok Shin , Jeongnim Kim , Hoonkyung Lee , Olle Heinonen , Anouar Benali , Yongkyung Kwon

We study electronic, charge, and magnetic properties of twisted bilayer graphene with fillings $2\leq n\leq 6$ per moire unit cell within the recently introduced formulation of extended dynamical mean-field theory (E-DMFT) for…

Strongly Correlated Electrons · Physics 2022-09-30 A. A. Katanin

Layered two-dimensional (2D) materials exhibit unique properties, expanding opportunities in material design. We investigate MX$_2$ transition metal dichalcogenides (TMDCs) (M = Mo, W; X = S, Se, Te) in homo- and heterobilayers with…

Materials Science · Physics 2025-03-13 Yu-Hsiu Lin , William P. Comaskey , Jose L. Mendoza-Cortes

The structural and vibrational properties of metal-organic interfaces have been examined by means of infrared (IR) absorption spectroscopy and density functional theory (DFT) with an approach accounting for long-range dispersive…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 N. L. Zaitsev , P. Jakob , R. Tonner

We employ ab-initio electronic structure calculations to investigate the charge-density waves and periodic lattice distortions in bilayer 2H-NbSe$_2$. We demonstrate that the vertical stacking can give rise to a variety of patterns that may…

Strongly Correlated Electrons · Physics 2024-11-08 Fabrizio Cossu , Dhani Nafday , Krisztian Palotás , Mehdi Biderang , Heung-Sik Kim , Alireza Akbari , Igor Di Marco

We investigate the electronic density redistribution of rotated bilayer graphene under a perpendicular electric field, showing that the layers are actually coupled even for large angles. This layer-layer coupling is evidenced by the charge…

Mesoscale and Nanoscale Physics · Physics 2012-03-26 E. Suárez Morell , P. Vargas , L. Chico , L. Brey

AA-stacked bilayer graphene supports Fermi circles in its bonding and antibonding bands which coincide exactly, leading to symmetry-breaking in the presence of electron-electron interactions. We analyze a continuum model of this system in…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 L. Brey , H. A. Fertig

Small-twist-angle bilayer graphene supports strongly correlated insulating states and superconductivity. Twisted few-layer graphene systems are likely to open up new directions for strong correlation physics in moir\'e superlattices. We…

Materials Science · Physics 2019-07-30 Xiao Li , Fengcheng Wu , Allan H. MacDonald

Twisted bilayer systems host a wealth of emergent phenomena, such as flat-band superconductivity, ferromagnetism, and ferroelectricity, arising from moir\'e superlattices and unconventional interlayer coupling. Despite their central role,…

Mesoscale and Nanoscale Physics · Physics 2026-01-21 A. Nakamura , Y. Chiashi , T. Shimojima , Y. Tanaka , S. Akatsuka , M. Sakano , S. Masubuchi , T. Machida , K. Watanabe , T. Taniguchi , K. Ishizaka

Stacking order has strong influence on the coupling between the two layers of twisted bilayer graphene (BLG), which in turn determines its physical properties. Here, we report the investigation of the interlayer coupling of the epitaxially…

Mesoscale and Nanoscale Physics · Physics 2020-01-28 Bing Deng , Binbin Wang , Ning Li , Rongtan Li , Yani Wang , Jilin Tang , Qiang Fu , Zhen Tian , Peng Gao , Jiamin Xue , Hailin Peng

In bilayers of two-dimensional (2D) semiconductors with stacking arrangements which lack inversion symmetry charge transfer between the layers due to layer-asymmetric interband hybridisation can generate a potential difference between the…

Mesoscale and Nanoscale Physics · Physics 2021-07-01 F. Ferreira , V. V. Enaldiev , V. I. Fal'ko , S. J. Magorrian

In this study, we use first-principles calculations to investigate the stacking-dependent electronic properties of GaSe/GaTe van der Waals heterobilayers. By analyzing five representative stacking configurations--AA, AA$'$, A$'$C, A$'$B,…

Materials Science · Physics 2025-06-24 Hsin-Yi Liu , Jhao-Ying Wu

We have explored the electronic properties of stacked graphene flakes with the help of the quantum chemistry methods. We found that the behavior of a bilayer system is governed by the strength of the repulsive interactions that arise…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Julia Berashevich , Tapash Chakraborty

The incommensurate 30$^{\circ}$ twisted bilayer graphene (BG) possesses both relativistic Dirac fermions and quasiperiodicity with 12-fold rotational symmetry arising from the interlayer interaction…

Mesoscale and Nanoscale Physics · Physics 2022-03-14 Guodong Yu , Yunhua Wang , Mikhail I. Katsnelson , Hai-Qing Lin , Shengjun Yuan

We investigate magnetism and band structure engineering in Moir\'e superlattice of blue phosphorus ($\beta$-P) and grey arsenene ($\beta$-As) bilayers, using \textit{ab initio} calculations. The electronic states near the valence and…

Materials Science · Physics 2019-05-20 Shantanu Agnihotri , Maneesh Kumar , Yogesh Singh Chauhan , Amit Agarwal , Somnath Bhowmick
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