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The transient-absorption spectrum of a $V$-type three-level system is investigated, when this is periodically excited by a train of equally spaced, $\delta$-like pump pulses as, e.g., from an optical-frequency-comb laser. We show that, even…

Atomic Physics · Physics 2019-01-30 Juliane Haug , Stefano M. Cavaletto

The last decade has witnessed a rapid advancement in laser technology, enabling the direct monitoring and control of electronic motion on its natural attosecond to sub-femtosecond timescales. Ultrafast processes are conventionally studied…

Chemical Physics · Physics 2026-05-27 Torsha Moitra

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

Atomic Physics · Physics 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

Recent advances in laser technology allow us to follow electronic motion at its natural time-scale with ultra-fast time resolution, leading the way towards attosecond physics experiments of extreme precision. In this work, we assess the use…

Other Condensed Matter · Physics 2016-06-22 Jessica Walkenhorst , Umberto De Giovannini , Alberto Castro , Angel Rubio

We present a spin-adapted time-dependent coupled cluster singles and doubles model for the molecular response to a sequence of ultrashort laser pulses. The implementation is used to calculate the electronic response to a valence-exciting…

Chemical Physics · Physics 2020-08-28 Andreas S. Skeidsvoll , Alice Balbi , Henrik Koch

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Fluctuation dissipation theorems connect the linear response of a physical system to a perturbation to the steady-state correlation functions. Until now, most of these theorems have been derived for finite-dimensional systems. However, many…

Statistical Mechanics · Physics 2019-08-22 Mohammad Mehboudi , Juan. M. R. Parrondo , Antonio Acin

The physical interpretation of time-resolved photoabsorption experiments is not as straightforward as for the more conventional photoabsorption experiments conducted on equilibrium systems. In fact, the relation between the transient…

Atomic Physics · Physics 2015-06-24 E. Perfetto , G. Stefanucci

This work models the propagation of an optical pulse in a 4-level atomic system in the electromagnetic induced transparency regime. By demonstrating that linear and nonlinear optical properties can be externally controlled and tailored by a…

Optics · Physics 2018-10-11 Nuno A. Silva , André L. Almeida , A. Guerreiro

A numerical method to calculate optical conductivity based on a pump-probe setup is presented. Its validity and limits are tested and demonstrated via the concrete numerical simulations on the half-filled one-dimensional extended Hubbard…

Strongly Correlated Electrons · Physics 2016-05-26 Can Shao , Takami Tohyama , Hong-Gang Luo , Hantao Lu

We analyze the optical pump-probe reflection and transmission coefficients when the photoinduced response depends nonlinearly on the incident pump intensity. Under these conditions, we expect the photoconductivity depth profile to change…

Strongly Correlated Electrons · Physics 2024-10-30 Leya Lopez , Derek G. Sahota , J. Steven Dodge

In this article, we study the effects of intrinsic nonlinear optomechanical interaction on the linear response of a driven-dissipative optomechanical system to a weak time-dependent perturbation. By calculating the linear response of the…

Quantum Physics · Physics 2025-02-17 B. Askari , A. Dalafi , M. J. Kazemi

We propose a new method of calculating nonlinear optical responses of interacting electronic systems. In this method, the total Hamiltonian (system + system-pump interaction) is transformed into a different form that (apparently) does not…

Materials Science · Physics 2009-10-31 Jun-ichi Inoue , Akira Shimizu

We present an effective linear response approach to pump-probe femtosecond coherence spectroscopy in the well separated pulse limit. The treatment presented here is based on a displaced and squeezed state representation for the…

Chemical Physics · Physics 2009-11-06 Anand T. N. Kumar , Florin Rosca , Allan Widom , Paul M. Champion

We introduce a numerically exact and computationally feasible nonlinear-response theory developed for lossy superconducting quantum circuits based on a framework of quantum dissipation in a minimally extended state space. Starting from the…

Quantum Physics · Physics 2025-03-27 V. Vadimov , M. Xu , J. T. Stockburger , J. Ankerhold , M. Möttönen

The sensitivity of the displacement transducer pumped with a train of high-intensity laser pulses is estimated. Due to the multicomponent character of the pump a consideration of transformations of the signal and the noises between optical…

Optics · Physics 2007-05-23 Victor V. Kulagin

Based on the work done by an electromagnetic field on an atomic or molecular electronic system, a general gauge invariant formulation of transient absorption spectroscopy is presented within the semi-classical approximation. Avoiding…

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

We develop a linear response theory to provide a unified description of two recent spectroscopy protocols for probing one-dimensional supersolid states realized in cold-atom systems. Both protocols involve applying a periodic optical…

Quantum Gases · Physics 2025-05-09 L. M. Platt , D. Baillie , P. B. Blakie

We study the optical response of a binary system of identical atoms in which one of them is excited by an incoherent pump. %We study the properties of photon scattering, absorption and emission, together with the time evolution of the…

Quantum Physics · Physics 2025-06-27 L. Acevedo , J. Sánchez-Cánovas , M. Donaire
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