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Related papers: Hyperpolarisation Dynamics: Asymptotic Polarisatio…

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We reveal an interplay between temperature and radical concentration necessary to establish thermal mixing (TM) as an efficient dynamic nuclear polarization (DNP) mechanism. We conducted DNP experiments by hyperpolarizing widely used DNP…

Quantum Physics · Physics 2024-04-12 Ludovica M. Epasto , Thibaud Maimbourg , Alberto Rosso , Dennis Kurzbach

Dynamic nuclear polarization (DNP) is an NMR sensitivity enhancement technique that mediates polarization transfer from unpaired electrons to NMR-active nuclei. Despite its success in elucidating important structural information on…

Spin-blockaded quantum dots provide a unique setting for studying nuclear-spin dynamics in a nanoscale system. Despite recent experimental progress, observing phase-sensitive phenomena in nuclear spin dynamics remains challenging. Here we…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 M. S. Rudner , I. Neder , L. S. Levitov , B. I. Halperin

We introduce a method for non-destructive quantification of nuclear spin polarization, of relevance to hyperpolarized spin tracers widely used in magnetic resonance from spectroscopy to in vivo imaging. In a bias field of around 30 nT we…

In solid_state hybrid electron_nuclear spin systems quantum entanglement plays vital role in allowing accessible transfer of information between subatomic particles, regardless of the host lattice coordination spatial geometry, revealing…

Quantum Physics · Physics 2013-11-25 Vesna Berec , J. S. Braunstein

The model considered in the paper is used nowadays to describe spin dynamics of quantum dots after optical excitation. Based on the exact diagonalization of a model Hamiltonian, we solve the problems of the electron spin polarization decay…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 G. G. Kozlov

Taking inspiration from NMR spectroscopy, periodic irradiation schemes have recently shown remarkable performance when implemented into pulsed dynamic nuclear polarization (DNP) sequences. This has prompted considerable interest in…

The ability to control and exploit quantum coherence and entanglement drives research across many fields ranging from ultra-cold quantum gases to spin systems in condensed matter. Transcending different physical systems, optical approaches…

Mesoscale and Nanoscale Physics · Physics 2014-08-26 K. Müller , T. Kaldewey , R. Ripszam , J. S. Wildmann , A. Bechtold , M. Bichler , G. Koblmüller , G. Abstreiter , J. J. Finley

Spatially nonhomogeneously spin polarized nuclei are proposed as a new mechanism to monitor electron states in a nanostructure, or as a means to createn and, if necessary, reshape such nanostructures in the course of the experiment. We…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 V. Fleurov , V. A. Ivanov , F. M. Peeters , I. D. Vagner

The active driving of the electron spin of a color center is known as a method for the hyperpolarization of the surrounding nuclear spin bath and to initialize a system with large number of spins. Here, we investigate the efficiency of this…

Quantum Physics · Physics 2023-08-15 F. T. Tabesh , M. Fani , J. S. Pedernales , M. B. Plenio , M. Abdi

In nuclear-spin-polarization-induced quantum dots the electrons are confined through local nuclear spin polarization. The model electron confinement potential is time-dependent due to the nuclear spin diffusion and relaxation processes. It…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 B. F. Samsonov , Yu. V. Pershin

A scheme for decoupling and selectively recoupling large networks of dipolar-coupled spins is proposed. The scheme relies on a combination of broadband, decoupling pulse sequences applied to all the nuclear spins with a band-selective pulse…

Quantum Physics · Physics 2007-05-23 Fumiko Yamaguchi , Thaddeus D. Ladd , Cyrus P. Master , Yoshihisa Yamamoto , Navin Khaneja

Precise knowledge of a quantum system's Hamiltonian is a critical pre-requisite for its use in many quantum information technologies. Here, we report a method for the precise characterization of the non-secular part of the excited-state…

Quantum Physics · Physics 2017-06-20 F. Poggiali , P. Cappellaro , N. Fabbri

We theoretically study the interplay of spin-orbit and hyperfine interactions in dynamical nuclear polarization in two-electron semiconductor double quantum dots near the singlet $(S)$ - triplet $(T_+)$ anticrossing. The goal of the scheme…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Marko J. Rančić , Guido Burkard

Hyperfine interactions between electron and nuclear spins in the quantum Hall regime provide powerful means for manipulation and detection of nuclear spins. In this work we demonstrate that significant changes in nuclear spin polarization…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Y. Q. Li , V. Umansky , K. von Klitzing , J. H. Smet

Algorithmic Cooling (AC) of spins applies entropy manipulation algorithms in open spin-systems in order to cool spins far beyond Shannon's entropy bound. AC of nuclear spins was demonstrated experimentally, and may contribute to nuclear…

Quantum Physics · Physics 2011-11-01 Yuval Elias , Tal Mor , Yossi Weinstein

Dynamic Nuclear Polarization (DNP) has revolutionized the field of solid-state NMR spectroscopy by significantly enhancing the sensitivity of nuclear magnetic resonance experiments. Conventionally, cross effect DNP relies on biradicals to…

Chemical Physics · Physics 2023-09-28 Amaria Javed , Asif Equbal

We describe a method for precise estimation of the polarization of a mesoscopic spin ensemble by using its coupling to a single two-level system. Our approach requires a minimal number of measurements on the two-level system for a given…

Quantum Physics · Physics 2009-11-11 G. Giedke , J. M. Taylor , D. D'Alessandro , M. D. Lukin , A. Imamoglu

In this work we present a new formalism to evaluate the nuclear spin dynamics driven by hyperfine interaction with non-equilibrium electron spins. To describe the dynamics up to second order in the hyperfine coupling, it suffices to…

Mesoscale and Nanoscale Physics · Physics 2011-07-12 J. Danon , Yu. V. Nazarov

We report on the dynamic nuclear polarization of a single charge-tunable self-assembled InAs/GaAs quantum dot in a longitudinal magnetic field of $\sim$0.2T. The hyperfine interaction between the optically oriented electron and nuclei spins…