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Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

Quantum Physics · Physics 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating non-thermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance…

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

We propose a new method for dynamic nuclear polarisation in a quasi one-dimensional quantum wire utilising the spin-orbit interaction, the hyperfine interaction, and a finite source-drain potential difference. In contrast with current…

Mesoscale and Nanoscale Physics · Physics 2008-03-05 V. Tripathi , A. C. H. Cheung , N. R. Cooper

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing

Dynamic nuclear spin polarization (DNP) mediated by paramagnetic point defects in semiconductors is a key resource for both initializing nuclear quantum memories and producing nuclear hyperpolarization. DNP is therefore an important process…

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

Nuclear spin hyperpolarization techniques, such as dynamic nuclear polarization (DNP) and parahydrogen-induced polarization (PHIP), have revolutionized nuclear magnetic resonance and magnetic resonance imaging. In these methods, a readily…

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

We discuss the polarization dynamics during solid effect dynamic nuclear polarization (DNP) in a central spin model that consists of an electron surrounded by many nuclei. To this end we use a recently developed formalism and validate first…

Other Condensed Matter · Physics 2016-03-23 Daniel Wiśniewski , Alexander Karabanov , Igor Lesanovsky , Walter Köckenberger

Nuclear spin polarization can be pumped into spin-blocked quantum dots by multiple Landau- Zener passages through singlet-triplet anticrossings. By numerical simulations of realistic systems including approximately $10^7$ nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Arne Brataas , Emmanuel I. Rashba

Initializing a set of qubits to a given quantum state is a basic prerequisite for the physical implementation of quantum-information protocols. Here, we discuss the polarization of the electronic and nuclear spin in a single nitrogen…

Quantum Physics · Physics 2017-07-26 Tanmoy Chakraborty , Jingfu Zhang , Dieter Suter

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

Photochemically induced dynamic nuclear polarization (photo-CIDNP) is a method to hyperpolarize nuclear spins using light. In most cases, CIDNP experiments are performed at a high magnetic field and the sample is irradiated by the light…

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

We report a versatile method to efficiently polarize single nuclear spins in diamond, which is based on optical pumping of a single NV color center and mediated by a level-anti crossing in its excited state. A nuclear spin polarization…

A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic…

Mesoscale and Nanoscale Physics · Physics 2010-09-30 F. Klotz , V. Jovanov , J. Kierig , E. C. Clark , M. Bichler , G. Abstreiter , M. S. Brandt , J. J. Finley , H. Schwager , G. Giedke