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Direct dynamic nuclear polarization of 1H nuclei in frozen water and water-ethanol mixtures is demonstrated using silicon nanoparticles as the polarizing agent. Electron spins at dangling-bond sites near the silicon surface are identified…

Mesoscale and Nanoscale Physics · Physics 2014-01-14 M. C. Cassidy , C. Ramanathan , D. G. Cory , J. W. Ager , C. M. Marcus

We demonstrate optically pumped dynamic nuclear polarization of 29-Si nuclear spins that are strongly coupled to paramagnetic color centers in 4H- and 6H-SiC. The 99 +/- 1% degree of polarization at room temperature corresponds to an…

We show theoretically that ultracold hydrogen atoms have very favorable properties for sympathetic cooling of molecules to microkelvin temperatures. We calculate the potential energy surfaces for spin-polarized interactions of H atoms with…

Atomic Physics · Physics 2013-11-20 Maykel L. Gonzalez-Martinez , Jeremy M. Hutson

We propose to use a new platform - ultracold polar molecules - for quantum computing with switchable interactions. The on/off switch is accomplished by selective excitation of one of the "0" or "1" qubits - long-lived molecular states - to…

Quantum Physics · Physics 2009-11-13 S. F. Yelin , K. Kirby , R. Cote

We show that ionization of noble gas atoms by strong infrared circularly polarized laser field under standard exerimental conditions can yield electrons with up to 100% spin polarization in energy resolved measurements. Spin polarization…

Atomic Physics · Physics 2013-07-18 Ingo Barth , Olga Smirnova

Polarized atomic ensembles play a crucial role in precision measurements. We demonstrate a novel method of creating atomic polarization in an alkali vapor in a continuous-wave regime. The method relies on a combination of optical pumping by…

Atomic Physics · Physics 2021-10-22 A. Tretiakov , C. A. Potts , Y. Y. Lu , J. P. Davis , L. J. LeBlanc

Spatially nonhomogeneously spin polarized nuclei are proposed as a new mechanism to monitor electron states in a nanostructure, or as a means to createn and, if necessary, reshape such nanostructures in the course of the experiment. We…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 V. Fleurov , V. A. Ivanov , F. M. Peeters , I. D. Vagner

While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…

Atomic Physics · Physics 2013-02-27 Felipe Herrera , Sabre Kais , K. Birgitta Whaley

It should be possible to generate multi-ampere spin-polarized beams of hydrogen isotopes by repeated charge-transfer collisions in highly spin-polarized Cs vapor. Estimates suggest that off-resonant Raman pumping with kW scale narrowband…

Atomic Physics · Physics 2026-05-19 Thad G. Walker , Cary B. Forest , Deniz D. Yavuz

In a dynamic nuclear polarization experiment on a 40 mM solution of 4-amino-TEMPO in a 40:60 water/glycerol mixture, we have observed that the bulk dipolar reservoir is cooled to a spin temperature of 15.5 micro-K, following microwave…

Other Condensed Matter · Physics 2009-04-01 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Ultracold polar molecules are an ideal platform for studying many-body physics with long-range dipolar interactions. Experiments in this field have progressed enormously, and several groups are pursuing advanced apparatus for manipulation…

Atomic Physics · Physics 2018-04-27 Jacob P. Covey , Luigi De Marco , Oscar L. Acevedo , Ana Maria Rey , Jun Ye

Recent experiments have demonstrated the efficacy of chiral helically shaped molecules in polarizing the scattered electron spin, an effect termed as chiral-induced spin selectivity (CISS). Here we solve a simple tight-binding model for…

Mesoscale and Nanoscale Physics · Physics 2016-02-03 Shlomi Matityahu , Yasuhiro Utsumi , Amnon Aharony , Ora Entin-Wohlman , Carlos A. Balseiro

We show that a large class of helium-containing cold polar molecules form readily in a cryogenic buffer gas, achieving densities as high as 10^12 cm^-3. We explore the spin relaxation of these molecules in buffer gas loaded magnetic traps,…

Atomic Physics · Physics 2011-04-29 N. Brahms , T. V. Tscherbul , P. Zhang , J. K los , H. R. Sadeghpour , A. Dalgarno , J. M. Doyle , T. G. Walker

We report on further investigation of nuclear hyperpolarization of helium-3 in magnetized plasma at a magnetic field of 3.66 T and at different experimental conditions in a dual cell of relatively large volume, compared to those reported in…

Atomic Physics · Physics 2022-08-16 Alexander Makarchenko , Vyacheslav Kuzmin , Kajum Safiullin , Murat Tagirov

We analyze cavity-assisted cooling schemes for polar molecules in the microwave domain, where molecules are excited on a rotational transition and energy is dissipated via strong interactions with a lossy stripline cavity, as recently…

Quantum Physics · Physics 2009-12-21 Margareta Wallquist , Peter Rabl , Mikhail D. Lukin , Peter Zoller

Nuclear spin polarization can be pumped into spin-blocked quantum dots by multiple Landau- Zener passages through singlet-triplet anticrossings. By numerical simulations of realistic systems including approximately $10^7$ nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Arne Brataas , Emmanuel I. Rashba

We propose a new mechanism of generating spin polarization in heavy-ion collisions dominated by nucleon degree of freedom. By incorporating the spin change in nucleon-nucleon scatterings based on the phase shift data together with the…

Nuclear Theory · Physics 2025-07-08 Rong-Jun Liu , Jun Xu , Yu-Gang Ma

We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external…

Atomic Physics · Physics 2013-08-01 I. Manai , R. Horchani , M. Hamamda , A. Fioretti , M. Allegrini , H. Lignier , P. Pillet , D. Comparat

We show how to use polar molecules in an optical lattice to engineer quantum spin models with arbitrary spin S >= 1/2 and with interactions featuring a direction-dependent spin anisotropy. This is achieved by encoding the effective spin…

Stimulated wave of polarization, triggered by a flip of a single spin, presents a simple model of quantum amplification. Previously, it has been found that such wave can be excited in a 1D Ising chain with nearest-neighbor interactions,…

Quantum Physics · Physics 2009-11-13 G. B. Furman , S. D. Goren , J. -S. Lee , A. K. Khitrin , V. M. Meerovich , V. L. Sokolovsky