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A variational approach, based on a discrete representation of the chain, is used to calculate free energy and conformational properties in polyelectrolytes. The true bond and Coulomb potentials are approximated by a trial isotropic harmonic…

chem-ph · Physics 2016-08-15 B. Jönsson , C. Peterson , B. Söderberg

We show that a difference in time scales of vertical and lateral dynamics permits one to analyze the problem of interacting electrons confined in an axially symmetric three-dimensional potential with a lateral oscillator confinement by…

Mesoscale and Nanoscale Physics · Physics 2008-09-26 N. S. Simonovic , R. G. Nazmitdinov

We build a double quantum-dot system with Coulomb coupling and aim at studying the connections among the entropy production, free energy, and information flow. By utilizing the concepts in stochastic thermodynamics and graph theory…

Statistical Mechanics · Physics 2021-09-01 Zhiyuan Lin , Tong Fu , Juying Xiao , Shanhe Su , Jincan Chen , Yanchao Zhang

We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we…

Quantum Physics · Physics 2015-10-02 M. Guggemos , D. Heinrich , O. A. Herrera-Sancho , R. Blatt , C. F. Roos

The hydrogen atom with the Coulomb interaction is one of the exactly solvable non-relativistic quantum models. Unlike many other exactly solvable models it describes a real physical object providing the formulas for energy levels and…

Quantum Physics · Physics 2013-08-02 Ruslan Sharipov

Conditions at which a quasi-one-dimensional (1D) electron system can be considered as a quantum liquid of impenetrable charged particles are theoretically analyzed. In the presence of an inert, neutralizing background, a motion of…

Superconductivity · Physics 2024-06-21 Yu. P. Monarkha

The screened Coulomb interaction between a pair of infinite parallel planes with spatially varying surface charge is considered in the limit of small electrical potentials for arbitrary Debye lengths. A simple expression for the disjoining…

Classical Physics · Physics 2017-04-12 Sandip Ghosal , John D. Sherwood

Understanding ion adsorption at electrified metal-electrolyte interfaces is essential for accurate modeling of electrochemical systems. Here, we systematically investigate the free energy profiles of Na$^+$, Cl$^-$, and F$^-$ ions at the…

Chemical Physics · Physics 2026-02-27 Fabrice Roncoroni , Abrar Faiyad , Yichen Li , Tao Ye , Ashlie Martini , David Prendergast

Recent studies on the solvation of atomistic and nanoscale solutes indicate that a strong coupling exists between the hydrophobic, dispersion, and electrostatic contributions to the solvation free energy, a facet not considered in current…

Statistical Mechanics · Physics 2009-11-11 J. Dzubiella , J. M. J. Swanson , J. A. McCammon

By splitting the Coulomb interaction into long-range and short-range components, we decompose the energy of a quantum electronic system into long-range and short-range contributions. We show that the long-range part of the energy can be…

Chemical Physics · Physics 2009-11-10 Julien Toulouse , Francois Colonna , Andreas Savin

Studies of the thermodynamics of complex coacervation of pairs of symmetric, strongly ionizable, oppositely charged polyelectrolyte chains are abundant. To generalize such understanding to asymmetric chain lengths and variable ionizability…

Soft Condensed Matter · Physics 2023-06-07 Souradeep Ghosh , Soumik Mitra , Arindam Kundagrami

A model for ionic solutions with an attractive short-range pair interaction between the ions is presented. The short-range interaction is accounted for by adding a quadratic non-local term to the Poisson-Boltzmann free energy. The model is…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

Can we avoid molecular dynamics simulations to estimate the electrostatic interaction between charged objects separated by a nanometric distance in water? To answer this question, we develop a continuous model for the dielectric properties…

Soft Condensed Matter · Physics 2020-05-05 M. Vatin , A. Porro , N. Sator , J-F. Dufrêche , H. Berthoumieux

Binary collisions between ions and electrons in an external magnetic field are considered in second-order perturbation theory, starting from the unperturbed helical motion of the electrons. The calculations are done with the help of an…

Plasma Physics · Physics 2007-05-23 Hrachya B. Nersisyan

Earlier, using phenomenological approach, we showed that in some cases polarizable models of condensed phase systems can be reduced to nonpolarizable equivalent models with scaled charges. Examples of such systems include ionic liquids,…

Chemical Physics · Physics 2015-04-30 Igor Leontyev , Alexei Stuchebrukhov

We propose a mean-field analytical model to account for the observed asymmetry in the ability to form long-range attraction by the negatively charged colloidal particles and not their equivalently charged positive counterpart. We conjecture…

Soft Condensed Matter · Physics 2009-11-13 William Kung , Monica Olvera de la Cruz

Thermodynamic quantities of Coulomb plasmas consisting of point-like ions immersed in a compressible, polarizable electron background are calculated for ion charges Z=1 to 26 and for a wide domain of plasma parameters ranging from the…

Plasma Physics · Physics 2016-09-08 G. Chabrier , A. Y. Potekhin

Counterion distribution around an isolated flexible polyelectrolyte in the presence of a divalent salt is evaluated using the adsorption model [M. Muthukumar, J. Chem. Phys. {\bf 120}, 9343 (2004)] that considers Bjerrum length, salt…

Soft Condensed Matter · Physics 2008-12-29 Arindam Kundagrami , M. Muthukumar

Polarizable particle systems, including charged colloids, polarizable ions, biomolecular assemblies, and soft nanomaterials, can exhibit contact electrostatic interactions that depart strongly from Coulomb behavior when dielectric mismatch…

Soft Condensed Matter · Physics 2026-05-13 Yanyu Duan , Zecheng Gan

We present a simple, unified theory for the self-energy of an ion near a dielectric interface. Our theory accounts for both the short-range (solvation) and long-range (image force) electrostatic forces, charge polarization induced by these…

Soft Condensed Matter · Physics 2015-06-17 Rui Wang , Zhen-Gang Wang
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