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This paper presents a new Bayesian model and associated algorithm for depth and intensity profiling using full waveforms from time-correlated single-photon counting (TCSPC) measurements in the limit of very low photon counts (i.e.,…

Instrumentation and Detectors · Physics 2016-10-14 Yoann Altmann , Ximing Ren , Aongus McCarthy , Gerald S. Buller , Steve McLaughlin

We introduce a local machine-learning method for predicting the electron densities of periodic systems. The framework is based on a numerical, atom-centred auxiliary basis, which enables an accurate expansion of the all-electron density in…

Chemical Physics · Physics 2021-11-10 Alan M. Lewis , Andrea Grisafi , Michele Ceriotti , Mariana Rossi

The increasing richness of data related to cold dense matter, from laboratory experiments to neutron-star observations, requires a framework for constraining the properties of such matter that makes use of all relevant information. Here, we…

High Energy Astrophysical Phenomena · Physics 2020-01-08 M. Coleman Miller , Cecilia Chirenti , Frederick K. Lamb

In the elastic scattering regime, probe position-averaged convergent beam electron diffraction (PACBED) patterns have proven robust for estimating specimen thickness and mistilt. Through simulation, we show that core-loss-filtered PACBED…

Other Condensed Matter · Physics 2025-10-27 Michael Deimetry , Timothy C. Petersen , Matthew Weyland , Scott D. Findlay

Determining the spectral density of a molecular system immersed in a proteomic scaffold and in contact to a solvent is a fundamental challenge in the coarse-grained description of, e.g., electron and energy transfer dynamics. Once the…

Quantum Physics · Physics 2014-11-04 Leonardo A. Pachon , Paul Brumer

Photon counting is a cornerstone of quantum optics. Here, we demonstrate precisely counting from 0 to over 9000 photons, beating the Poisson noise limit by at least $4.1~\mathrm{dB}$ across this range. We achieve sub-single-photon precision…

The routine atomic-resolution structure determination of single particles is expected to have profound implications for probing the structure-function relationship in systems ranging from energy materials to biological molecules.…

Single biomolecular imaging using XFEL radiation is an emerging method for protein structure determination using the "diffraction before destruction" method at near atomic resolution. Crucial parameters for such bio-imaging experiments are…

The saturation density of nuclear matter $\rho_0$ is a fundamental nuclear physics property that is difficult to predict from fundamental principles. The saturation density is closely related to the interior density of a heavy nucleus, such…

Nuclear Theory · Physics 2020-10-21 C. J. Horowitz , J. Piekarewicz , Brendan Reed

To operate quantum sensors at their quantum limit in real time, it is crucial to identify efficient data inference tools for rapid parameter estimation. In photodetection, the key challenge is the fast interpretation of click-patterns that…

Quantum Physics · Physics 2026-02-24 Mateusz Molenda , Lewis A. Clark , Marcin Płodzień , Jan Kolodynski

Photon-limited imaging arises when the number of photons collected by a sensor array is small relative to the number of detector elements. Photon limitations are an important concern for many applications such as spectral imaging, night…

Computer Vision and Pattern Recognition · Computer Science 2014-04-29 Joseph Salmon , Zachary Harmany , Charles-Alban Deledalle , Rebecca Willett

The diffraction patterns of crystalline materials with local order contain sharp Bragg reflections as well as highly structured diffuse scattering. The instrumental requirements, experimental parameters and data processing techniques for…

Materials Science · Physics 2023-11-29 Romy Poppe , Joke Hadermann

The development of multi-layer optics which allow to focus photons up to 100 keV and more promises an enormous jump in sensitivity in the hard X-ray energy band. This technology is already planned to be exploited by future missions…

Instrumentation and Methods for Astrophysics · Physics 2015-06-04 Fabio Muleri , Riccardo Campana

Scanning electron microscopy (SEM) has been widely utilized in the field of materials science due to its significant advantages, such as large depth of field, wide field of view, and excellent stereoscopic imaging. However, at high…

AIMS: Clinical radiographic imaging is seated upon the principle of differential keV photon transmission through an object. At clinical x-ray energies the scattering of photons causes signal noise and is utilized solely for transmission…

Medical Physics · Physics 2022-06-22 Ida Häggström , Lukas M. Carter , Thomas J. Fuchs , Adam L. Kesner

The resolution of X-ray diffraction microscopy is limited by the maximum dose that can be delivered prior to sample damage. In the proposed Serial Crystallography method, the damage problem is addressed by distributing the total dose over…

In a previous paper, we outlined a new Bayesian method for inferring the properties of extended gravitational lenses, given data in the form of resolved images. This method holds the most promise for optimally extracting information from…

Astrophysics · Physics 2008-11-26 Brendon J. Brewer , Geraint F. Lewis

In this study, we explore the potential of machine learning for modeling molecular electronic spectral intensities as a continuous function in a given wavelength range. Since presently available chemical space datasets provide excitation…

Chemical Physics · Physics 2022-08-02 Prakriti Kayastha , Sabyasachi Chakraborty , Raghunathan Ramakrishnan

Future ultrafast x-ray light sources might image ultrafast coherent electron motion in real-space and in real-time. For a rigorous understanding of such an imaging experiment, we extend the theory of non-resonant x-ray scattering to the…

Atomic Physics · Physics 2015-06-19 Gopal Dixit , Jan Malte Slowik , Robin Santra