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We present the results of molecular dynamics simulations of SPC/E water confined in a realistic model of a silica pore. The single-particle dynamics have been studied at ambient temperature for different hydration levels. The confinement…

Statistical Mechanics · Physics 2009-10-31 P. Gallo , M. Rovere , M. A. Ricci , C. Hartnig , E. Spohr

A molecular dynamics simulation of water confined in a silica pore is performed in order to compare it with recent experimental results on water confined in porous Vycor glass at room temperature. A cylindrical pore of 40 A is created…

Statistical Mechanics · Physics 2009-10-31 M. Rovere , M. A. Ricci , D. Vellati , F. Bruni

In contrast to the abundance of work on the anomalous behavior of water, the relationship between the water's thermodynamic anomalies and kinetics of phase transition from metastable water is relatively unexplored. In this work, we have…

Soft Condensed Matter · Physics 2022-12-15 Yuvraj Singh , Mantu Santra , Rakesh S. Singh

We investigate mixed (50/50) clusters of parahydrogen and orthodeuterium at low temperature, by means of Quantum Monte Carlo simulations. Our results provide evidence of liquid-like behavior and partial isotopic separation in a cluster of…

Mesoscale and Nanoscale Physics · Physics 2025-03-27 Kiril M. Kolevski , Jie-Ru Hu , Massimo Boninsegni

In simulations of aqueous systems it is common to freeze the bond vibration and angle bending modes in water to allow for a longer time-step $\delta t$ for integrating the equations of motion. Thus $\delta t = 2$ fs is often used in…

Soft Condensed Matter · Physics 2023-08-17 Dilipkumar N. Asthagiri , Thomas L. Beck

The inner crust of neutron stars is supposed to be inhomogeneous and composed of dense structures (clusters) that are immersed in a dilute gas of unbound neutrons. Here we consider spherical clusters forming a BCC crystal and cylindrical…

Nuclear Theory · Physics 2016-12-09 Noël Martin , Michael Urban

The process of homogeneous crystal nucleation has been considered in a model liquid, where the interparticle interaction is described by a short-range spherical oscillatory potential. Mechanisms of initiating structural ordering in the…

Materials Science · Physics 2018-12-18 Bulat N. Galimzyanov , Dinar T. Yarullin , Anatolii V. Mokshin

We perform lengthy molecular dynamics simulations of the SPC/E model of water to investigate the dynamics under pressure at many temperatures and compare with experimental measurements. We calculate the isochrones of the diffusion constant…

Condensed Matter · Physics 2009-10-31 Francis W. Starr , Stephen Harrington , Francesco Sciortino , H. Eugene Stanley

We use molecular dynamics simulations to study the diffusion of water inside deformed carbon nanotubes, with different degrees of eccentricity at 300K. We found a water structural transition between tubular-like to single-file for the (7,7)…

We study conditions under which carbon clusters of different sizes form and stabilize. {We describe an approach to equilibrium by simulating tenuous carbon gas dynamics to long times.} First, we use reactive molecular dynamics simulations…

Astrophysics of Galaxies · Physics 2015-06-18 N. Patra , P. Kral , H. R. Sadeghpour

We examine ice crystal growth from water vapor at temperatures near the melting point, when surface premelting creates a quasiliquid layer at the solid/vapor interface. Recent ice growth measurements as a function of vapor supersaturation…

Materials Science · Physics 2014-07-04 Kenneth G. Libbrecht

Molecular dynamics (MD) simulations of equilibrium structures and flows of polar water, nonpolar argon and methane, and mixtures of water and methane confined by single - walled carbon nanotubes (SWCNTs) with different rectangular cross…

Mesoscale and Nanoscale Physics · Physics 2018-12-27 L. V. Mirantsev , A. K. Abramyan

Confinement can modify the dynamics, the thermodynamics and the structural properties of liquid water, the prototypical anomalous liquid. By considering a general anomalous liquid, suitable for globular proteins, colloids or liquid metals,…

Soft Condensed Matter · Physics 2015-06-19 Fabio Leoni , Giancarlo Franzese

We perform direct large molecular dynamics simulations of homogeneous SPC/E water nucleation, using up to $\sim 4\cdot 10^6$ molecules. Our large system sizes allow us to measure extremely low and accurate nucleation rates, down to $\sim…

Atomic and Molecular Clusters · Physics 2015-09-02 R. Angelil , J. Diemand , K. Tanaka , H. Tanaka

The crystallization of a metastable melt is one of the most important non equilibrium phenomena in condensed matter physics, and hard sphere colloidal model systems have been used for several decades to investigate this process by…

Soft Condensed Matter · Physics 2015-05-20 Tanja Schilling , Sven Dorosz , Hans Joachim Schoepe , George Opletal

Surface tension of small grains and droplets makes them stable only at a much lower temperature than in bulk. This makes spontaneous nucleation unfavorable in many cases. Kinetic approaches are delicate in that one can easily generate…

Statistical Mechanics · Physics 2014-06-03 Clifford Chafin

We have used atomistic molecular dynamics (MD) simulations to study the structure and dynamics of water molecules inside an open ended carbon nanotube placed in a bath of water molecules. The size of the nanotube allows only a single file…

Statistical Mechanics · Physics 2007-12-20 Biswaroop Mukherjee , Prabal K. Maiti , Chandan Dasgupta , A. K. Sood

NaCl crystal nucleation from metastable solutions has long been considered to occur according to a single-step mechanism. Recent experimental observations suggest that NaCl crystals emerge from disordered intermediates which is seemingly at…

Materials Science · Physics 2022-10-12 Aaron R. Finney , Matteo Salvalaglio

As one of the most fascinating confined water/ice phenomena, two-dimensional square ice has been extensively studied and experimentally confirmed in recent years. Apart from the unidirectional homogeneous square icing patterns considered in…

Fluid Dynamics · Physics 2023-01-18 Zhen Zeng , Tianyou Wang , Rui Chen , Mengshan Suo , Kai Sun , Panagiotis E. Theodorakis , Zhizhao Che

The phase behaviour and dynamics of molecular ionic liquids are studied using primitive models and extensive computer simulations. The models account for size disparity between cation and anion, charge location on the cation, and…

Soft Condensed Matter · Physics 2012-02-23 G. C. Ganzenmüller , P. J. Camp
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