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We report a detailed experimental and theoretical study on the effect of hydrostatic pressure on the structural and magnetic aspects of the layered honeycomb antiferromagent $\alpha$-RuCl$_{3}$. Magnetic susceptibility measurements…

A pressure-induced collapse of magnetic ordering in $\beta$-Li$_2$IrO$_3$ at $P_m\sim1.5- 2$ GPa has previously been interpreted as evidence for possible emergence of spin liquid states in this hyperhoneycomb iridate, raising prospects for…

We report the discovery of an intriguing pressure-driven phase transformation in the layered Kitaev-material $\alpha$-RuCl$_3$. By analyzing both the Bragg scattering as well as the diffuse scattering of high-quality single crystals, we…

Strongly Correlated Electrons · Physics 2022-09-20 Quirin Stahl , Tobias Ritschel , Gaston Garbarino , Frederico Cova , Anna Isaeva , Thomas Doert , Jochen Geck

We present high-pressure (2 GPa) $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyper-honeycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. The spectra show evidence for a structural phase transition around 200 K…

Strongly Correlated Electrons · Physics 2025-12-16 Aimé Verrier , Vikram Nagarajan , Louis-Thomas Gendron , James G. Analytis , Jeffrey A. Quilliam

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

$\mathrm{Cu_2IrO_3}$ is among the newest layered honeycomb iridates and a promising candidate to harbor a Kitaev quantum spin liquid state. Here, we investigate the pressure and temperature dependence of its structure through a combination…

Strongly Correlated Electrons · Physics 2021-07-14 G. Fabbris , A. Thorn , W. Bi , M. Abramchuk , F. Bahrami , J. H. Kim , T. Shinmei , T. Irifune , F. Tafti , A. N. Kolmogorov , D. Haskel

We investigate the effects of hydrostatic pressure on $\alpha$-RuCl$_3$, a prototypical material for the Kitaev spin model on a honeycomb lattice with a possible spin-liquid ground state. Using ultrasound measurements at pressures up to…

Strongly Correlated Electrons · Physics 2025-03-07 A. Hauspurg , Susmita Singh , T. Yanagisawa , V. Tsurkan , J. Wosnitza , Wolfram Brenig , Natalia B. Perkins , S. Zherlitsyn

We report a comprehensive single-crystal neutron diffraction investigation of the Kitaev quantum magnet $\alpha$-RuCl$_{3}$ under hydrostatic pressure. Utilizing a He-gas pressure cell, we successfully applied an ideal hydrostatic pressure…

Strongly Correlated Electrons · Physics 2023-04-04 Xiao Wang , Fengfeng Zhu , Navid Qureshi , Ketty Beauvois , Junda Song , Thomas Mueller , Thomas Brückel , Yixi Su

Magnetization and high-resolution x-ray diffraction measurements of the Kitaev-Heisenberg material alpha-RuCl3 reveal a pressure-induced crystallographic and magnetic phase transition at a hydrostatic pressure of p=0.2 GPa. This structural…

We use magnetization measurements under pressure along with \textit{ab initio} and cluster many-body calculations to investigate magnetism of the Kitaev candidate Li$_2$RhO$_3$. Hydrostatic compression leads to a decrease in the magnitude…

ErAl$_3$ can form in either a trigonal ($\alpha$) or cubic ($\beta$) polymorph and this paper investigates the physical properties of these polymorphs through characterizations of single crystals grown in an aluminum flux. We demonstrate…

Strongly Correlated Electrons · Physics 2025-07-15 Karolina Gornicka , Brenden R. Ortiz , Andrew D. Christianson , Andrew F. May

Thermodynamics of the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ is studied for different directions of in-plane magnetic field using measurements of the magnetic Gr\"uneisen parameter $\Gamma_B$ and specific heat $C$. We identify two…

Strongly Correlated Electrons · Physics 2021-03-03 S. Bachus , D. A. S. Kaib , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valentí , P. Gegenwart

Single-crystal x-ray diffraction studies with synchrotron radiation on the honeycomb iridate $\alpha$-Li$_{2}$IrO$_{3}$ reveal a pressure-induced structural phase transition with symmetry lowering from monoclinic to triclinic at a critical…

Hydrostatic pressure effects on the temperature- and magnetic field dependencies of the in-plane and out-of-plane magnetization of the bi-layered perovskite Sr3Ru2O7 have been studied by SQUID magnetometer measurements under a hydrostatic…

Materials Science · Physics 2009-11-10 Yuri V. Sushko , Bruno DeHarak , Gang Cao , G. Shaw , D. K. Powell , J. W. Brill

We present magnetization measurements carried out on polycrystalline and single-crystalline samples of $\alpha$-Li$_2$IrO$_3$ under hydrostatic pressures up to 2 GPa and establish the temperature-pressure phase diagram of this material. The…

The honeycomb antiferromagnet BaCo2(AsO4)2, in which small in-plane magnetic fields (H1 = 0.26 T and H2 = 0.52 T at T = 1.8 K < TN = 5.4 K) induce two magnetic phase transitions, has attracted attention as a possible candidate material for…

Strongly Correlated Electrons · Physics 2022-06-15 Shuyuan Huyan , Juan Schmidt , Elena Gati , Ruidan Zhong , Robert J. Cava , Paul C. Canfield , Sergey L. Bud'ko

We have investigated the magnetic properties of highly anisotropic layered ferromagnetic semiconductor CrI$_3$ in presence of hydrostatic pressure ($P$). At ambient pressure, magnetization exhibits a clear anomaly below 212 K along with a…

The layered honeycomb lattice iridate Cu$_2$IrO$_3$ is the closest realization of the Kitaev quantum spin liquid, primarily due to the enhanced interlayer separation and nearly ideal honeycomb lattice. We report pressure-induced structural…

Raman scattering has been employed to investigate lattice and magnetic excitations of the honeycomb Kitaev material $\alpha$-RuCl$_3$ and its Heisenberg counterpart CrCl$_3$. Our phonon Raman spectra give evidence for a first-order…

Strongly Correlated Electrons · Physics 2017-06-07 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Kwon , K. -Y. Choi

Temperature-pressure phase diagram of the Kitaev hyperhoneycomb iridate $\beta$-Li$_2$IrO$_3$ is explored using magnetization, thermal expansion, magnetostriction, and muon spin rotation ($\mu$SR) measurements, as well as single-crystal…

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