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In this paper, an exact analytical solution is presented for achieving coherent population transfer and creating arbitrary coherent superposition states in a five-state chainwise system by a train of coincident pulses. We show that the…

Quantum Physics · Physics 2024-08-21 Jiahui Zhang

Stimulated Raman Adiabatic Passage (STIRAP) and its variants, such as multi-state chainwise-STIRAP allow efficiently transferring the populations in multi-state system and have been widely used to prepare ultracold deeply-bound molecules.…

Quantum Physics · Physics 2024-07-30 Jiahui Zhang

We suggest and analyze a novel technique for efficient and robust creation of dense ultracold molecular ensembles in their ground rovibrational state. In our approach a molecule is brought to the ground state through a series of…

Quantum Physics · Physics 2009-11-13 Elena Kuznetsova , Philippe Pellegrini , Robin Côté , M. D. Lukin , S. F. Yelin

We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and…

Quantum Physics · Physics 2011-11-18 Amarendra K. Sarma , Parvendra Kumar

We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…

Atomic Physics · Physics 2026-01-14 Emanuel F. de Lima

Optical Feshbach resonances [Phys. Rev. Lett. 94, 193001 (2005)] and pump-dump photoassociation with short laser pulses [Phys. Rev. A 73, 033408 (2006)] have been proposed as means to coherently form stable ultracold alkali dimer molecules.…

Atomic Physics · Physics 2009-01-05 Christiane P. Koch

We propose to create ultracold ground state molecules in an atomic Bose-Einstein condensate by adiabatic crossing of an optical Feshbach resonance. We envision a scheme where the laser intensity and possibly also frequency are linearly…

Quantum Physics · Physics 2007-05-23 Christiane P. Koch Françoise Masnou-Seeuws Ronnie Kosloff

We present a method for the creation and control of cold molecules that involves coherently combining Feshbach Resonances and STIRAP. We present analytical and numerical results showing how to optimize this process that can be implemented…

Atomic Physics · Physics 2019-10-09 Phillip Price , Susanne Yelin

Chainwise stimulated Raman adiabatic passage (C-STIRAP) in M-type molecular system is a good alternative in creating ultracold deeply-bound molecules when the typical STIRAP in {\Lambda}-type system does not work due to weak Frank-Condon…

Quantum Physics · Physics 2024-08-06 Jiahui Zhang , Li Deng , Yueping Niu , Shangqing Gong

We investigate pump-dump photoassociation of ultracold molecules with amplitude- and phase-modulated femtosecond laser pulses. For this purpose a perturbative model for the light-matter interaction is developed and combined with a genetic…

A technique for complete population transfer between the two end states $\ket{1}$ and $\ket{3}$ of a three-state quantum system with a train of $N$ pairs of resonant and coincident pump and Stokes pulses is introduced. A simple analytic…

Quantum Physics · Physics 2015-06-03 Andon A. Rangelov , Nikolay V. Vitanov

We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice…

Photoassociation of two ultracold rubidium atoms and the subsequent formation of stable molecules in the singlet ground and lowest triplet states is investigated theoretically. The method employs laser pulses inducing transitions via…

Atomic Physics · Physics 2007-05-23 Christiane P. Koch , Ronnie Kosloff , Françoise Masnou-Seeuws

In this work we analyse the structure of highly-entangled multimode squeezed states, such as those generated by broadband pulses undergoing type-II parametric down-conversion (PDC). Such down-conversion has previously been touted as a…

Quantum Physics · Physics 2018-01-03 Nedasadat Hosseinidehaj , Robert Malaney

We create an ultracold dense quantum gas of ground state molecules bound by more than 1000 wavenumbers by stimulated two-photon transfer of molecules associated on a Feshbach resonance from a Bose-Einstein condensate of cesium atoms. The…

This theoretical paper investigates the formation of ground state molecules from ultracold cesium atoms in a two-color scheme. Following previous work on photoassociation with chirped picosecond pulses [Luc-Koenig et al., Phys. Rev. A {\bf…

Atomic Physics · Physics 2007-05-23 Christiane P. Koch , Eliane Luc-Koenig , Françoise Masnou-Seeuws

This work presents a method for achieving complete, robust, and efficient population transfer between the two ground states in a three-level loop quantum system. The approach utilizes composite pulse sequences by effectively mapping the…

Quantum Physics · Physics 2025-04-09 Peter Chernev , Andon A. Rangelov

Using a non-selective broadband detection scheme we discovered an efficient mechanism of formation of ultracold Cs$_2$ molecules in deeply bound levels ($v=1-9$) of their electronic ground state X$^1 \Sigma_g^+$. They are formed by a…

In this work, we propose a composite pulses scheme by modulating phases to achieve high fidelity population transfer in three-level systems. To circumvent the obstacle that not enough variables are exploited to eliminate the systematic…

Quantum Physics · Physics 2022-02-17 Zhi-Cheng Shi , Cheng Zhang , Du Ran , Yan Xia , Reuven Ianconescu , Aharon Friedman , X. X. Yi , Shi-Biao Zheng

Recently, the quest for an ultracold and dense ensemble of polar molecules has attracted strong interest. Polar molecules have bright prospects for novel quantum gases with long-range and anisotropic interactions, for quantum information…

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