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A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

We numerically study models of $\mathrm{H}_2$ and $\mathrm{LiH}$ molecules, aligned collinearly with the linear polarization of the external field, to elucidate the possible role of correlation in the enhanced-ionization phenomena.…

Atomic Physics · Physics 2016-01-06 S. Chattopadhyay , S. Bauch , L. B. Madsen

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

We investigate electron correlation effects in internuclear-distance-dependent enhanced ionization of $\mathrm{H}_2$, $\mathrm{LiH}$, and $\mathrm{HF}$ molecules by intense near-infrared laser pulses using a 3D description of the systems…

Atomic Physics · Physics 2019-02-27 Siddhartha Chattopadhyay , Lars Bojer Madsen

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…

Atomic Physics · Physics 2020-09-30 Stefan Donsa , Manuel Ederer , Renate Pazourek , Joachim Burgdörfer , Iva Březinová

We explore the relationship between symmetrisation and entanglement through measurements on few-particle systems in a multi-well potential. In particular, considering two or three trapped atoms, we measure and distinguish correlations…

We illustrate how attosecond light pulses can be used to directly mapping out the time-dependence of the correlated motion of two excited atomic electrons, discuss how the two-electron correlations manifest themselves in realistic…

Atomic Physics · Physics 2007-05-23 Toru Morishita , Shinichi Watanabe , C. D. Lin

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

A theoretical investigation of the radiative capture of an electron into a bound state of heavy, hydrogen-like ion is presented. Special attention is paid to the question of how the linear polarization of the emitted radiation is affected…

Atomic Physics · Physics 2015-05-28 A. Surzhykov , A. N. Artemyev , V. A. Yerokhin

We study the impact of competing time delays in coupled stochastic synchronization and coordination problems. We consider two types of delays: transmission delays between interacting elements and processing, cognitive, or execution delays…

Statistical Mechanics · Physics 2011-01-12 D. Hunt , G. Korniss , B. K. Szymanski

We apply a three-dimensional (3D) implementation of the time-dependent restricted-active-space self-consistent-field (TD-RASSCF) method to investigate effects of electron correlation in the ground state of Be as well as in its…

Atomic Physics · Physics 2017-06-07 Juan J. Omiste , Wenliang Li , Lars Bojer Madsen

We analyse the influence of entanglement on the emission properties of atoms. To this end, first, we propose a scheme for the preparation of a pair of entangled Helium atoms, one in the ortho and the other in the para spin configuration. We…

Quantum Physics · Physics 2009-07-07 Pedro Sancho , Luis Plaja

We investigate the effects of heterogeneous delays in the coupling of two excitable neural systems. Depending upon the coupling strengths and the time delays in the mutual and self-coupling, the compound system exhibits different types of…

Adaptation and Self-Organizing Systems · Physics 2015-06-05 Anastasiia Panchuk , David P. Rosin , Philipp Hövel , Eckehard Schöll

We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shake-up of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond…

Atomic Physics · Physics 2013-05-24 Renate Pazourek , Stefan Nagele , Johannes Feist , Joachim Burgdörfer

We study numerically stabilization against ionization of a fully correlated two-electron model atom in an intense laser pulse. We concentrate on two frequency regimes: very high frequency, where the photon energy exceeds both, the…

Atomic Physics · Physics 2009-10-31 D. Bauer , F. Ceccherini

Attosecond photoionization delays have mostly been interpreted within the single-particle approximation of multi-electron systems. The strong electron correlation between the photoionization channels associated with the 3p and 3s orbitals…

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

Atomic Physics · Physics 2015-06-19 J. M. Dahlström , E. Lindroth
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