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We present a scalable machine learning (ML) framework for large-scale kinetic Monte Carlo (kMC) simulations of itinerant electron Ising systems. As the effective interactions between Ising spins in such itinerant magnets are mediated by…

Statistical Mechanics · Physics 2024-12-02 Alexa Tyberg , Yunhao Fan , Gia-Wei Chern

The paper studies spin-orbit interaction (i.e. the effect the spin has on the particle's trajectory in a magnetic field) as a model of quantum computation. The two-level spin quantum system is examined using the stochastic mechanics…

Mathematical Physics · Physics 2011-02-11 Gerasimos G. Rigatos

Vibrational properties of solids are key to determining stability, response and functionality. However, they are challenging to computationally predict at Ab-Initio accuracy, even for elemental systems. Ab-Initio methods for modeling atomic…

Materials Science · Physics 2024-06-25 Mgcini Keith Phuthi , Yang Huang , Michael Widom , Venkatasubramanian Viswanathan

We propose a method for the evaluation of magnetic exchange couplings based on noncollinear spin-density functional calculations. The method employs the second derivative of the total Kohn-Sham energy of a single reference state, in…

Materials Science · Physics 2009-11-13 Juan E. Peralta , Veronica Barone

In recent years, significant progress has been made in the development of machine learning potentials (MLPs) for atomistic simulations with applications in many fields from chemistry to materials science. While most current MLPs are based…

Chemical Physics · Physics 2023-05-19 Tsz Wai Ko , Jonas A. Finkler , Stefan Goedecker , Jörg Behler

Building upon the worldline effective field theory (EFT) formalism for spinning bodies developed for the Post-Newtonian regime, we generalize the EFT approach to Post-Minkowskian (PM) dynamics to include rotational degrees of freedom in a…

High Energy Physics - Theory · Physics 2022-05-30 Zhengwen Liu , Rafael A. Porto , Zixin Yang

Electric fields represent an ideal means for controlling spins at the nanoscale and, more specifically, for manipulating protected degrees of freedom in multispin systems. Here we perform low-temperature magnetic far-IR spectroscopy on a…

Mesoscale and Nanoscale Physics · Physics 2025-02-03 Florian le Mardelé , Ivan Mohelský , Jan Wyzula , Milan Orlita , Philippe Turek , Filippo Troiani , Athanassios K. Boudalis

Quantum spin models with a large number of interaction partners per spin are frequently used to describe modern many-body quantum optical systems like arrays of Rydberg atoms, atom-cavity systems or trapped ion crystals. For theoretical…

Quantum Gases · Physics 2024-12-03 Benedikt Schneider , Ruben Burkard , Beatriz Olmos , Igor Lesanovsky , Björn Sbierski

Physics-based, atom-centered machine learning (ML) representations have been instrumental to the effective integration of ML within the atomistic simulation community. Many of these representations build off the idea of atoms as having…

Computational Physics · Physics 2024-03-29 Arthur Y. Lin , Kevin K. Huguenin-Dumittan , Yong-Cheol Cho , Jigyasa Nigam , Rose K. Cersonsky

Machine Learning (ML) techniques are revolutionizing the way to perform efficient materials modeling. Nevertheless, not all the ML approaches allow for the understanding of microscopic mechanisms at play in different phenomena. To address…

Materials Science · Physics 2022-06-22 Udaykumar Gajera , Loriano Storchi , Danila Amoroso , Francesco Delodovici , Silvia Picozzi

Many rotational invariants for crystal structure representations have been used to describe the structure-property relationship by machine learning. The machine learning interatomic potential (MLIP) is one of the applications of rotational…

Computational Physics · Physics 2019-07-03 Atsuto Seko , Atsushi Togo , Isao Tanaka

We investigate the dynamical and steady-state spin response of the nonequilibrium Anderson model to magnetic fields, bias voltage, and temperature using a numerically exact method combining a bold-line quantum Monte Carlo technique with the…

Strongly Correlated Electrons · Physics 2013-05-14 Guy Cohen , Emanuel Gull , David R. Reichman , Andrew J. Millis , Eran Rabani

In spin-crossover materials, the volume of a molecule changes depending on whether it is in the high-spin (HS) or low-spin (LS) state. This change causes distortion of the lattice. Elastic interactions among these distortions play an…

Materials Science · Physics 2009-11-13 Seiji Miyashita , Yusuké Konishi , Masamichi Nishino , Hiroko Tokoro , Per Arne Rikvold

We develop a method to estimate the spin-spin interactions in the Hamiltonian from the observed magnetization curve by machine learning based on Bayesian inference. In our method, plausible spin-spin interactions are determined by…

Statistical Mechanics · Physics 2018-03-08 Ryo Tamura , Koji Hukushima

In order to derive tensorial exchange interactions and local magnetic anisotropies in itinerant magnetic systems, an approach combining the Spin-Cluster Expansion with the Relativistic Disordered Local Moment scheme is introduced. The…

Strongly Correlated Electrons · Physics 2015-05-20 L. Szunyogh , L. Udvardi , J. Jackson , U. Nowak , R. Chantrell

The use of machine learning (ML) in chemical physics has enabled the construction of interatomic potentials having the accuracy of ab initio methods and a computational cost comparable to that of classical force fields. Training an ML model…

Chemical Physics · Physics 2023-06-21 Zeyuan Tang , Stefan T. Bromley , Bjørk Hammer

We derive an explicit matrix representation for the Hamiltonian of the Ising model in mutually orthogonal external magnetic fields, using as basis the eigenstates of a system of non-interacting \mbox{spin~$1/2$} particles in external…

We investigate the efficiency of the recently proposed Restricted Boltzmann Machine (RBM) representation of quantum many-body states to study both the static properties and quantum spin dynamics in the two-dimensional Heisenberg model on a…

Strongly Correlated Electrons · Physics 2019-07-10 G. Fabiani , J. H. Mentink

In spite of decades of research, much remains to be discovered about folding: the detailed structure of the initial (unfolded) state, vestigial folding instructions remaining only in the unfolded state, the interaction of the molecule with…

Biological Physics · Physics 2018-11-26 Walter A. Simmons

Atomistic modeling is a widely employed theoretical method of computational materials science. It has found particular utility in the study of magnetic materials. Initially, magnetic empirical interatomic potentials or spin-polarized…

Atomic Physics · Physics 2024-07-02 Tatiana S. Kostiuchenko , Alexander V. Shapeev , Ivan S. Novikov