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High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

We study the effect of electron-electron correlations on the quantum state of the light emitted from high-harmonic generation (HHG). The quantum state of the emitted light is obtained by using a fully quantum mechanical description of both…

Quantum Physics · Physics 2024-03-19 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

By employing the exact diagonalization method, we investigate the high-harmonic generation (HHG) of the correlated systems under the strong laser irradiation. For the extended Hubbard model on a periodic chain, HHG close to the quantum…

Strongly Correlated Electrons · Physics 2022-03-07 Can Shao , Hantao Lu , Xiao Zhang , Chao Yu , Takami Tohyama , Ruifeng Lu

Using Floquet theory and the hierarchy of correlations, we study the non-equilibrium dynamics of the Mott insulator state in the Fermi-Hubbard model under the influence of a harmonically oscillating electric field representing the pump…

Strongly Correlated Electrons · Physics 2023-09-06 Friedemann Queisser , Ralf Schützhold

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

High harmonic generation (HHG) is a highly nonlinear emission process in which systems driven by intense laser pulses emit integer multiples (harmonics) of the driving field. This feature is considered universal to all occurrences of HHG.…

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

Other Condensed Matter · Physics 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm

We show that the Floquet approach with a Sturmian basis means an efficient description of high-order harmonic generation with monochromatic excitation. This method, although involves numerical calculations, is close to analytic approaches…

Atomic Physics · Physics 2017-11-30 Jozsef Kasza Peter Dombi , Peter Foldi

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

Optics · Physics 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

Recent developments on intense laser sources is opening a new field of optical sciences. An intense coherent light beam strongly interacting with the matter causes a coherent motion of a particle, forming a strongly dressed excited…

Quantum Physics · Physics 2017-10-23 Hidemasa Yamane , Satoshi Tanaka , Michelangelo Domina , Roberto Passante , Tomio Petrosky

We demonstrate that high-harmonic generation (HHG) in solids dominantly originates from strongly localized surface states through non-perturbative processes. Measurements reveal that HHG from bulk states is suppressed by at least 1-2 orders…

Optics · Physics 2018-05-02 J. Seres , E. Seres , C. Serrat , T. Schumm

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

We studied the multi-plateau high-order harmonic generation (HHG) from solids numerically. It is found that the HHG spectrum in the second or higher plateau is redshifted in short laser pulses due to the nonadiabatic effect. The…

Optics · Physics 2017-09-20 Guang-Rui Jia , Xue-Bin Bian

We present Floquet calculations of high harmonic generation (HHG) for the lowest two electronic states of the $\mbox{H}_2^+$ ion by strong continuous-wave laser fields. We solve the non-Hermitian matrix problem to get accurate solutions to…

Atomic Physics · Physics 2015-06-18 Ts Tsogbayar , M Horbatsch

An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…

Optics · Physics 2026-01-01 A. V. Flegel , Liang-Wen Pi , M. V. Frolov
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