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The description of excited state dynamics in multichromophoric systems constitutes both a theoretical and experimental challenge in modern physical chemistry. An experimental protocol which can systematically characterize both coherent and…

Quantum Physics · Physics 2011-10-31 Joel Yuen-Zhou , Jacob J. Krich , Masoud Mohseni , Alán Aspuru-Guzik

Transmon qubits are a cornerstone of modern superconducting quantum computing platforms. Temporal fluctuations of energy relaxation in these qubits are widely attributed to microscopic two-level systems (TLSs) in device dielectrics and…

The physics of a single Josephson junction coupled to a resistive environment is a long-standing fundamental problem at the center of an intense debate, strongly revived by the advent of superconducting platforms with high-impedance…

Quantum Physics · Physics 2025-04-22 Luca Giacomelli , Cristiano Ciuti

Excited states of many-body quantum systems play a key role in a wide range of physical and chemical phenomena. Unlike ground states, for which many efficient variational techniques exist, there are few ways to systematically construct…

Quantum Physics · Physics 2025-08-04 D. A. Millar , L. W. Anderson , E. Altamura , O. Wallis , M. E. Sahin , J. Crain , S. J. Thomson

The recent developments of quantum computing present potential novel pathways for quantum chemistry, as the increased computational power of quantum computers could be harnessed to naturally encode and solve electronic structure problems.…

Quantum Physics · Physics 2024-03-01 Lila Cadi Tazi , Alex J. W. Thom

Quantum computers promise to efficiently solve important problems that are intractable on a conventional computer. For quantum systems, where the dimension of the problem space grows exponentially, finding the eigenvalues of certain…

Quantum phase transitions occur when the ground state of a quantum system undergoes a qualitative change when an external control parameter reaches a critical value. Here, we demonstrate a technique for studying quantum systems undergoing a…

Quantum Physics · Physics 2008-03-14 Jingfu Zhang , Xinhua Peng , Nageswaran Rajendran , Dieter Suter

The new integrable quantum spin model is proposed. The model has a biaxial magnetic anisotropy of alternating coupling between spins together with multiple spin interactions. Our model gives the possibility to exactly find thermodynamic…

Strongly Correlated Electrons · Physics 2015-05-19 A. A. Zvyagin

We study the structure of the eigenstates and the dynamics of a system that undergoes an excited state quantum phase transition (ESQPT). The analysis is performed for two-level pairing models characterized by a U(n+1) algebraic structure.…

Statistical Mechanics · Physics 2015-12-02 Lea F. Santos , Francisco Pérez-Bernal

We study the quantum phase transitions of a model that describes the interconversion of interacting bosonic atoms and molecules. Using a classical analysis, we identify a threshold coupling line separating a molecular phase and a mixed…

Quantum Gases · Physics 2010-07-07 Gilberto Santos , Angela Foerster , Jon Links , Eduardo Mattei , Silvio R. Dahmen

The efficient calculation of Hamiltonian spectra, a problem often intractable on classical machines, can find application in many fields, from physics to chemistry. Here, we introduce the concept of an "eigenstate witness" and through it…

We study a three-mode Hamiltonian modelling a heteronuclear molecular Bose--Einstein condensate. Two modes are associated with two distinguishable atomic constituents, which can combine to form a molecule represented by the third mode.…

The variational quantum eigensolver (VQE) is one of the most promising algorithms to find eigenvalues and eigenvectors of a given Hamiltonian on noisy intermediate-scale quantum (NISQ) devices. A particular application is to obtain ground…

The study of quantum phase transitions requires the preparation of a many-body system near its ground state, a challenging task for many experimental systems. The measurement of quench dynamics, on the other hand, is now a routine practice…

Quantum Physics · Physics 2019-09-13 Paraj Titum , Joseph T. Iosue , James R. Garrison , Alexey V. Gorshkov , Zhe-Xuan Gong

The variational approach is a cornerstone of computational physics, considering both conventional and quantum computing computational platforms. The variational quantum eigensolver (VQE) algorithm aims to prepare the ground state of a…

Quantum Physics · Physics 2022-12-16 Nikita Astrakhantsev , Guglielmo Mazzola , Ivano Tavernelli , Giuseppe Carleo

We present a variational quantum thermalizer (VQT), called quantum-VQT (qVQT), which extends the variational quantum eigensolver (VQE) to finite temperatures. The qVQT makes use of an intermediate measurement between two variational…

Quantum Physics · Physics 2024-06-05 Johannes Selisko , Maximilian Amsler , Thomas Hammerschmidt , Ralf Drautz , Thomas Eckl

We study the evolution of a V-type three-level system, whose two resonances are coherently excited and coupled by two ultrashort laser pump and probe pulses, separated by a varying time delay. We relate the quantum dynamics of the excited…

Atomic Physics · Physics 2015-04-02 Z. Liu , S. M. Cavaletto , C. Ott , K. Meyer , Y. Mi , Z. Harman , C. H. Keitel , T. Pfeifer

Non-equilibrium quantum many-body systems, which are difficult to study via classical computation, have attracted wide interest. Quantum simulation can provide insights into these problems. Here, using a programmable quantum simulator with…

Accurately solving the Schr\"odinger equation remains a central challenge in computational physics, chemistry, and materials science. Here, we propose an alternative eigenvalue problem based on a system's autocorrelation function, avoiding…

Quantum Physics · Physics 2025-07-22 Timothy Stroschein , Davide Castaldo , Markus Reiher

Quantum phase transitions occur at zero temperature, when the ground state of a Hamiltonian undergoes a qualitative change as a function of a control parameter. We consider a particularly interesting system with competing one-, two- and…

Quantum Physics · Physics 2010-03-05 Xinhua Peng , Jingfu Zhang , Jiangfeng Du , Dieter Suter
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